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Register a new userPurcell-enhanced single-photon emission from nitrogen-vacancy centers coupled to a tunable microcavity
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Optical microcavities are a powerful tool to enhance spontaneous emission of individual quantum emitters. However, the broad emission spectra encountered in the solid state at room temperature limit the influence of a cavity, and call for ultra-small mode volume. We demonstrate Purcell-enhanced single photon emission from nitrogen-vacancy (NV) centers in nanodiamonds coupled to a tunable fiber-based microcavity with a mode volume down to $1.0,lambda^{3}$. We record cavity-enhanced fluorescence images and study several single emitters with one cavity. The Purcell effect is evidenced by enhanced fluorescence collection, as well as tunable fluorescence lifetime modification, and we infer an effective Purcell factor of up to 2.0. With numerical simulations, we furthermore show that a novel regime for light confinement can be achieved, where a Fabry-Perot mode is combined with additional mode confinement by the nanocrystal itself. In this regime, effective Purcell factors of up to 11 for NV centers and 63 for silicon vacancy centers are feasible, holding promise for bright single photon sources and efficient spin readout under ambient conditions.
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The nitrogen-vacancy (NV) center in diamond has been established as a prime building block for quantum networks. However, scaling beyond a few network nodes is currently limited by low spin-photon entanglement rates, resulting from the NV centers low probability of coherent photon emission and collection. Integration into a cavity can boost both values via the Purcell effect, but poor optical coherence of near-surface NV centers has so far prevented their resonant optical control, as would be required for entanglement generation. Here, we overcome this challenge, and demonstrate resonant addressing of individual, fiber-cavity-coupled NV centers, and collection of their Purcell-enhanced coherent photon emission. Utilizing off-resonant and resonant addressing protocols, we extract Purcell factors of up to 4, consistent with a detailed theoretical model. This model predicts that the probability of coherent photon detection per optical excitation can be increased to 10% for realistic parameters - an improvement over state-of-the art solid immersion lens collection systems by two orders of magnitude. The resonant operation of an improved optical interface for single coherent quantum emitters in a closed-cycle cryogenic system at T $sim$ 4 K is an important result towards extensive quantum networks with long coherence.
Hybrid quantum devices, in which disparate quantum elements are combined in order to achieve enhanced functionality, have received much attention in recent years due to their exciting potential to address key problems in quantum information processing, communication, and control. Specifically, significant progress has been made in the field of hybrid mechanical devices, in which a qubit is coupled to a mechanical oscillator. Strong coupling in such devices has been demonstrated with superconducting qubits, and coupling defect qubits to mechanical elements via crystal strain has enabled novel methods of qubit measurement and control. In this paper we demonstrate the fabrication of diamond optomechanical crystals with embedded nitrogen-vacancy (NV) centers, a preliminary step toward reaching the quantum regime with defect qubit hybrid mechanical devices. We measure optical and mechanical resonances of diamond optomechanical crystals as well as the spin coherence of single embedded NV centers. We find that the spin has long coherence times $T_2^* = 1.5 mu s$ and $T_2 = 72 mu s$ despite its proximity to nanofabricated surfaces. Finally, we discuss potential improvements of these devices and prospects for future experiments in the quantum regime.
We show that nitrogen-vacancy (NV) centers in diamond can produce a novel quantum hyperbolic metamaterial. We demonstrate that a hyperbolic dispersion relation in diamond with NV centers can be engineered and dynamically tuned by applying a magnetic field. This quantum hyperbolic metamaterial with a tunable window for the negative refraction allows for the construction of a superlens beyond the diffraction limit. In addition to subwavelength imaging, this NV-metamaterial can be used in spontaneous emission enhancement, heat transport and acoustics, analogue cosmology, and lifetime engineering. Therefore, our proposal interlinks the two hotspot fields, i.e., NV centers and metamaterials.
We propose a scheme to realize optical quantum memories in an ensemble of nitrogen-vacancy centers in diamond that are coupled to a micro-cavity. The scheme is based on off-resonant Raman coupling, which allows one to circumvent optical inhomogeneous broadening and store optical photons in the electronic spin coherence. This approach promises a storage time of order one second and a time-bandwidth product of order 10$^7$. We include all possible optical transitions in a 9-level configuration, numerically evaluate the efficiencies and discuss the requirements for achieving high efficiency and fidelity.
We demonstrate quantum interference between indistinguishable photons emitted by two nitrogen-vacancy (NV) centers in distinct diamond samples separated by two meters. Macroscopic solid immersion lenses are used to enhance photon collection efficiency. Quantum interference is verified by measuring a value of the second-order cross-correlation function $g^{(2)}(0) = 0.35 pm 0.04<0.5$. In addition, optical transition frequencies of two separated NV centers are tuned into resonance with each other by applying external electric fields. Extension of the present approach to generate entanglement of remote solid-state qubits is discussed.
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