No Arabic abstract
Two-color multiphoton emission from polycrystalline tungsten nanotips has been demonstrated using two-color laser fields. The two-color photoemission is assisted by a three-photon multicolor quantum channel, which leads to a twofold increase in quantum efficiency. Weak-field control of two-color multiphoton emission was achieved by changing the efficiency of the quantum channel with pulse delay. The result of this study complements two-color tunneling photoemission in strong fields, and has potential applications for nanowire-based photonic devices. Moreover, the demonstrated two-color multiphoton emission may be important for realizing ultrafast spin-polarized electron sources via optically injected spin current.
We demonstrate cavity-enhanced Raman emission from a single atomic defect in a solid. Our platform is a single silicon-vacancy center in diamond coupled with a monolithic diamond photonic crystal cavity. The cavity enables an unprecedented frequency tuning range of the Raman emission (100 GHz) that significantly exceeds the spectral inhomogeneity of silicon-vacancy centers in diamond nanostructures. We also show that the cavity selectively suppresses the phonon-induced spontaneous emission that degrades the efficiency of Raman photon generation. Our results pave the way towards photon-mediated many-body interactions between solid-state quantum emitters in a nanophotonic platform.
Optical microcavities are a powerful tool to enhance spontaneous emission of individual quantum emitters. However, the broad emission spectra encountered in the solid state at room temperature limit the influence of a cavity, and call for ultra-small mode volume. We demonstrate Purcell-enhanced single photon emission from nitrogen-vacancy (NV) centers in nanodiamonds coupled to a tunable fiber-based microcavity with a mode volume down to $1.0,lambda^{3}$. We record cavity-enhanced fluorescence images and study several single emitters with one cavity. The Purcell effect is evidenced by enhanced fluorescence collection, as well as tunable fluorescence lifetime modification, and we infer an effective Purcell factor of up to 2.0. With numerical simulations, we furthermore show that a novel regime for light confinement can be achieved, where a Fabry-Perot mode is combined with additional mode confinement by the nanocrystal itself. In this regime, effective Purcell factors of up to 11 for NV centers and 63 for silicon vacancy centers are feasible, holding promise for bright single photon sources and efficient spin readout under ambient conditions.
We demonstrate a quantum nanophotonics platform based on germanium-vacancy (GeV) color centers in fiber-coupled diamond nanophotonic waveguides. We show that GeV optical transitions have a high quantum efficiency and are nearly lifetime-broadened in such nanophotonic structures. These properties yield an efficient interface between waveguide photons and a single GeV without the use of a cavity or slow-light waveguide. As a result, a single GeV center reduces waveguide transmission by $18 pm 1%$ on resonance in a single pass. We use a nanophotonic interferometer to perform homodyne detection of GeV resonance fluorescence. By probing the photon statistics of the output field, we demonstrate that the GeV-waveguide system is nonlinear at the single-photon level.
Some optomechanical systems can be transparent to a probe field when a strong driving field is applied. These systems can provide an optomechanical analogue of electromagnetically-induced transparency (EIT). We study the transmission of a probe field through a hybrid optomechanical system consisting of a cavity and a mechanical resonator with a two-level system (qubit). The qubit might be an intrinsic defect inside the mechanical resonator, a superconducting artificial atom, or another two-level system. The mechanical resonator is coupled to the cavity field via radiation pressure and to the qubit via the Jaynes-Cummings interaction. We find that the dressed two-level system and mechanical phonon can form two sets of three-level systems. Thus, there are two transparency windows in the discussed system. We interpret this effect as an optomechanical analog of two-color EIT (or double-EIT). We demonstrate how to switch between one and two EIT windows by changing the transition frequency of the qubit. We show that the absorption and dispersion of the system are mainly affected by the qubit-phonon coupling strength and the transition frequency of the qubit.
Stimulated emission and absorption are two fundamental processes of light-matter interaction, and the coefficients of the two processes should be equal in general. However, we will describe a generic method to realize significant difference between the stimulated emission and absorption coefficients of two nondegenerate energy levels, which we refer to as nonreciprocal transition. As a simple implementation, a cyclic three-level atom system, comprising two nondegenerate energy levels and one auxiliary energy level, is employed to show nonreciprocal transition via a combination of synthetic magnetism and reservoir engineering. Moreover, a single-photon nonreciprocal transporter is proposed using two one dimensional semi-infinite coupled-resonator waveguides connected by an atom with nonreciprocal transition effect. Our work opens up a route to design atom-mediated nonreciprocal devices in a wide range of physical systems.