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$^{133}text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive material, we trap and laser-cool the synthetic $A$ = 133 radioisotope of barium II in a radio-frequency ion trap. Using the same, single trapped atom, we measure the isotope shifts and hyperfine structure of the $6^2 text{P}_{1/2}$ $leftrightarrow$ $6^2 text{S}_{1/2}$ and $6^2 text{P}_{1/2}$ $leftrightarrow$ $5^2 text{D}_{3/2}$ electronic transitions that are needed for laser cooling, state preparation, and state detection of the clock-state hyperfine and optical qubits. We also report the $6^2 text{P}_{1/2}$ $leftrightarrow$ $5^2 text{D}_{3/2}$ electronic transition isotope shift for the rare $A$ = 130 and 132 barium nuclides, completing the spectroscopic characterization necessary for laser cooling all long-lived barium II isotopes.
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Molecules are the most demanding quantum systems to be simulated by quantum computers because of their complexity and the emergent role of quantum nature. The recent theoretical proposal of Huh et al. (Nature Photon., 9, 615 (2015)) showed that a multi-photon network with a Gaussian input state can simulate a molecular spectroscopic process. Here, we report the first experimental demonstration of molecular vibrational spectroscopy of SO$_{2}$ with a trapped-ion system. In our realization, the molecular scattering operation is decomposed to a series of elementary quantum optical operations, which are implemented through Raman laser beams, resulting in a multimode Gaussian (Bogoliubov) transformation. The molecular spectroscopic signal is reconstructed from the collective projection measurements on phonon modes of the trapped-ion system. Our experimental demonstration would pave the way to large-scale molecular quantum simulations, which are classically intractable.
In recent years, arrays of atomic ions in a linear RF trap have proven to be a particularly successful platform for quantum simulation. However, a wide range of quantum models and phenomena have, so far, remained beyond the reach of such simulators. In this work we introduce a technique that can substantially extend this reach using an external field gradient along the ion chain and a global, uniform driving field. The technique can be used to generate both static and time-varying synthetic gauge fields in a linear chain of trapped ions, and enables continuous simulation of a variety of coupling geometries and topologies, including periodic boundary conditions and high dimensional Hamiltonians. We describe the technique, derive the corresponding effective Hamiltonian, propose a number of variations, and discuss the possibility of scaling to quantum-advantage sized simulators. Additionally, we suggest several possible implementations and briefly examine two: the Aharonov-Bohm ring and the frustrated triangular ladder.
We demonstrate key multi-qubit quantum logic primitives in a dual-species trapped-ion system based on $^{40}$Ca+ and $^{88}$Sr+ ions, using two optical qubits with quantum-logic-control frequencies in the red to near-infrared range. With all ionization, cooling, and control wavelengths in a wavelength band similar for the two species and centered in the visible, and with a favorable mass ratio for sympathetic cooling, this pair is a promising candidate for scalable quantum information processing. Same-species and dual-species two-qubit gates, based on the Moelmer-Soerensen interaction and performed in a cryogenic surface-electrode trap, are characterized via the fidelity of generated entangled states; we achieve fidelities of 98.8(2)% and 97.5(2)% in Ca+ - Ca+ and Sr+ - Sr+ gates, respectively. For a similar Ca+ - Sr+ gate, we achieve a fidelity of 94.3(3)%, and carrying out a Sr+ - Sr+ gate performed with a Ca+ sympathetic cooling ion in a Sr+ - Ca+ - Sr+ crystal configuration, we achieve a fidelity of 95.7(3)%. These primitives form a set of trapped-ion capabilities for logic with sympathetic cooling and ancilla readout or state transfer for general quantum computing and communication applications.
We introduce a measurement scheme that utilizes a single ion as a local field probe. The ion is confined in a segmented Paul trap and shuttled around to reach different probing sites. By the use of a single atom probe, it becomes possible characterizing fields with spatial resolution of a few nm within an extensive region of millimeters. We demonstrate the scheme by accurately investigating the electric fields providing the confinement for the ion. For this we present all theoretical and practical methods necessary to generate these potentials. We find sub-percent agreement between measured and calculated electric field values.
We demonstrate a coherence time of 2.1(1)~s for electron spin superposition states of a single trapped $^{40}$Ca$^+$ ion. The coherence time, measured with a spin-echo experiment, corresponds to residual rms magnetic field fluctuations $leq$~2.7$times$10$^{-12}$~T. The suppression of decoherence induced by fluctuating magnetic fields is achieved by combining a two-layer $mu$-metal shield, which reduces external magnetic noise by 20 to 30~dB for frequencies of 50~Hz to 100~kHz, with Sm$_2$Co$_{17}$ permanent magnets for generating a quantizing magnetic field of 0.37~mT. Our results extend the coherence time of the simple-to-operate spin qubit to ultralong coherence times which so far have been observed only for magnetic insensitive transitions in atomic qubits with hyperfine structure.
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