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The recent detection of fullerene (C$_{60}$) in space and the positive assignment of five diffuse interstellar bands to C$_{60}^+$ reinforce the notion that fullerene-related compounds can be efficiently formed in circumstellar envelopes and be present in significant quantities in the interstellar medium. Experimental studies have shown that C$_{60}$ can be readily hydrogenated, raising the possibility that hydrogenated fullerenes (or fulleranes, C$_{60}$H$_m$, $m=1-60$) may be abundant in space. In this paper, we present theoretical studies of the vibrational modes of isomers of C$_{60}$H$_m$. Our results show that the four mid-infrared bands from the C$_{60}$ skeletal vibrations remain prominent in slightly hydrogenated C$_{60}$, but their strengths diminish in different degrees with increasing hydrogenation. It is therefore possible that the observed infrared bands assigned to C$_{60}$ could be due to a mixture of fullerenes and fulleranes. This provides a potential explanation for the observed scatter of the C$_{60}$ band ratios. Our calculations suggest that a feature around 15$mu$m due to the breathing mode of heavily hydrogenated C$_{60}$ may be detectable astronomically. A preliminary search for this feature in 35 C$_{60}$ sources is reported.
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Carbon monoxide (CO) is the most abundant molecule after molecular hydrogen and is important for the chemistry in circumstellar envelopes around evolved stars. When modelling the strength and shape of molecular lines, the size of the CO envelope is an input parameter and influences the derived mass-loss rates. In particular the low-J transition CO lines are sensitive to the CO photodissociation radius. Recently, new CO photodissociation radii have been published using different formalisms that differ considerably. One set of calculations is based on an escape-probability formalisms that uses numerical approximations derived in the early-eighties. The accuracy of these approximations is investigated and it is shown that they are less accurate than claimed. Improved formalism are derived. Nevertheless, the changes in CO envelope size are small to moderate, less than 2% for models with $10^{-7}< dot{M}< 10^{-4}$ msolyr and at most 7% for model with $dot{M} = 10^{-8}$ msolyr.
We present a new approach aimed at constraining the typical size and optical properties of carbon dust grains in Circumstellar envelopes (CSEs) of carbon-rich stars (C-stars) in the Small Magellanic Cloud (SMC). To achieve this goal, we apply our recent dust growth description, coupled with a radiative transfer code to the CSEs of C-stars evolving along the TP-AGB, for which we compute spectra and colors. Then we compare our modeled colors in the near- and mid-infrared (NIR and MIR) bands with the observed ones, testing different assumptions in our dust scheme and employing several data sets of optical constants for carbon dust available in the literature. Different assumptions adopted in our dust scheme change the typical size of the carbon grains produced. We constrain carbon dust properties by selecting the combination of grain size and optical constants which best reproduces several colors in the NIR and MIR at the same time. The different choices of optical properties and grain size lead to differences in the NIR and MIR colors greater than two magnitudes in some cases. We conclude that the complete set of observed NIR and MIR colors are best reproduced by small grains, with sizes between $sim$0.035 and $sim$0.12~$mu$m, rather than by large grains between $sim0.2$ and $0.7$~$mu$m. The inability of large grains to reproduce NIR and MIR colors seems independent of the adopted optical data set. We also find a possible trend of the grain size with mass-loss and/or carbon excess in the CSEs of these stars.
We report a search for the diatomic hydrides SiH, PH, and FeH along the line of sight toward the chemically rich circumstellar envelopes of IRC+10216 and VY Canis Majoris. These molecules are thought to form in high temperature regions near the photospheres of these stars, and may then further react via gas-phase and dust-grain interactions leading to more complex species, but have yet to be constrained by observation. We used the GREAT spectrometer on SOFIA to search for rotational emission lines of these molecules in four spectral windows ranging from 600 GHz to 1500 GHz. Though none of the targeted species were detected in our search, we report their upper limit abundances in each source and discuss how they influence the current understanding of hydride chemistry in dense circumstellar media. We attribute the non-detections of these hydrides to their compact source sizes, high barriers of formation, and proclivity to react with other molecules in the winds.
Carbon monoxide is the most abundant molecule after H$_2$ and is important for chemistry in circumstellar envelopes around late-type stars. The size of the envelope is important when modelling low-J transition lines and deriving mass-loss rates from such lines. Now that ALMA is coming to full power the extent of the CO emitting region can be measured directly for nearby asymptotic giant branch (AGB) stars. In parallel, it has become obvious in the past few years that the strength of the interstellar radiation field (ISRF) can have a significant impact on the interpretation of the emission lines. In this paper an update and extension of the classical Mamon et al. (1988; ApJ 328, 797) paper is presented; these authors provided the CO abundance profile, described by two parameters, as a function of mass-loss rate and expansion velocity. Following recent work an improved numerical method and updated H$_2$ and CO shielding functions are used and a larger grid is calculated that covers more parameter space, including the strength of the ISRF. The effect of changing the photodissociation radius on the low-J CO line intensities is illustrated in two cases.
The small-scale bipolar jets having short dynamical ages from water fountain (WF) sources are regarded as an indication of the onset of circumstellar envelope morphological metamorphosis of intermediate-mass stars. Such process usually happens at the end of the asymptotic giant branch (AGB) phase. However, recent studies found that WFs could be AGB stars or even early planetary nebulae. This fact prompted the idea that WFs may not necessarily be objects at the beginning of the morphological transition process. In the present work, we show that WFs could have different envelope morphologies by studying their spectral energy distribution profiles. Some WFs have spherical envelopes that resembles usual AGB stars, while others have aspherical envelopes which are more common to post-AGB stars. The results imply that WFs may not represent the earliest stage of the morphological metamorphosis. We further argue that the dynamical age of a WF jet, which can be calculated from maser proper motions, may not be the real age of the jet. The dynamical age cannot be used to justify the moment when the envelope begins to become aspherical, nor to tell the concrete evolutionary status of the object. A WF jet could be the innermost part of a larger well-developed jet, which is not necessarily a young jet.
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