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We experimentally demonstrate ultrathin flat lenses with a thickness of 7 {AA}, which corresponds to the fundamental physical limit of the thickness of the material, is fabricated in a large area, monolayer, CVD-prepared tungsten chalcogenides single crystals using the low-cost flexible laser writing method. The lenses apply the ultra-high refractive index to introduce abrupt amplitude modulation of the incident light to achieve three-dimensional (3D) focusing diffraction-limited resolution (0.5{lambda}) and a focusing efficiency as high as 31%. An analytical physical model based diffraction theory is derived to simulate the focusing process, which shows excellent agreement with the experimental results.
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Two-dimensional (2D) materials have emerged as promising candidates for miniaturized optoelectronic devices, due to their strong inelastic interactions with light. On the other hand, a miniaturized optical system also requires strong elastic light-matter interactions to control the flow of light. Here, we report giant optical path length (OPL) from a single-layer molybdenum disulfide (MoS2), which is around one order of magnitude larger than that from a single-layer graphene. Using such giant OPL to engineer the phase front of optical beams, we demonstrated, to the best of our knowledge, the worlds thinnest optical lens consisting of a few layers of MoS2 less than 6.3 nm thick. Moreover, we show that MoS2 has much better dielectric response than good conductor (like gold) and other dielectric materials (like Si, SiO2 or graphene). By taking advantage of the giant elastic scattering efficiency in ultra-thin high-index 2D materials, we demonstrated high-efficiency gratings based on a single- or few-layers of MoS2. The capability of manipulating the flow of light in 2D materials opens an exciting avenue towards unprecedented miniaturization of optical components and the integration of advanced optical functionalities.
Cassegrain designs can be used to build thin lenses. We analyze the relationships between system thickness and aperture sizes of the two mirrors as well as FoV size. Our analysis shows that decrease in lens thickness imposes tight constraint on the aperture and FoV size. To mitigate this limitation, we propose to fill the gaps between the primary and the secondary with high index material. The Gassegrain optics cuts the track length into half and high index material reduces ray angle and height, consequently the incident ray angle can be increased, i.e., the FoV angle is extended. Defining telephoto ratio as the ratio of lens thickness to focal length, we achieve telephoto ratios as small as 0.43 for a visible Cassegrain thin lens and 1.20 for an infrared Cassegrain thin lens. To achieve an arbitrary FoV coverage, we present an strategy by integrating multiple thin lenses on one plane with each unit covering a different FoV region. To avoid physically tilting each unit, we propose beam steering with metasurface. By image stitching, we obtain wide FoV images.
Deep subwavelength integration of high-definition plasmonic nanostructures is of key importance for the development of future optical nanocircuitry for high-speed communication, quantum computation and lab-on-a-chip applications. So far the experimental realization of proposed extended plasmonic networks consisting of multiple functional elements remains challenging, mainly due to the multi-crystallinity of commonly used thermally evaporated gold layers. Resulting structural imperfections in individual circuit elements will drastically reduce the yield of functional integrated nanocircuits. Here we demonstrate the use of very large (>100 micron^2) but thin (<80 nm) chemically grown single-crystalline gold flakes, which, after immobilization, serve as an ideal basis for focused-ion beam milling and other top-down nanofabrication techniques on any desired substrate. Using this methodology we obtain high-definition ultrasmooth gold nanostructures with superior optical properties and reproducible nano-sized features over micrometer length scales. Our approach provides a possible solution to overcome the current fabrication bottleneck and to realize high-definition plasmonic nanocircuitry.
Stacked layers of metal meshes embedded in a dielectric substrate are routinely used for providing spectral selection at THz frequencies. Recent work has shown that particular geometries allow the refractive index to be tuned to produce practical artificial materials. Here we show that by spatially grading in the plane of the mesh we can manufacture a Graded Index (GrIn) thin flat lens optimized for use at THz frequencies. Measurements on a prototype lens show we are able to obtain the parabolic profile of a Woods type lens which is dependent only on the mesh parameters. This technique could realize other exotic optical devices.
One-dimensional (1D) materials have attracted significant research interest due to their unique quantum confinement effects and edge-related properties. Atomically thin 1D nanoribbon is particularly interesting because it is a valuable platform with physical limits of both thickness and width. Here, we develop a catalyst-free growth method and achieves the growth of Bi2O2Se nanostructures with tunable dimensionality. Significantly, Bi2O2Se nanoribbons with thickness down to 0.65 nm, corresponding to monolayer, are successfully grown for the first time. Electrical and optoelectronic measurements show that Bi2O2Se nanoribbons possess decent performance in terms of mobility, on/off ratio, and photoresponsivity, suggesting their promising for devices. This work not only reports a new method for the growth of atomically thin nanoribbons but also provides a platform to study properties and applications of such nanoribbon materials at thickness limit.
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