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Radiogenic Neutron Yield Calculations for Low-Background Experiments

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 Added by Shawn Westerdale
 Publication date 2017
  fields Physics
and research's language is English




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Nuclear recoil backgrounds are one of the most dangerous backgrounds for many dark matter experiments. A primary source of nuclear recoils is radiogenic neutrons produced in the detector material itself. These neutrons result from fission and $(alpha,n)$ reactions originating from uranium and thorium contamination. In this paper, we discuss neutron yields from these sources. We compile a list of $(alpha,n)$ yields for many materials common in low-background detectors, calculated using NeuCBOT, a new tool introduced in this paper, available at https://github.com/shawest/neucbot. These calculations are compared to computations made using data compilations and SOURCES-4A



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Ultra-low-background experiments address some of the most important open questions in particle physics, cosmology and astrophysics: the nature of dark matter, whether the neutrino is its own antiparticle, and does the proton decay. These rare event searches require well-understood and minimized backgrounds. Simulations are used to understand backgrounds caused by naturally occurring radioactivity in the rock and in every piece of shielding and detector material used in these experiments. Most important are processes like spontaneous fission and ({alpha},n) reactions in material close to the detectors that can produce neutrons. A comparison study between two dedicated software packages is detailed. The cross section libraries, neutron yields, and spectra from the Mei-Zhang-Hime and the SOURCES-4A codes are presented. The resultant yields and spectra are used as inputs to direct dark matter detector toy models in GEANT4, to study the impact of their differences on background estimates and fits. Although differences in neutron yield calculations up to 50% were seen, there was no systematic difference between the Mei-Hime-Zhang and SOURCES-4A results. Neutron propagation simulations smooth differences in spectral shape and yield, and both tools were found to meet the broad requirements of the low-background community.
We report a novel correlated background in the antineutrino detection using the inverse beta decay reaction. Spontaneous fissions and $(alpha,n)$ reactions in peripheral materials of the antineutrino detector, such as borosilicate glass of photomultipliers, produce fast neutrons and prompt gamma rays. If the shielding from the material to the detector target were not thick enough, neutrons and gammas could enter the target volume and mimic antineutrino signals. This paper revisits the yields and energy spectra of neutrons produced in B$(alpha,n)$N and F$(alpha,n)$Na reactions. A Geant4 based simulation has been carried out using a simplified detector geometry for the present generation reactor neutrino experiments. The background rates in these experiments are estimated. If this background was not taken into account, the value of the neutrino mixing angle $sin^22theta_{13}$ would be underestimated. We recommend that Daya Bay, RENO, Double Chooz, and JUNO, carefully examine the masses and radiopurity levels of detector materials that are close to the target and rich in boron and fluorine.
The response of a scintillation detector with a cylindrical 1.5-inch LaBr3:Ce crystal to incident neutrons has been measured in the energy range En = 2-12 MeV. Neutrons were produced by proton irradiation of a Li target at Ep = 5-14.6 MeV with pulsed proton beams. Using the time-of-flight information between target and detector, energy spectra of the LaBr3:Ce detector resulting from fast neutron interactions have been obtained at 4 different neutron energies. Neutron-induced gamma rays emitted by the LaBr3:Ce crystal were also measured in a nearby Ge detector at the lowest proton beam energy. In addition, we obtained data for neutron irradiation of a large-volume high-purity Ge detector and of a NE-213 liquid scintillator detector, both serving as monitor detectors in the experiment. Monte-Carlo type simulations for neutron interactions in the liquid scintillator, the Ge and LaBr3:Ce crystals have been performed and compared with measured data. Good agreement being obtained with the data, we present the results of simulations to predict the response of LaBr3:Ce detectors for a range of crystal sizes to neutron irradiation in the energy range En = 0.5-10 MeV
We characterize two 40 kBq sources of electrodeposited Th-228 for use in low-background experiments. The sources efficiently emanate Rn-220, a noble gas that can diffuse in a detector volume. Rn-220 and its daughter isotopes produce alpha, beta, and gamma-radiation, which may used to calibrate a variety of detector responses and features, before decaying completely in only a few days. We perform various tests to place limits on the release of other long-lived isotopes. In particular, we find an emanation of <0.008 atoms/min/kBq (90% CL) for Th-228 and 1.53 atoms/min/kBq for Ra-224. The sources lend themselves in particular to the calibration of detectors employing liquid noble elements such as argon and xenon. With the source mounted in a noble gas system, we demonstrate that filters are highly efficient in reducing the activity of these longer-lived isotopes further. We thus confirm the suitability of these sources even for use in next-generation experiments, such as XENON1T/XENONnT, LZ, and nEXO.
157 - D.S. Akerib , X. Bai , E. Bernard 2012
Results are presented from radioactivity screening of two models of photomultiplier tubes designed for use in current and future liquid xenon experiments. The Hamamatsu 5.6 cm diameter R8778 PMT, used in the LUX dark matter experiment, has yielded a positive detection of four common radioactive isotopes: 238U, 232Th, 40K, and 60Co. Screening of LUX materials has rendered backgrounds from other detector materials subdominant to the R8778 contribution. A prototype Hamamatsu 7.6 cm diameter R11410 MOD PMT has also been screened, with benchmark isotope counts measured at <0.4 238U / <0.3 232Th / <8.3 40K / 2.0+-0.2 60Co mBq/PMT. This represents a large reduction, equal to a change of times 1/24 238U / times 1/9 232Th / times 1/8 40K per PMT, between R8778 and R11410 MOD, concurrent with a doubling of the photocathode surface area (4.5 cm to 6.4 cm diameter). 60Co measurements are comparable between the PMTs, but can be significantly reduced in future R11410 MOD units through further material selection. Assuming PMT activity equal to the measured 90% upper limits, Monte Carlo estimates indicate that replacement of R8778 PMTs with R11410 MOD PMTs will change LUX PMT electron recoil background contributions by a factor of times1/25 after further material selection for 60Co reduction, and nuclear recoil backgrounds by a factor of times 1/36. The strong reduction in backgrounds below the measured R8778 levels makes the R11410 MOD a very competitive technology for use in large-scale liquid xenon detectors.
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