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Register a new userTrapped ions in Rydberg-dressed atomic gases
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We theoretically study trapped ions that are immersed in an ultracold gas of Rydberg-dressed atoms. By off-resonant coupling on a dipole-forbidden transition, the adiabatic atom-ion potential can be made repulsive. We study the energy exchange between the atoms and a single trapped ion and find that Langevin collisions are inhibited in the ultracold regime for these repulsive interactions. Therefore, the proposed system avoids recently observed ion heating in hybrid atom-ion systems caused by coupling to the ions radio frequency trapping field and retains ultracold temperatures even in the presence of excess micromotion.
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In dense atomic gases the interaction between transition dipoles and photons leads to the formation of many-body states with collective dissipation and long-ranged forces. Despite decades of research, a full understanding of this paradigmatic many-body problem is still lacking. Here, we put forward and explore a scenario in which a dense atomic gas is weakly excited by an off-resonant laser field. We develop the theory for describing such dressed many-body ensembles and show that collective excitations are responsible for the emergence of many-body interactions, i.e. effective potentials that cannot be represented as a sum of binary terms. We illustrate how interaction effects may be probed through microwave spectroscopy via the analysis of time-dependent line-shifts, and show that these signals are sensitive to the phase pattern of the dressing laser. Our study offers a new perspective on dense atomic ensembles interacting with light and promotes this platform as a setting for the exploration of rich non-equilibrium many-body physics.
We provide a detailed theoretical and conceptual study of a planned experiment to excite Rydberg states of ions trapped in a Paul trap. The ultimate goal is to exploit the strong state dependent interactions between Rydberg ions to implement quantum information processing protocols and to simulate the dynamics of strongly interacting spin systems. We highlight the promises of this approach when combining the high degree of control and readout of quantum states in trapped ion crystals with the novel and fast gate schemes based on interacting giant Rydberg atomic dipole moments. We discuss anticipated theoretical and experimental challenges on the way towards its realization.
Conical intersections between electronic potential energy surfaces are paradigmatic for the study of non-adiabatic processes in the excited states of large molecules. However, since the corresponding dynamics occurs on a femtosecond timescale, their investigation remains challenging and requires ultrafast spectroscopy techniques. We demonstrate that trapped Rydberg ions are a platform to engineer conical intersections and to simulate their ensuing dynamics on larger length and time scales of the order of nanometers and microseconds, respectively; all this in a highly controllable system. Here, the shape of the potential energy surfaces and the position of the conical intersection can be tuned thanks to the interplay between the high polarizability and the strong dipolar exchange interactions of Rydberg ions. We study how the presence of a conical intersection affects both the nuclear and electronic dynamics demonstrating, in particular, how it results in the inhibition of the nuclear motion. These effects can be monitored in real-time via a direct spectroscopic measurement of the electronic populations in a state-of-the-art experimental setup.
We describe a simple approach to the problem of incorporating the response time of an atom or ion being Doppler-cooled into the theory of the cooling process. The system being cooled does not in general respond instantly to the changing laser frequencies it experiences in its rest frame, and this dynamic effect can affect significantly the temperatures attainable. It is particularly important for trapped ions when there is a slow decay out of the cooling cycle requiring the use of a repumping beam. We treat the cases of trapped ions with two and three internal states, then apply the theory to $^{40}{rm Ca}^+$. For this ion experimental data exist showing the ion to be cold under conditions for which heating is predicted if the dynamic effect is neglected. The present theory accounts for the observed behaviour.
We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of continuous driving fields to form a pair of dressed states essentially free of all relevant shifts. Specifically, the clock transition is robust to magnetic shifts, quadrupole and other tensor shifts, and amplitude fluctuations of the driving fields. The scheme is applicable to either a single ion or an ensemble of ions, and is relevant for several types of ions, such as $^{40}mathrm{Ca}^{+}$, $^{88}mathrm{Sr}^{+}$, $^{138}mathrm{Ba}^{+}$ and $^{176}mathrm{Lu}^{+}$. Taking a spherically symmetric Coulomb crystal formed by 400 $^{40}mathrm{Ca}^{+}$ ions as an example, we show through numerical simulations that the inhomogeneous linewidth of tens of Hertz in such a crystal together with linear Zeeman shifts of order 10~MHz are reduced to form a linewidth of around 1~Hz. We estimate a two-order-of-magnitude reduction in averaging time compared to state-of-the art single ion frequency references, assuming a probe laser fractional instability of $10^{-15}$. Furthermore, a statistical uncertainty reaching $2.9times 10^{-16}$ in 1~s is estimated for a cascaded clock scheme in which the dynamically decoupled Coulomb crystal clock stabilizes the interrogation laser for an $^{27}mathrm{Al}^{+}$ clock.
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