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Register a new userAchieving 50 femtosecond resolution in MeV ultrafast electron diffraction with a double bend achromat compressor
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We propose and demonstrate a novel scheme to produce ultrashort and ultrastable MeV electron beam. In this scheme, the electron beam produced in a photocathode radio-frequency (rf) gun first expands under its own Coulomb force with which a positive energy chirp is imprinted in the beam longitudinal phase space. The beam is then sent through a double bend achromat with positive longitudinal dispersion where electrons at the bunch tail with lower energies follow shorter paths and thus catch up with the bunch head, leading to longitudinal bunch compression. We show that with optimized parameter sets, the whole beam path from the electron source to the compression point can be made isochronous such that the time of flight for the electron beam is immune to the fluctuations of rf amplitude. With a laser-driven THz deflector, the bunch length and arrival time jitter for a 20 fC beam after bunch compression are measured to be about 29 fs (FWHM) and 22 fs (FWHM), respectively. Such an ultrashort and ultrastable electron beam allows us to achieve 50 femtosecond (FWHM) resolution in MeV ultrafast electron diffraction where lattice oscillation at 2.6 THz corresponding to Bismuth A1g mode is clearly observed without correcting both the short-term timing jitter and long-term timing drift. Furthermore, oscillating weak diffuse scattering signal related to phonon coupling and decay is also clearly resolved thanks to the improved temporal resolution and increased electron flux. We expect that this technique will have a strong impact in emerging ultrashort electron beam based facilities and applications.
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We report the experimental demonstration of femtosecond electron diffraction using high-brightness MeV electron beams. High-quality, single-shot electron diffraction patterns for both polycrystalline aluminum and single-crystal 1T-TaS2 are obtained utilizing a 5 femto-Coulomb (~3x10^4 electrons) pulse of electrons at 2.8 MeV. The high quality of the electron diffraction patterns confirm that electron beam has a normalized emittance of ~50 nm-rad. The corresponding transverse and longitudinal coherence length are ~11 nm and ~2.5 nm, respectively. The timing jitter between the pump laser and probe electron beam was found to be ~ 100 fs (rms). The temporal resolution is demonstrated by observing the evolution of Bragg and superlattice peaks of 1T-TaS2 following an 800 nm optical pump and was found to be 130 fs. Our results demonstrate the advantages of MeV electron diffraction: such as longer coherent lengths, large scattering cross-section and larger signal-to-noise ratio, and the feasibility of ultimately realizing 10 fs time-resolved electron diffraction.
We present the first demonstration of THz-driven bunch compression and timing stabilization of a few-fC relativistic electron beam with kinetic energy of 2.5 MeV using quasi-single-cycle strong field THz radiation in a shorted parallel-plate structure. Compression by nearly a factor of 3 produced a 39 fs rms bunch length and a reduction in timing jitter by more than a factor of 2, to 31 fs rms, offering a significant improvement to beam performance for applications like ultrafast electron diffraction. This THz-driven technique provides a critical step towards unprecedented timing resolution in ultrafast sciences and other accelerator applications using femtosecond-scale electron beams.
The Double Triple Bend Achromat (DTBA) lattice~cite{DTBAipac16} is a novel lattice design for a next generation 3 GeV Synchrotron Light Source. Starting from a modification of the Hybrid Multi Bend Achromat (HMBA) lattice~cite{ESRF} developed at ESRF and inspired by the Double-Double Bend Achromat (DDBA) lattice~cite{Diamond1, Diamond2} developed at Diamond, DTBA combines the advantages of both cells. The typical MBA lattice cells have one straight section dedicated to an insertion device, whereas this new cell layout has two such drifts, thus increasing the fraction of available space for the installation of insertion devices. The DTBA lattice achieves an emittance of $simmathrm{132~pm}$, a dynamic aperture of $mathrm{simpm10pm1~mm}$ (calculated at the injection point), an injection efficiency of $mathrm{simmathrm88pm5%}$ and a lifetime of $mathrm{1.4pm0.2~h}$ with errors. The characteristics of DTBA, the methodology and results of the linear and non-linear optics optimisations, with and without the presence of errors, are presented in detail.
We present the development of the first ultrafast transmission electron microscope (UTEM) driven by localized photoemission from a field emitter cathode. We describe the implementation of the instrument, the photoemitter concept and the quantitative electron beam parameters achieved. Establishing a new source for ultrafast TEM, the Gottingen UTEM employs nano-localized linear photoemission from a Schottky emitter, which enables operation with freely tunable temporal structure, from continuous wave to femtosecond pulsed mode. Using this emission mechanism, we achieve record pulse properties in ultrafast electron microscopy of 9 {AA} focused beam diameter, 200 fs pulse duration and 0.6 eV energy width. We illustrate the possibility to conduct ultrafast imaging, diffraction, holography and spectroscopy with this instrument and also discuss opportunities to harness quantum coherent interactions between intense laser fields and free electron beams.
The dynamics of the photoinduced commensurate to incommensurate charge density wave (CDW) phase transition in 4Hb-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime the CDW reforms on a 150 ps timescale, which is two orders of magnitude slower than in other transition-metal dichalcogenides. We attribute this to a weak coupling between the CDW carrying T-layers and thus demonstrate the importance of three-dimensionality for the existence of CDWs. With increasing optical excitation the phase transition is achieved showing a second order character in contrast to the first order behavior in thermal equilibrium.
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