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Probing the Efimov discrete scaling in atom-molecule collision

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 Added by M. T. Yamashita
 Publication date 2017
  fields Physics
and research's language is English




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The discrete Efimov scaling behavior, well-known in the low-energy spectrum of three-body bound systems for large scattering lengths (unitary limit), is identified in the energy dependence of atom-molecule elastic cross-section in mass imbalanced systems. That happens in the collision of a heavy atom with mass $m_H$ with a weakly-bound dimer formed by the heavy atom and a lighter one with mass $m_L ll m_H$. Approaching the heavy-light unitary limit the $s-$wave elastic cross-section $sigma$ will present a sequence of zeros/minima at collision energies following closely the Efimov geometrical law. Our results open a new perspective to detect the discrete scaling behavior from low-energy scattering data, which is timely in view of the ongoing experiments with ultra-cold binary mixtures having strong mass asymmetries, such as Lithium and Caesium or Lithium and Ytterbium.



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83 - M.T. Yamashita 2019
Efimov physics is drastically affected by the change of spatial dimensions. Efimov states occur in a tridimensional (3D) environment, but disappear in two (2D) and one (1D) dimensions. In this paper, dedicated to the memory of Prof. Faddeev, we will review some recent theoretical advances related to the effect of dimensionality in the Efimov phenomenon considering three-boson systems interacting by a zero-range potential. We will start with a very ideal case with no physical scales, passing to a system with finite energies in the Born-Oppenheimer (BO) approximation and finishing with a general system. The physical reason for the appearance of the Efimov effect is given essentially by two reasons which can be revealed by the BO approximation - the form of the effective potential is proportional to $1/R^2$ ($R$ is the relative distance between the heavy particles) and its strength is smaller than the critical value given by $-(D-2)^2/4$, where $D$ is the effective dimension.
Understanding ultracold collisions involving molecules is of fundamental importance for current experiments, where inelastic collisions typically limit the lifetime of molecular ensembles in optical traps. Here we present a broad study of optically trapped ultracold RbCs molecules in collisions with one another, in reactive collisions with Rb atoms, and in nonreactive collisions with Cs atoms. For experiments with RbCs alone, we show that by modulating the intensity of the optical trap, such that the molecules spend 75% of each modulation cycle in the dark, we partially suppress collisional loss of the molecules. This is evidence for optical excitation of molecule pairs mediated via sticky collisions. We find that the suppression is less effective for molecules not prepared in the spin-stretched hyperfine ground state. This may be due either to longer lifetimes for complexes or to laser-free decay pathways. For atom-molecule mixtures, RbCs+Rb and RbCs+Cs, we demonstrate that the rate of collisional loss of molecules scales linearly with the density of atoms. This indicates that, in both cases, the loss of molecules is rate-limited by two-body atom-molecule processes. For both mixtures, we measure loss rates that are below the thermally averaged universal limit.
The existence of the Efimov effect is drastically affected by the dimensionality of the space in which the system is embedded. The effective spatial dimension containing an atomic cloud can be continuously modified by compressing it in one or two directions. In the present article we determine for a general $AAB$ system formed by two identical bosons $A$ and a third particle $B$ in the two-body unitary limit, the dimensionsality $D$ for which the Efimov effect can exist for different values of the mass ratio $mathpzc{A}=m_B/m_A$. In addition, we provide a prediction for the Efimov discrete scaling factor, ${rm exp},(pi/s)$, as a function of a wide range of values of $mathpzc{A}$ and $D$, which can be tested in experiments that can be realized with currently available technology.
We study a three-body system, formed by two identical heavy bosons and a light particle, in the Born-Oppenheimer approximation for an arbitrary dimension $D$. We restrict $D$ to the interval $2,<,D,<,4$, and derive the heavy-heavy $D$-dimensional effective potential proportional to $1/R^2$ ($R$ is the relative distance between the heavy particles), which is responsible for the Efimov effect. We found that the Efimov states disappear once the critical strength of the heavy-heavy effective potential $1/R^2$ approaches the limit $-(D-2)^2/4$. We obtained the scaling function for the $^{133}$Cs-$^{133}$Cs-$^6$Li system as the limit cycle of the correlation between the energies of two consecutive Efimov states as a function of $D$ and the heavy-light binding energy $E^{D}_2$. In addition, we found that the energy of the $(N+1)^{rm th}$ excited state reaches the two-body continuum independently of the dimension $D$ when $sqrt{E^{D}_2/E_3^{(N)}}=0.89$, where $E_3^{(N)}$ is the $N^{rm th}$ excited three-body binding energy.
We investigate collisional loss in an ultracold mixture of $^{40}$K$^{87}$Rb molecules and $^{87}$Rb atoms, where chemical reactions between the two species are energetically forbidden. Through direct detection of the KRb$_{2}^{*}$ intermediate complexes formed from atom-molecule collisions, we show that a $1064$ nm laser source used for optical trapping of the sample can efficiently deplete the complex population via photo-excitation, an effect which can explain the universal two-body loss observed in the mixture. By monitoring the time-evolution of the KRb$_{2}^{*}$ population after a sudden reduction in the $1064$ nm laser intensity, we measure the lifetime of the complex ($0.39(6)$ ms), as well as the photo-excitation rate for $1064$ nm light ($0.50(3)$ $mu$s$^{-1}($kW/cm$^{2})^{-1}$). The observed lifetime is ${sim}10^{5}$ times longer than recent estimates based on the Rice-Ramsperger-Kassel-Marcus statistical theory, which calls for new insight to explain such a dramatic discrepancy.
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