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Quadrupolar quantum criticality on a fractal

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 Added by Ribhu Kaul
 Publication date 2017
  fields Physics
and research's language is English




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We study the ground state ordering of quadrupolar ordered $S=1$ magnets as a function of spin dilution probability $p$ on the triangular lattice. In sharp contrast to the ordering of $S=1/2$ dipolar Neel magnets on percolating clusters, we find that the quadrupolar magnets are quantum disordered at the percolation threshold, $p=p^*$. Further we find that long-range quadrupolar order is present for all $p<p^*$ and vanishes first exactly at $p^*$. Strong evidence for scaling behavior close to $p^*$ points to an unusual quantum criticality without fine tuning that arises from an interplay of quantum fluctuations and randomness.

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PrV2Al20 is the heavy fermion superconductor based on the cubic Gamma3 doublet that exhibits non- magnetic quadrupolar ordering below ~ 0.6 K. Our magnetotransport study on PrV2Al20 reveals field-induced quadrupolar quantum criticality at Hc ~ 11 T applied along the [111] direction. Near the critical field Hc required to suppress the quadrupolar state, we find a marked enhancement of the resistivity rho(H, T), a divergent effective mass of quasiparticles and concomitant non-Fermi liquid (NFL) behavior (i.e. rho(T) ~ T^n with n < 0.5). We also observe the Shubnikov de Haas-effect above ?Hc, indicating the enhanced effective mass m/m0 ~ 10. This reveals the competition between the nonmagnetic Kondo effect and the intersite quadrupolar coupling, leading to the pronounced NFL behavior in an extensive region of T and H emerging from the quantum critical point.
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