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Non-Hermitian coupled-mode theory for incoherently pumped exciton-polariton condensates

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 Added by Saeed Khan
 Publication date 2016
  fields Physics
and research's language is English




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The generalized Gross-Pitaevskii equation (gGPE) is an effective phenomenological description for the dynamics of incoherently pumped exciton-polariton condensates. However, a brute force numerical simulation of the gGPE provides little physical insight into condensate formation under arbitrary pumping configurations, and is demanding in terms of computational resources. We introduce in this paper a modal description of polariton condensation under incoherent pumping of arbitrary spatial profile, based on eigenmodes of the non-Hermitian generator of the linearized dynamics. A pump-dependent basis is then introduced to formulate a temporal coupled-mode theory that captures condensate dynamics in the presence of all nonlinear interactions. Simulations using a single set of modes for a given pumping and trapping configuration agree very well with a full integration of the gGPE in diverse dynamical regimes, supporting the validity of this modal description, while also providing a speedup in simulation times.



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We observe for the first time two-photon excited condensation of exciton-polaritons. The angle-resolved photoluminescence (PL) from the Lower Polariton (LP) ground state in our planar GaAs-based microcavity structure exhibits a clear intensity threshold as a function of increased two-photon excitation power, coinciding with an interaction-induced blueshift and a narrowing of spectral linewidth, characteristic of the transition from a thermal distribution of lower polaritons to polariton condensation. Two-Photon Absorption (TPA) is evidenced in the quadratic dependence of the input-output curves below and above the threshold region. Second Harmonic Generation (SHG) is ruled out by both this threshold behavior and by scanning the pump photon energy and observing a lack of dependence of the LP emission peak energy. Our results pave the way towards realization of a polariton-based stimulated THz radiation source, stemming from the dipole-allowed transition from the Quantum Well (QW) 2p dark exciton state to the 1s-exciton-based LP ground state, as theoretically predicted in [A. V. Kavokin et al., Phys. Rev. Lett. 108, 197401 (2012)].
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We examine the photoluminescence of highly-excited exciton-polariton condensates in semiconductor microcavities. Under strong pumping, exciton-polariton condensates have been observed to undergo a lasing transition where strong coupling between the excitons and photons is lost. We discuss an alternative high-density scenario, where the strong coupling is maintained. We find that the photoluminescence smoothly transitions between the lower polariton energy to the cavity photon energy. An intuitive understanding of the change in spectral characteristics is given, as well as differences to the photoluminescence characteristics of the lasing case.
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