No Arabic abstract
The complete characterisation of the charge transport in a mesoscopic device is provided by the Full Counting Statistics (FCS) $P_t(m)$, describing the amount of charge $Q = me$ transmitted during the time $t$. Although numerous systems have been theoretically characterized by their FCS, the experimental measurement of the distribution function $P_t(m)$ or its moments $langle Q^n rangle$ are rare and often plagued by strong back-action. Here, we present a strategy for the measurement of the FCS, more specifically its characteristic function $chi(lambda)$ and moments $langle Q^n rangle$, by a qubit with a set of different couplings $lambda_j$, $j = 1,dots,k,dots k+p$, $k = lceil n/2 rceil$, $p geq 0$, to the mesoscopic conductor. The scheme involves multiple readings of Ramsey sequences at the different coupling strengths $lambda_j$ and we find the optimal distribution for these couplings $lambda_j$ as well as the optimal distribution $N_j$ of $N = sum N_j$ measurements among the different couplings $lambda_j$. We determine the precision scaling for the moments $langle Q^n rangle$ with the number $N$ of invested resources and show that the standard quantum limit can be approached when many additional couplings $pgg 1$ are included in the measurement scheme.
We study analytically the full counting statistics of charge transport through single molecules, strongly coupled to a weakly damped vibrational mode. The specifics of transport in this regime - a hierarchical sequence of avalanches of transferred charges, interrupted by quiet periods - make the counting statistics strongly non-Gaussian. We support our findings for the counting statistics as well as for the frequency-dependent noise power by numerical simulations, finding excellent agreement.
Molecular electronics is a rapidly developing field focused on using molecules as the structural basis for electronic components. It is common in such devices for the system of interest to couple simultaneously to multiple environments. Here we consider a model comprised of a double quantum dot (or molecule) coupled strongly to vibrations and weakly to two electronic leads held at arbitrary bias voltage. The strong vibrational coupling invalidates treating the bosonic and electronic environments simply as acting additively, as would be the case in the weak coupling regime or for flat leads at infinite bias. Instead, making use of the reaction coordinate framework we incorporate the dominant vibrational coupling effects within an enlarged system Hamiltonian. This allows us to derive a non-additive form for the lead couplings that accounts properly for the influence of strong and non-Markovian coupling between the double dot system and the vibrations. Applying counting statistics techniques we track electron flow between the double dot and the electronic leads, revealing both strong-coupling and non-additive effects in the electron current, noise and Fano factor.
We develop a method for calculation of charge transfer statistics of persistent current in nanostructures in terms of the cumulant generating function (CGF) of transferred charge. We consider a simply connected one-dimensional system (a wire) and develop a procedure for the calculation of the CGF of persistent currents when the wire is closed into a ring via a weak link. For the non-interacting system we derive a general formula in terms of the two-particle Greens functions. We show that, contrary to the conventional tunneling contacts, the resulting cumulant generating function has a doubled periodicity as a function of the counting field. We apply our general formula to short tight-binding chains and show that the resulting CGF perfectly reproduces the known evidence for the persistent current. Its second cumulant turns out to be maximal at the switching points and vanishes identically at zero temperature. Furthermore, we apply our formalism for a computation of the charge transfer statistics of genuinely interacting systems. First we consider a ring with an embedded Anderson impurity and employing a self-energy approximation find an overall suppression of persistent current as well as of its noise. Finally, we compute the charge transfer statistics of a double quantum dot system in the deep Kondo limit using an exact analytical solution of the model at the Toulouse point. We analyze the behaviour of the resulting cumulants and compare them with those of a noninteracting double quantum dot system and find several pronounced differences, which can be traced back to interaction effects.
We develop a scheme for the computation of the full-counting statistics of transport described by Markovian master equations with an arbitrary time dependence. It is based on a hierarchy of generalized density operators, where the trace of each operator yields one cumulant. This direct relation offers a better numerical efficiency than the equivalent number-resolved master equation. The proposed method is particularly useful for conductors with an elaborate time-dependence stemming, e.g., from pulses or combinations of slow and fast parameter switching. As a test bench for the evaluation of the numerical stability, we consider time-independent problems for which the full-counting statistics can be computed by other means. As applications, we study cumulants of higher order for two time-dependent transport problems of recent interest, namely steady-state coherent transfer by adiabatic passage and Landau-Zener-Stuckelberg-Majorana interference in an open double quantum dot.
Stochastic systems feature, in general, both coherent dynamics and incoherent transitions between different states. We propose a method to identify the coherent part in the full counting statistics for the transitions. The proposal is illustrated for electron transfer through a quantum-dot spin valve, which combines quantum-coherent spin precession with electron tunneling. We show that by counting the number of transferred electrons as a function of time, it is possible to distill out the coherent dynamics from the counting statistics even in transport regimes, in which other tools such as the frequency-dependent current noise and the waiting-time distribution fail.