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Register a new userNonlinear continuous-wave optical propagation in nematic liquid crystals: interplay between reorientational and thermal effects
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Added by
Alessandro Alberucci
Publication date
2017
fields
Physics
and research's language is
English
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Thanks to their unique properties, nematic liquid crystals feature a variety of mechanisms for light-matter interactions. For continuous-wave optical excitations, the two dominant contributions stem from reorientational and thermal nonlinearities. We thoroughly analyze the competing roles of these two nonlinear responses with reference to self-focusing/defocusing and, eventually, the formation of nonlinear diffraction-free wavepackets, the so-called spatial optical solitons. To this extent we refer to dye-doped nematic liquid crystals in planar cells and continuous-wave beams at two distinct wavelengths in order to adjust the relative weights of the two responses. The theoretical analysis is complemented by numerical simulations in the highly nonlocal approximation and compared to experimental results.
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In uniaxial soft matter with a reorientational nonlinearity, such as nematic liquid crystals, a light beam in the extraordinary polarization walks off its wavevector due to birefringence, while it undergoes self-focusing via an increase in refractive index and eventually forms a spatial soliton. Hereby the trajectory evolution of solitons in nematic liquid crystals- nematicons- in the presence of a linearly varying transverse orientation of the optic axis is analysed. In this study we use and compare two approaches: i) a slowly varying (adiabatic) approximation based on momentum conservation of the soliton in a Hamiltonian sense; ii) the Frank-Oseen elastic theory coupled with a fully vectorial and nonlinear beam propagation method. The models provide comparable results in such a non-homogeneously oriented uniaxial medium and predict curved soliton paths with either monotonic or non-monotonic curvatures. The minimal power needed to excite a solitary wave via reorientation remains essentially the same in both uniform and modulated cases.
We analyze the existence and stability of two-component vector solitons in nematic liquid crystals for which one of the components carries angular momentum and describes a vortex beam. We demonstrate that the nonlocal, nonlinear response can dramatically enhance the field coupling leading to the stabilization of the vortex beam when the amplitude of the second beam exceeds some threshold value. We develop a variational approach to describe this effect analytically.
Nonlinear optical propagation in cholesteric liquid crystals (CLC) with a spatially periodic helical molecular structure is studied experimentally and modeled numerically. This periodic structure can be seen as a Bragg grating with a propagation stopband for circularly polarized light. The CLC nonlinearity can be strengthened by adding absorption dye, thus reducing the nonlinear intensity threshold and the necessary propagation length. As the input power increases, a blue shift of the stopband is induced by the self-defocusing nonlinearity, leading to a substantial enhancement of the transmission and spreading of the beam. With further increase of the input power, the self-defocusing nonlinearity saturates, and the beam propagates as in the linear-diffraction regime. A system of nonlinear couple-mode equations is used to describe the propagation of the beam. Numerical results agree well with the experiment findings, suggesting that modulation of intensity and spatial profile of the beam can be achieved simultaneously under low input intensities in a compact CLC-based micro-device.
We consider the simplified Ericksen-Leslie model in three dimensional bounded Lipschitz domains. Applying a semilinear approach, we prove local and global well-posedness (assuming a smallness condition on the initial data) in critical spaces for initial data in $L^3_{sigma}$ for the fluid and $W^{1,3}$ for the director field. The analysis of such models, so far, has been restricted to domains with smooth boundaries.
We present in this paper a detailed analysis of the flexoelectric instability of a planar nematic layer in the presence of an alternating electric field (frequency $omega$), which leads to stripe patterns (flexodomains) in the plane of the layer. This equilibrium transition is governed by the free energy of the nematic which describes the elasticity with respects to the orientational degrees of freedom supplemented by an electric part. Surprisingly the limit $omega to 0$ is highly singular. In distinct contrast to the dc-case, where the patterns are stationary and time-independent, they appear at finite, small $omega$ periodically in time as sudden bursts. Flexodomains are in competition with the intensively studied electro-hydrodynamic instability in nematics, which presents a non-equilibrium dissipative transition. It will be demonstrated that $omega$ is a very convenient control parameter to tune between flexodomains and convection patterns, which are clearly distinguished by the orientation of their stripes.
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