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Register a new userPhotoluminescence of high-density exciton-polariton condensates
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We examine the photoluminescence of highly-excited exciton-polariton condensates in semiconductor microcavities. Under strong pumping, exciton-polariton condensates have been observed to undergo a lasing transition where strong coupling between the excitons and photons is lost. We discuss an alternative high-density scenario, where the strong coupling is maintained. We find that the photoluminescence smoothly transitions between the lower polariton energy to the cavity photon energy. An intuitive understanding of the change in spectral characteristics is given, as well as differences to the photoluminescence characteristics of the lasing case.
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We observe for the first time two-photon excited condensation of exciton-polaritons. The angle-resolved photoluminescence (PL) from the Lower Polariton (LP) ground state in our planar GaAs-based microcavity structure exhibits a clear intensity threshold as a function of increased two-photon excitation power, coinciding with an interaction-induced blueshift and a narrowing of spectral linewidth, characteristic of the transition from a thermal distribution of lower polaritons to polariton condensation. Two-Photon Absorption (TPA) is evidenced in the quadratic dependence of the input-output curves below and above the threshold region. Second Harmonic Generation (SHG) is ruled out by both this threshold behavior and by scanning the pump photon energy and observing a lack of dependence of the LP emission peak energy. Our results pave the way towards realization of a polariton-based stimulated THz radiation source, stemming from the dipole-allowed transition from the Quantum Well (QW) 2p dark exciton state to the 1s-exciton-based LP ground state, as theoretically predicted in [A. V. Kavokin et al., Phys. Rev. Lett. 108, 197401 (2012)].
We demonstrate, both experimentally and theoretically, a new phenomenon: the presence of dissipative coupling in the system of driven bosons. This is evidenced for a particular case of externally excited spots of exciton-polariton condensates in semiconductor microcavities. We observe that for two spatially separated condensates the dissipative coupling leads to the phase locking, either in-phase or out-of-phase, between the condensates. The effect depends on the distance between the condensates. For several excited spots, we observe the appearance of spontaneous vorticity in the system.
The quest to realise strongly interacting photons remains an outstanding challenge both for fundamental science and for applications. Here, we explore mediated photon-photon interactions in a highly imbalanced two-component mixture of exciton-polaritons in a semiconductor microcavity. Using a theory that takes into account non-perturbative correlations between the excitons as well as strong light-matter coupling, we demonstrate the high tunability of an effective interaction between quasiparticles formed by minority component polaritons interacting with a Bose-Einstein condensate (BEC) of a majority component polaritons. In particular, the interaction, which is mediated by the exchange of sound modes in the BEC can be made strong enough to support a bound state of two quasiparticles. Since these quasiparticles consist partly of photons, this in turn corresponds to a dimer state of photons propagating through the BEC. This gives rise to a new light transmission line where the bound state wave function is directly mapped onto correlations between outgoing photons. Our findings open up new routes for realising highly non-linear optical materials and novel hybrid light-matter quantum systems.
Optically pumping high quality semiconductor microcavities allows for the spontaneous formation of polariton condensates, which can propagate over distances of many microns. Tightly focussed pump spots here are found to produce expanding incoherent bottleneck polaritons which coherently amplify the ballistic polaritons and lead to the formation of unusual ring condensates. This quantum liquid is found to form a remarkable sunflower-like spatial ripple pattern which arises from self interference with Rayleigh-scattered coherent polariton waves in the Cerenkov regime.
We study driven-dissipative Bose-Einstein condensates in a two-mode Josephson system, such as a double-well potential, with asymmetrical pumping. We investigate nonlinear effects on the condensate populations and mode transitions. The generalized Gross-Pitaevskii equations are modified in order to treat pumping of only a single mode. We characterize the steady-state solutions in such a system as well as criteria for potential trapping of a condensate mode. There are many possible steady-states, with different density and/or phase profiles. Transitions between different condensate modes can be induced by varying the parameters of the junction or the initial conditions, or by applying external fields.
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