Do you want to publish a course? Click here

Spin dynamics in helical molecules with non-linear interactions

67   0   0.0 ( 0 )
 Publication date 2017
  fields Physics
and research's language is English




Ask ChatGPT about the research

It is widely admitted that the helical conformation of certain chiral molecules may induce a sizable spin selectivity observed in experiments. Spin selectivity arises as a result of the interplay between a helicity-induced spin-orbit coupling and electric dipole fields in the molecule. From the theoretical point of view, different phenomena might affect the spin dynamics in helical molecules, such as quantum dephasing, dissipation and the role of metallic contacts. Previous studies neglected the local deformation of the molecule about the carrier thus far, but this assumption seems unrealistic to describe charge transport in molecular systems. We introduce an effective model describing the electron spin dynamics in a deformable helical molecule with weak spin-orbit coupling. We find that the electron-lattice interaction allows the formation of stable solitons such as bright solitons with well defined spin projection onto the molecule axis. We present a thorough study of these bright solitons and analyze their possible impact on the spin dynamics in deformable helical molecules.

rate research

Read More

In this paper an effective integrable non-linear model describing the electron spin dynamics in a deformable helical molecule with weak spin-orbit coupling is presented. Non-linearity arises from the electron-lattice interaction and it enables the formation of a variety of stable solitons such as bright solitons, breathers and rogue waves, all of them presenting well defined spin projection onto the molecule axis. A thorough study of the soliton solutions is presented and discussed.
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, using a cyclic spin system as reference. We consider three variants of antiferromagnetic molecular ring, i.e. Cr$_8$, Cr$_7$Zn and Cr$_7$Ni, characterized by low lying states with different total spin $S$. We theoretically and experimentally study the low-temperature behavior of the magnetic torque as a function of the applied magnetic field. Near level crossings, this observable selectively probes quantum fluctuations of the total spin ($S$ mixing) induced by lowering of the ideal ring symmetry. We show that while a typical distortion of a model molecular structure is very ineffective in opening new $S$-mixing channels, the spin topology is a major ingredient to control the degree of $S$ mixing. This conclusion is further substantiated by low-temperature heat capacity measurements.
72 - Sonu Verma , Arijit Kundu 2018
An infinite edge of a quantum Hall system prohibits indirect exchange coupling between two spins whereas a quantum spin-Hall edge prohibits out-of-plane coupling. In this study we analyze an unexpected breakdown of this behaviors in a finite system, where the two spins can interact also via a longer path that traverses the whole perimeter of the system. We explain this using an analytical model as well as using tight binding models in real space. Based on this finding, we propose how using a lead far away from the spins can switch the coupling on and off among them non-locally.
We investigate theoretically the spin-spin interaction of two-electrons in vertically coupled QDs as a function of the angle between magnetic field and growth axis. Our numerical approach is based on a real-space description of single-particle states in realistic samples and exact diagonalization of carrier-carrier Coulomb interaction. In particular, the effect of the in-plane field component on tunneling and, therefore, spin-spin interaction will be discussed; the singlet-triplet phase diagram as a function of the field strength and direction is drawn.
Spin-helical states, which arise in quasi-one-dimensional (1D) channels with spin-orbital (SO) coupling, underpin efforts to realize topologically-protected quantum bits based on Majorana modes in semiconductor nanowires. Detecting helical states is challenging due to non-idealities present in real devices. Here we show by means of tight-binding calculations that by using ferromagnetic contacts it is possible to detect helical modes with high sensitivity even in the presence of realistic device effects, such as quantum interference. This is possible because of the spin-selective transmission properties of helical modes. In addition, we show that spin-polarized contacts provide a unique path to investigate the spin texture and spin-momentum locking properties of helical states. Our results are of interest not only for the ongoing development of Majorana qubits, but also as for realizing possible spin-based quantum devices, such as quantum spin modulators and interconnects based on spin-helical channels.
comments
Fetching comments Fetching comments
Sign in to be able to follow your search criteria
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا