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Register a new userDouble pair breaking peak in Raman scattering spectra of triple layer cuprate Bi2223
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We report the Raman scattering measurements on the triple layer Bi2Sr2Ca2Cu3O10 (Bi2223) crystals of four different doping levels from slightly overdoped to strongly underdoped regimes. We observed a double pair-breaking peak in the antinodal B1g configuration that we attribute to the two antinodal gaps opening on the outer and inner CuO2-plane (OP and IP) band, respectively. The doping dependence of the pair-breaking peak energy was investigated. Considering the difference in doping level between the IP and OP, all the B1g pair-breaking peak energies for OP and IP were found to align on a single line as a function of doping, which is consistent with the previous results on the double and mono-layer cuprates. Within our experimental accuracy the IP and OP peaks start to appear almost at the same temperature. These findings suggest some sort of interaction between the layers. The observed gap energy is very large, not scaling with Tc.
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We performed Raman experiments on superconducting ${rm Bi_2 Sr_2 (Ca_{1-x} Y_x) Cu_2 O_{8+delta}}$ (Bi-2212) and ${rm YBa_{2} Cu_{3}O_{6+x}}$ (Y-123) single crystals. These results in combination with earlier ones enable us to analyze systematically the spectral features in the doping range $0.07 le p le 0.23$. In $B_{2g}$ ($xy$) symmetry we find universal spectra and the maximal gap energy $Delta_0$ to follow the superconducting transition temperature $T_c$. The $B_{1g}$ ($x^2-y^2$) spectra in Bi-2212 show an anomalous increase of the intensity towards overdoping, indicating that the corresponding energy scale is neither related to the pairing energy nor to the pseudogap, but possibly stems from a symmetry breaking transition at the onset point of superconductivity at $p_{rm sc2} simeq 0.27$.
Checkerboard patterns have been proposed in order to explain STM experiments on the cuprates BSCCO and Na-CCOC. However the presence of these patterns has not been confirmed by a bulk probe such as neutron scattering. In particular, simple checkerboard patterns are inconsistent with neutron scattering data, in that they have low energy incommsensurate (IC) spin peaks rotated 45 degrees from the direction of the charge IC peaks. However, it is unclear whether other checkerboard patterns can solve the problem. In this paper, we have studied more complicated checkerboard patterns (modulated checkerboards) by using spin wave theory and analyzed noncollinear checkerboards as well. We find that the high energy response of the modulated checkerboards is inconsistent with neutron scattering results, since they fail to exhibit a resonance peak at (pi,pi), which has recently been shown to be a universal feature of cuprate superconductors. We further argue that the newly proposed noncollinear checkerboard also lacks a resonance peak. We thus conclude that to date no checkerboard pattern has been proposed which satisfies both the low energy constraints and the high energy constraints imposed by the current body of experimental data in cuprate superconductors.
Electronic Raman scattering with in and out of (ab) plane polarizations have been performed on HgBa2Ca2Cu3O8+d in a slightly underdoped single crystal with a critical temperature Tc=122 K. We find that the d-wave pairing gap at the antinodes is higher in energy (14 kBTc) than in other cuprates and that it varies very slowly up to Tc. This hints at a strong coupling nature of the pairing mechanism. Interestingly, we reveal that the pairing-gap feature in the Raman response displays a complex peak-dip-hump structure, in a fashion reminiscent of what observed by angle resolved photo-emission spectroscopy in Bi2Sr2CaCu2O8+d (Bi-2212). We detect two other distinct superconducting peaks at 5kBTc and 7kBTc when probing respectively around the nodes and on the whole Fermi surface. Finally we establish that the pairing gap at the antinodes is detected both for (ab) plane and for c-axis light polarizations. This shows that the quasiparticle dynamics along the c-axis is intimately connected to the antinodal one in the (ab) plane.
The recently deduced normal and anomalous self-energies from photoemission spectra of cuprate superconductors via the machine learning technique are calling for an explanation. Here the normal and anomalous self-energies in cuprate superconductors are analyzed within the framework of the kinetic-energy-driven superconductivity. It is shown that the exchanged spin excitations give rise to the well-pronounced low-energy peak-structures in both the normal and anomalous self-energies, however, they do not cancel in the total self-energy. In particular, the peak-structure in the normal self-energy is mainly responsible for the peak-dip-hump structure in the single-particle excitation spectrum, and can persist into the normal-state, while the sharp peak in the anomalous self-energy gives rise to a crucial contribution to the superconducting gap, and vanishes in the normal-state. Moreover, the evolution of the peak-structure with doping and momentum are also analyzed.
The key ingredients in any superconductor are the Cooper pairs, in which two electrons combine to form a composite boson. In all conventional superconductors the pairing strength alone sets the majority of the physical properties including the superconducting transition temperature T$_c$. In the cuprate high temperature superconductors, no such link has yet been found between the pairing interactions and T$_c$. Using a new variant of photoelectron spectroscopy we measure both the pair-forming ($Delta$) and a self energy/pair-breaking term ($Gamma_s$) as a function of sample type and sample temperature, and we make the measurements over a wide range of doping and temperatures within and outside of the pseudogap/competing order doping regimes. In all cases we find that T$_c$ is approximately set by a crossover between the pair-forming strength $Delta$ and 3 times the self-energy term $Gamma_s$ - a new paradigm for superconductivity. In addition to departing from conventional superconductivity in which the pairing alone sets T$_c$, these results indicate the zero-order importance of the near-nodal self-energy effects compared to competing order/pseudogap effects.
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