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Longitudinal relaxation of a nitrogen-vacancy center in a spin bath by generalized cluster-correlation expansion method

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 Added by Qing Ai Dr.
 Publication date 2018
  fields Physics
and research's language is English




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We theoretically study the longitudinal relaxation of a nitrogen-vacancy (NV) center surrounded by a 13C nuclear spin bath in diamond. By incorporating electron spin in the cluster, we generalize the cluster-correlation expansion (CCE) to theoretically simulate the population dynamics of electron spin of NV center. By means of the generalized CCE, we numerically demonstrate the decay process of electronic state induced by cross relaxation at the ambient temperature. It is shown that the CCE method is not only capable of describing pure-dephasing effect at large-detuning regime, but it can also simulate the quantum dynamics of populations in the nearly-resonant regime.

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We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic field $B$. NV$^-$ centers were created by irradiating a Type 1b single-crystal diamond along the [100] axis with 200 keV electrons from a transmission electron microscope with varying doses to achieve spots of different NV$^-$ center concentrations. Values of ($1/T_1$) were measured for each spot as a function of $B$.
The diamond nitrogen-vacancy (NV) center is a leading platform for quantum information science due to its optical addressability and room-temperature spin coherence. However, measurements of the NV centers spin state typically require averaging over many cycles to overcome noise. Here, we review several approaches to improve the readout performance and highlight future avenues of research that could enable single-shot electron-spin readout at room temperature.
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