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Register a new userTwo-photon pumped exciton-polariton condensation
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Nadav Landau
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We observe for the first time two-photon excited condensation of exciton-polaritons. The angle-resolved photoluminescence (PL) from the Lower Polariton (LP) ground state in our planar GaAs-based microcavity structure exhibits a clear intensity threshold as a function of increased two-photon excitation power, coinciding with an interaction-induced blueshift and a narrowing of spectral linewidth, characteristic of the transition from a thermal distribution of lower polaritons to polariton condensation. Two-Photon Absorption (TPA) is evidenced in the quadratic dependence of the input-output curves below and above the threshold region. Second Harmonic Generation (SHG) is ruled out by both this threshold behavior and by scanning the pump photon energy and observing a lack of dependence of the LP emission peak energy. Our results pave the way towards realization of a polariton-based stimulated THz radiation source, stemming from the dipole-allowed transition from the Quantum Well (QW) 2p dark exciton state to the 1s-exciton-based LP ground state, as theoretically predicted in [A. V. Kavokin et al., Phys. Rev. Lett. 108, 197401 (2012)].
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The quest to realise strongly interacting photons remains an outstanding challenge both for fundamental science and for applications. Here, we explore mediated photon-photon interactions in a highly imbalanced two-component mixture of exciton-polaritons in a semiconductor microcavity. Using a theory that takes into account non-perturbative correlations between the excitons as well as strong light-matter coupling, we demonstrate the high tunability of an effective interaction between quasiparticles formed by minority component polaritons interacting with a Bose-Einstein condensate (BEC) of a majority component polaritons. In particular, the interaction, which is mediated by the exchange of sound modes in the BEC can be made strong enough to support a bound state of two quasiparticles. Since these quasiparticles consist partly of photons, this in turn corresponds to a dimer state of photons propagating through the BEC. This gives rise to a new light transmission line where the bound state wave function is directly mapped onto correlations between outgoing photons. Our findings open up new routes for realising highly non-linear optical materials and novel hybrid light-matter quantum systems.
We develop a theory for the dynamics of the density matrix describing a multimode polariton condensate. In such a condensate several single-particle orbitals become highly occupied, due to stimulated scattering from reservoirs of high-energy excitons. A generic few-parameter model for the system leads to a Lindblad equation which includes saturable pumping, decay, and condensate interactions. We show how this theory can be used to obtain the population distributions, and the time-dependent first- and second-order coherence functions, in such a multimode condensate. As a specific application, we consider a polaritonic Josephson junction, formed from a double-well potential. We obtain the population distributions, emission line shapes, and widths (first-order coherence functions), and predict the dephasing time of the Josephson oscillations.
We examine the photoluminescence of highly-excited exciton-polariton condensates in semiconductor microcavities. Under strong pumping, exciton-polariton condensates have been observed to undergo a lasing transition where strong coupling between the excitons and photons is lost. We discuss an alternative high-density scenario, where the strong coupling is maintained. We find that the photoluminescence smoothly transitions between the lower polariton energy to the cavity photon energy. An intuitive understanding of the change in spectral characteristics is given, as well as differences to the photoluminescence characteristics of the lasing case.
Modulational instabilities play a key role in a wide range of nonlinear optical phenomena, leading e.g. to the formation of spatial and temporal solitons, rogue waves and chaotic dynamics. Here we experimentally demonstrate the existence of a modulational instability in condensates of cavity polaritons, arising from the strong coupling of cavity photons with quantum well excitons. For this purpose we investigate the spatiotemporal coherence properties of polariton condensates in GaAs-based microcavities under continuous-wave pumping. The chaotic behavior of the instability results in a strongly reduced spatial and temporal coherence and a significantly inhomogeneous density. Additionally we show how the instability can be tamed by introducing a periodic potential so that condensation occurs into negative mass states, leading to largely improved coherence and homogeneity. These results pave the way to the exploration of long-range order in dissipative quantum fluids of light within a controlled platform.
We report the formation of a ring-shaped array of vortices after injection of angular momentum in a polariton superfluid. The angular momentum is injected by a $ell= 8$ Laguerre-Gauss beam, whereas the global rotation of the fluid is hindered by a narrow Gaussian beam placed at its center. In the linear regime a spiral interference pattern containing phase defects is visible. In the nonlinear (superfluid) regime, the interference disappears and the vortices nucleate as a consequence of the angular momentum quantization. The radial position of the vortices evolves freely in the region between the two pumps as a function of the density. Hydrodynamic instabilities resulting in the spontaneous nucleation of vortex-antivortex pairs when the system size is sufficiently large confirm that the vortices are not constrained by interference when nonlinearities dominate the system.
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