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Imaging nanoscale spatial modulation of a relativistic electron beam with a MeV ultrafast electron microscope

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 Added by Chao Lu
 Publication date 2018
  fields Physics
and research's language is English




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Accelerator-based MeV ultrafast electron microscope (MUEM) has been proposed as a promising tool to study structural dynamics at the nanometer spatial scale and picosecond temporal scale. Here we report experimental tests of a prototype MUEM where high quality images with nanoscale fine structures were recorded with a pulsed 3 MeV picosecond electron beam. The temporal and spatial resolution of the MUEM operating in single-shot mode is about 4 ps (FWHM) and 100 nm (FWHM), corresponding to a temporal-spatial resolution of 4e-19 s*m, about 2 orders of magnitude higher than that achieved with state-of-the-art single-shot keV UEM. Using this instrument we offer the demonstration of visualizing the nanoscale periodic spatial modulation of an electron beam, which may be converted into longitudinal density modulation through emittance exchange to enable production of high-power coherent radiation at short wavelengths. Our results mark a great step towards single-shot nanometer-resolution MUEMs and compact intense x-ray sources that may have wide applications in many areas of science.



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We propose and demonstrate a novel scheme to produce ultrashort and ultrastable MeV electron beam. In this scheme, the electron beam produced in a photocathode radio-frequency (rf) gun first expands under its own Coulomb force with which a positive energy chirp is imprinted in the beam longitudinal phase space. The beam is then sent through a double bend achromat with positive longitudinal dispersion where electrons at the bunch tail with lower energies follow shorter paths and thus catch up with the bunch head, leading to longitudinal bunch compression. We show that with optimized parameter sets, the whole beam path from the electron source to the compression point can be made isochronous such that the time of flight for the electron beam is immune to the fluctuations of rf amplitude. With a laser-driven THz deflector, the bunch length and arrival time jitter for a 20 fC beam after bunch compression are measured to be about 29 fs (FWHM) and 22 fs (FWHM), respectively. Such an ultrashort and ultrastable electron beam allows us to achieve 50 femtosecond (FWHM) resolution in MeV ultrafast electron diffraction where lattice oscillation at 2.6 THz corresponding to Bismuth A1g mode is clearly observed without correcting both the short-term timing jitter and long-term timing drift. Furthermore, oscillating weak diffuse scattering signal related to phonon coupling and decay is also clearly resolved thanks to the improved temporal resolution and increased electron flux. We expect that this technique will have a strong impact in emerging ultrashort electron beam based facilities and applications.
Coulomb interaction between charged particles is a well-known phenomenon in many areas of researches. In general the Coulomb repulsion force broadens the pulse width of an electron bunch and limits the temporal resolution of many scientific facilities such as ultrafast electron diffraction and x-ray free-electron lasers. Here we demonstrate a scheme that actually makes use of Coulomb force to compress a relativistic electron beam. Furthermore, we show that the Coulomb-driven bunch compression process does not introduce additional timing jitter, which is in sharp contrast to the conventional radio-frequency buncher technique. Our work not only leads to enhanced temporal resolution in electron beam based ultrafast instruments that may provide new opportunities in probing material systems far from equilibrium, but also opens a promising direction for advanced beam manipulation through self-field interactions.
352 - N. Sudar , P. Musumeci , I. Gadjev 2017
We present results of an experiment showing the first successful demonstration of a cascaded micro-bunching scheme. Two modulator-chicane pre-bunchers arranged in series and a high power mid-IR laser seed are used to modulate a 52 MeV electron beam into a train of sharp microbunches phase-locked to the external drive laser. This configuration allows to increase the fraction of electrons trapped in a strongly tapered inverse free electron laser (IFEL) undulator to 96%, with up to 78% of the particles accelerated to the final design energy yielding a significant improvement compared to the classical single buncher scheme. These results represent a critical advance in laser-based longitudinal phase space manipulations and find application both in high gradient advanced acceleration as well as in high peak and average power coherent radiation sources.
Current models of the effect of spontaneous emission on the electron beam dynamics neglect the discreteness of electron recoil associated with photon emission. We present a novel, one-dimensional model of the effect of spontaneous emission on the electron beam dynamics in an undulator both in the classical regime where discrete electron recoil is negligible, and the quantum regime where it is significant. It is shown that in the classical regime, continuous decrease of the average electron energy and diffusive growth of the electron energy spread occurs, in agreement with previous classical models. In the quantum regime, it is shown that the evolution of the electron momentum distribution occurs as discrete momentum groups according to a Poisson distribution. The narrow momentum features of the quantum regime may be useful for generation of coherent radiation, which relies on electron beams having sufficiently narrow momentum/energy distributions.
We propose and demonstrate a novel method to reduce the pulse width and timing jitter of a relativistic electron beam through THz-driven beam compression. In this method the longitudinal phase space of a relativistic electron beam is manipulated by a linearly polarized THz pulse in a dielectric tube such that the bunch tail has a higher velocity than the bunch head, which allows simultaneous reduction of both pulse width and timing jitter after passing through a drift. In this experiment, the beam is compressed by more than a factor of four from 130 fs to 28 fs with the arrival time jitter also reduced from 97 fs to 36 fs, opening up new opportunities in using pulsed electron beams for studies of ultrafast dynamics. This technique extends the well known rf buncher to the THz frequency and may have a strong impact in accelerator and ultrafast science facilities that require femtosecond electron beams with tight synchronization to external lasers.
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