No Arabic abstract
Knowledge gained through X-ray crystallography fostered structural determination of materials and greatly facilitated the development of modern science and technology in the past century. Atomic details of sample structures is achievable by X-ray crystallography, however, it is only applied to crystalline structures. Imaging techniques based on X-ray coherent diffraction or zone plates are capable of resolving the internal structure of non-crystalline materials at nanoscales, but it is still a challenge to achieve atomic resolution. Here we demonstrate a novel lensless Fourier-transform ghost imaging method with pseudo-thermal hard X-rays by measuring the second-order intensity correlation function of the light. We show that high resolution Fourier-transform diffraction pattern of a complex amplitude sample can be achieved at Fresnel region and the amplitude and phase distributions of a sample in spatial domain can be retrieved successfully. The method of lensless X-ray Fourier-transform ghost imaging extends X-ray crystallography to non-crystalline samples, and its spatial resolution is limited only by the wavelength of the X-ray, thus atomic resolution should be routinely obtainable. Since highly coherent X-ray source is not required, comparing to conventional X-ray coherent diffraction imaging, the method can be implemented with laboratory X-ray sources, and it also provides a potential solution for lensless diffraction imaging with fermions, such as neutron and electron where the intensive coherent source usually is not available.
For conventional imaging, shaking of the imaging system or the target leads to the degradation of imaging resolution. In this work, the influence of the targets shaking to fourier-transform ghost diffraction (FGD) is investigated. The analytical results, which are backed up by numerical simulation and experiments, demonstrate that the quiver of target has no effect on the resolution of FGD, thus the targets imaging with high spatial resolution can be always achieved by phase-retrieval method from the FGD patterns. This approach can be applied in high-precision imaging systems, to overcome the influence of the systems shaking to imaging resolution.
Established x-ray diffraction methods allow for high-resolution structure determination of crystals, crystallized protein structures or even single molecules. While these techniques rely on coherent scattering, incoherent processes like Compton scattering or fluorescence emission -- often the predominant scattering mechanisms -- are generally considered detrimental for imaging applications. Here we show that intensity correlations of incoherently scattered x-ray radiation can be used to image the full 3D structure of the scattering atoms with significantly higher resolution compared to conventional coherent diffraction imaging and crystallography, including additional three-dimensional information in Fourier space for a single sample orientation. We present a number of properties of incoherent diffractive imaging that are conceptually superior to those of coherent methods.
Fourier analysis of ghost imaging (FAGI) is proposed in this paper to analyze the properties of ghost imaging with thermal light sources. This new theory is compatible with the general correlation theory of intensity fluctuation and could explain some amazed phenomena. Furthermore we design a series of experiments to verify the new theory and investigate the inherent properties of ghost imaging.
Recently, ghost imaging has been attracting attentions because its mechanism would lead to many applications inaccessible to conventional imaging methods. However, it is challenging for high contrast and high resolution imaging, due to its low signal-to-noise ratio (SNR) and the demand of high sampling rate in detection. To circumvent these challenges, we here propose a ghost imaging scheme that exploits Haar wavelets as illuminating patterns with a bi-frequency light projecting system and frequency-selecting single-pixel detectors. This method provides a theoretically 100% image contrast and high detection SNR, which reduces the requirement of high dynamic range of detectors, enabling high resolution ghost imaging. Moreover, it can highly reduce the sampling rate (far below Nyquist limit) for a sparse object by adaptively abandoning unnecessary patterns during the measurement. These characteristics are experimentally verified with a resolution of 512 times 512 and a sampling rate lower than 5%. A high-resolution (1000 times 1000 times 1000) 3D reconstruction of an object is also achieved from multi-angle images.
We present a lensless, Fourier-transform ghost imaging scheme by exploring the fourth-order correlation function of spatially incoherent thermal neutron waves. This technique is established on the Fermi-Dirac statistics and the anti-bunching effect of fermionic fields, and the analysis must be fully quantum mechanical. The spinor representation of neutron waves and the derivation purely from the Schrodinger equation makes our work the first, rigorous, robust and truly fermionic ghost imaging scheme. The investigation demonstrates that the coincidence of the intensity fluctuations between the reference arm and the sample arm is directly related to the lateral Fourier-transform of the longitudinal projection of the samples atomic and magnetic spatial distribution. By avoiding lens systems in neutron optics, our method can potentially achieve de Broglie wavelength level resolution, incomparable by current neutron imaging techniques. Its novel capability to image crystallined and noncrystallined samples, especially the micro magnetic structures, will bring important applications to various scientific frontiers.