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Molecules are the most demanding quantum systems to be simulated by quantum computers because of their complexity and the emergent role of quantum nature. The recent theoretical proposal of Huh et al. (Nature Photon., 9, 615 (2015)) showed that a multi-photon network with a Gaussian input state can simulate a molecular spectroscopic process. Here, we report the first experimental demonstration of molecular vibrational spectroscopy of SO$_{2}$ with a trapped-ion system. In our realization, the molecular scattering operation is decomposed to a series of elementary quantum optical operations, which are implemented through Raman laser beams, resulting in a multimode Gaussian (Bogoliubov) transformation. The molecular spectroscopic signal is reconstructed from the collective projection measurements on phonon modes of the trapped-ion system. Our experimental demonstration would pave the way to large-scale molecular quantum simulations, which are classically intractable.
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We present a cryogenic ion trapping system designed for large scale quantum simulation of spin models. Our apparatus is based on a segmented-blade ion trap enclosed in a 4 K cryostat, which enables us to routinely trap over 100 $^{171}$Yb$^+$ ions in a linear configuration for hours due to a low background gas pressure from differential cryo-pumping. We characterize the cryogenic vacuum by using trapped ion crystals as a pressure gauge, measuring both inelastic and elastic collision rates with the molecular background gas. We demonstrate nearly equidistant ion spacing for chains of up to 44 ions using anharmonic axial potentials. This reliable production and lifetime enhancement of large linear ion chains will enable quantum simulation of spin models that are intractable with classical computer modelling.
$^{133}text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive material, we trap and laser-cool the synthetic $A$ = 133 radioisotope of barium II in a radio-frequency ion trap. Using the same, single trapped atom, we measure the isotope shifts and hyperfine structure of the $6^2 text{P}_{1/2}$ $leftrightarrow$ $6^2 text{S}_{1/2}$ and $6^2 text{P}_{1/2}$ $leftrightarrow$ $5^2 text{D}_{3/2}$ electronic transitions that are needed for laser cooling, state preparation, and state detection of the clock-state hyperfine and optical qubits. We also report the $6^2 text{P}_{1/2}$ $leftrightarrow$ $5^2 text{D}_{3/2}$ electronic transition isotope shift for the rare $A$ = 130 and 132 barium nuclides, completing the spectroscopic characterization necessary for laser cooling all long-lived barium II isotopes.
Modern computation relies crucially on modular architectures, breaking a complex algorithm into self-contained subroutines. A client can then call upon a remote server to implement parts of the computation independently via an application programming interface (API). Present APIs relay only classical information. Here we implement a quantum API that enables a client to estimate the absolute value of the trace of a server-provided unitary $U$. We demonstrate that the algorithm functions correctly irrespective of what unitary $U$ the server implements or how the server specifically realizes $U$. Our experiment involves pioneering techniques to coherently swap qubits encoded within the motional states of a trapped Yb ion, controlled on its hyperfine state. This constitutes the first demonstration of modular computation in the quantum regime, providing a step towards scalable, parallelization of quantum computation.
Scaling-up from prototype systems to dense arrays of ions on chip, or vast networks of ions connected by photonic channels, will require developing entirely new technologies that combine miniaturized ion trapping systems with devices to capture, transmit and detect light, while refining how ions are confined and controlled. Building a cohesive ion system from such diverse parts involves many challenges, including navigating materials incompatibilities and undesired coupling between elements. Here, we review our recent efforts to create scalable ion systems incorporating unconventional materials such as graphene and indium tin oxide, integrating devices like optical fibers and mirrors, and exploring alternative ion loading and trapping techniques.
Quantum-mechanical principles can be used to process information (QIP). In one approach, linear arrays of trapped, laser cooled ion qubits (two-level quantum systems) are confined in segmented multi-zone electrode structures. The ion trap approach to QIP requires trapping and control of numerous ions in electrode structures with many trapping zones. I investigated microfabrication of structures to trap, transport and couple large numbers of ions. Using 24Mg+ I demonstrated loading and transport between zones in microtraps made of boron doped silicon. This thesis describes the fundamentals of ion trapping, the characteristics of silicon-based traps amenable to QIP work and apparatus to trap ions and characterize traps. Microfabrication instructions appropriate for nonexperts are included. Ion motional heating was measured. <<>> Using MEMs techniques I built a Si micro-mechanical oscillator and demonstrated a method to reduce the kinetic energy of its lowest order mechanical mode via capacitive coupling to a driven radio frequency (RF) oscillator. Cooling resulted from a RF capacitive force, phase shifted relative to the cantilever motion. The technique was demonstrated by cooling the 7 kHz fundamental mode from room temperature to 45 K. <<>> I also discuss an implementation of the semiclassical quantum Fourier transform (QFT) using three beryllium ion qubits. The QFT is a crucial step in a number of quantum algorithms including Shors algorithm, a quantum approach to integer factorization which is exponentially faster than the fastest known classical factoring algorithm. This demonstration incorporated the key elements of a scalable ion-trap architecture for QIP.
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