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Pseudogap temperature $T^star$ of cuprate superconductors from the Nernst effect

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 Publication date 2017
  fields Physics
and research's language is English




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We use the Nernst effect to delineate the boundary of the pseudogap phase in the temperature-doping phase diagram of cuprate superconductors. New data for the Nernst coefficient $ u(T)$ of YBa$_{2}$Cu$_{3}$O$_{y}$ (YBCO), La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_4$ (Eu-LSCO) and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ (Nd-LSCO) are presented and compared with previous data including La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). The temperature $T_ u$ at which $ u/T$ deviates from its high-temperature behaviour is found to coincide with the temperature at which the resistivity deviates from its linear-$T$ dependence, which we take as the definition of the pseudogap temperature $T^star$- in agreement with gap opening detected in ARPES data. We track $T^star$ as a function of doping and find that it decreases linearly vs $p$ in all four materials, having the same value in the three LSCO-based cuprates, irrespective of their different crystal structures. At low $p$, $T^star$ is higher than the onset temperature of the various orders observed in underdoped cuprates, suggesting that these orders are secondary instabilities of the pseudogap phase. A linear extrapolation of $T^star(p)$ to $p=0$ yields $T^star(pto 0)simeq T_N(0)$, the Neel temperature for the onset of antiferromagnetic order at $p=0$, suggesting that there is a link between pseudogap and antiferromagnetism. With increasing $p$, $T^star(p)$ extrapolates linearly to zero at $psimeq p_{rm c2}$, the critical doping below which superconductivity emerges at high doping, suggesting that the conditions which favour pseudogap formation also favour pairing. We also use the Nernst effect to investigate how far superconducting fluctuations extend above $T_{rm c}$, as a function of doping, and find that a narrow fluctuation regime tracks $T_{rm c}$, and not $T^star$. This confirms that the pseudogap phase is not a form of precursor superconductivity.



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In a multiorbital model of the cuprate high-temperature superconductors soft antiferromagnetic (AF) modes are assumed to reconstruct the Fermi surface to form nodal pockets. The subsequent charge ordering transition leads to a phase with a spatially modulated transfer of charge between neighboring oxygen p_x and p_y orbitals and also weak modulations of the charge density on the copper d_{x^2-y^2} orbitals. As a prime result of the AF Fermi surface reconstruction, the wavevectors of the charge modulations are oriented along the crystalline axes with a periodicity that agrees quantitatively with experiments. This resolves a discrepancy between experiments, which find axial order, and previous theoretical calculations, which find modulation wavevectors along the Brillouin zone (BZ) diagonal. The axial order is stabilized by hopping processes via the Cu4s orbital, which is commonly not included in model analyses of cuprate superconductors.
We calculate scattering interference patterns for various electronic states proposed for the pseudogap regime of the cuprate superconductors. The scattering interference models all produce patterns whose wavelength changes as a function of energy, in contradiction to the energy-independent wavelength seen by scanning tunneling microscopy (STM) experiments in the pseudogap state. This suggests that the patterns seen in STM local density of states measurements are not due to scattering interference, but are rather the result of some form of ordering.
We report in-plane resistivity ($rho$) and transverse magnetoresistance (MR) measurements in underdoped HgBa$_2$CuO$_{4+delta}$ (Hg1201). Contrary to the longstanding view that Kohlers rule is strongly violated in underdoped cuprates, we find that it is in fact satisfied in the pseudogap phase of Hg1201. The transverse MR shows a quadratic field dependence, $deltarho/rho_o=a H^{2}$, with $a(T)propto T^{-4}$. In combination with the observed $rhopropto T^2$ dependence, this is consistent with a single Fermi-liquid quasiparticle scattering rate. We show that this behavior is universal, yet typically masked in cuprates with lower structural symmetry or strong disorder effects.
The properties of cuprate high-temperature superconductors are largely shaped by competing phases whose nature is often a mystery. Chiefly among them is the pseudogap phase, which sets in at a doping $p^*$ that is material-dependent. What determines $p^*$ is currently an open question. Here we show that the pseudogap cannot open on an electron-like Fermi surface, and can only exist below the doping $p_{FS}$ at which the large Fermi surface goes from hole-like to electron-like, so that $p^*$ $leq$ $p_{FS}$. We derive this result from high-magnetic-field transport measurements in La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ under pressure, which reveal a large and unexpected shift of $p^*$ with pressure, driven by a corresponding shift in $p_{FS}$. This necessary condition for pseudogap formation, imposed by details of the Fermi surface, is a strong constraint for theories of the pseudogap phase. Our finding that $p^*$ can be tuned with a modest pressure opens a new route for experimental studies of the pseudogap.
A model of charged hole-pair bosons, with long range Coulomb interactions and very weak interlayer coupling, is used to calculate the order parameter -Phi- of underdoped cuprates. Model parameters are extracted from experimental superfluid densities and plasma frequencies. The temperature dependence -Phi(T)- is characterized by a trapezoidal shape. At low temperatures, it declines slowly due to harmonic phase fluctuations which are suppressed by anisotropic plasma gaps. Above the single layer Berezinski-Kosterlitz-Thouless (BKT) temperature, Phi(T) falls rapidly toward the three dimensional transition temperature. The theoretical curves are compared to c-axis superfluid density data by H. Kitano et al., (J. Low Temp. Phys. 117, 1241 (1999)) and to the -transverse nodal velocity- measured by angular resolved photoemmission spectra on BSCCO samples by W.S. Lee et al., (Nature 450, 81 (2007)), and by A. Kanigel, et al., (Phys. Rev. Lett. 99, 157001 (2007)).
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