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Phase separation and proximity effects in itinerant ferromagnet-superconductor heterostructures

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 Added by Andreas Bill
 Publication date 2018
  fields Physics
and research's language is English




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Heterostructures made of itinerant ferromagnets and superconductors are studied. In contrast to most previous models, ferromagnetism is not enforced as an external Zeeman field but induced in a correlated single-band model (CSBM) that displays itinerant ferromagnetism as a mean-field ground state. This allows us to investigate the influence of an adjacent superconducting layer on the properties of the ferromagnet in a self-consistent Bogoliubov-de Gennes approach. The CSBM displays a variety features not present in the Zeeman exchange model that influence the behavior of order parameters close to the interface, as e.g. phase separation and the competition between magnetism and superconducting orders.



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We review the present status of the experimental and theoretical research on the proximity effect in heterostructures composed of superconducting (S) and ferromagnetic (F) thin films. First, we discuss traditional effects originating from the oscillatory behavior of the superconducting pair wave function in the F-layer. Then, we concentrate on recent theoretical predictions for S/F layer systems. These are a) generation of odd triplet superconductivity in the F-layer and b) ferromagnetism induced in the S-layer below the superconducting transition temperature $T_{c}$ (inverse proximity effect). The second part of the review is devoted to discussion of experiments relevant to the theoretical predictions of the first part. In particular, we present results of measurements of the critical temperature $T_{c}$ as a function of the thickness of F-layers and we review experiments indicating existence of odd triplet superconductivity, cryptoferromagnetism and inverse proximity effect.
We report an investigation of the structural and electronic properties of hybrid superconductor/ferromagnet (S/F) bilayers of composition Nb/Cu$_{60}$Ni$_{40}$ prepared by magnetron sputtering. X-ray and neutron reflectometry show that both the overall interfacial roughness and vertical correlations of the roughness of different interfaces are lower for heterostructures deposited on Al$_2$O$_3$(1$bar{1}$02) substrates than for those deposited on Si(111). Mutual inductance experiments were then used to study the influence of the interfacial roughness on the superconducting transition temperature, $T_C$. These measurements revealed a $sim$ 4% higher $T_C$ in heterostructures deposited on Al$_2$O$_3$, compared to those on Si. We attribute this effect to a higher mean-free path of electrons in the S layer, caused by a suppression of diffusive scattering at the interfaces. However, the dependence of the $T_C$ on the thickness of the ferromagnetic layer is not significantly different in the two systems, indicating a weak influence of the interfacial roughness on the transparency for Cooper pairs.
We investigate inverse proximity effects in a spin-triplet superconductor (TSC) interfaced with a ferromagnet (FM), assuming different types of magnetic profiles and chiral or helical pairings. The region of the coexistence of spin-triplet superconductivity and magnetism is significantly influenced by the orientation and spatial extension of the magnetization with respect to the spin configuration of the Cooper pairs, resulting into clearcut anisotropy signatures. A characteristic mark of the inverse proximity effect arises in the induced spin-polarization at the TSC interface. This is unexpectedly stronger when the magnetic proximity is weaker, thus unveiling immediate detection signatures for spin-triplet pairs. We show that an anomalous magnetic proximity can occur at the interface between the itinerant ferromagnet, SrRuO$_3$, and the unconventional superconductor Sr$_2$RuO$_4$. Such scenario indicates the potential to design characteristic inverse proximity effects in experimentally available SrRuO$_3$-Sr$_2$RuO$_4$ heterostructures and to assess the occurrence of spin-triplet pairs in the highly debated superconducting phase of Sr$_2$RuO$_4$.
In this work, magnetization dynamics is studied in superconductor/ferromagnet/superconductor three-layered films in a wide frequency, field, and temperature ranges using the broad-band ferromagnetic resonance measurement technique. It is shown that in presence of both superconducting layers and of superconducting proximity at both superconductor/ferromagnet interfaces a massive shift of the ferromagnetic resonance to higher frequencies emerges. The phenomenon is robust and essentially long-range: it has been observed for a set of samples with the thickness of ferromagnetic layer in the range from tens up to hundreds of nanometers. The resonance frequency shift is characterized by proximity-induced magnetic anisotropies: by the positive in-plane uniaxial anisotropy and by the drop of magnetization. The shift and the corresponding uniaxial anisotropy grow with the thickness of the ferromagnetic layer. For instance, the anisotropy reaches 0.27~T in experiment for a sample with 350~nm thick ferromagnetic layer, and about 0.4~T in predictions, which makes it a ferromagnetic film structure with the highest anisotropy and the highest natural resonance frequency ever reported. Various scenarios for the superconductivity-induced magnetic anisotropy are discussed. As a result, the origin of the phenomenon remains unclear. Application of the proximity-induced anisotropies in superconducting magnonics is proposed as a way for manipulations with a spin-wave spectrum.
We study the physical properties of a ballistic heterostructure made of a ferromagnet (FM) and a spin-triplet superconductor (TSC) with a layered structure stacking along the direction perpendicular to the planes where a chiral px+ipy pairing occurs and assuming spin dependent processes at the interface. We use a self-consistent Bogoliubov-de Gennes approach on a three-dimensional lattice to obtain the spatial profiles of the pairing amplitude and the magnetization. We find that, depending on the strength of the ferromagnetic exchange field, the ground state of the system can have two distinct configurations with a parallel or anti-parallel collinearity between the magnetic moments in the bulk and at the interface. We demonstrate that a magnetic state having non coplanar interface, bulk and Cooper pairs spins may be stabilized if the bulk magnetization is assumed to be fixed along a given direction. The study of the density of states reveals that the modification of the electronic spectrum in the FM plays an important role in the setting of the optimal magnetic configuration. Finally, we find the existence of induced spin-polarized pair correlations in the FM-TSC system.
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