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Full counting statistics of strongly non-Ohmic transport through single molecules

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 Added by Felix von Oppen
 Publication date 2005
  fields Physics
and research's language is English




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We study analytically the full counting statistics of charge transport through single molecules, strongly coupled to a weakly damped vibrational mode. The specifics of transport in this regime - a hierarchical sequence of avalanches of transferred charges, interrupted by quiet periods - make the counting statistics strongly non-Gaussian. We support our findings for the counting statistics as well as for the frequency-dependent noise power by numerical simulations, finding excellent agreement.



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A mesoscopic Coulomb blockade system with two identical transport channels is studied in terms of full counting statistics. It is found that the average current cannot distinguish the quantum constructive interference from the classical non-interference, but the shot noise and skewness are more sensitive to the nature of quantum mechanical interference and can fulfill that task. The interesting super-Poisson shot noise is found and is demonstrated as a consequence of constructive interference, which induces an effective system with fast-and-slow transport channels. Dephasing effects on the counting statistics are carried out to display the continuous transition from quantum interfering to non-interfering transports.
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The complete characterisation of the charge transport in a mesoscopic device is provided by the Full Counting Statistics (FCS) $P_t(m)$, describing the amount of charge $Q = me$ transmitted during the time $t$. Although numerous systems have been theoretically characterized by their FCS, the experimental measurement of the distribution function $P_t(m)$ or its moments $langle Q^n rangle$ are rare and often plagued by strong back-action. Here, we present a strategy for the measurement of the FCS, more specifically its characteristic function $chi(lambda)$ and moments $langle Q^n rangle$, by a qubit with a set of different couplings $lambda_j$, $j = 1,dots,k,dots k+p$, $k = lceil n/2 rceil$, $p geq 0$, to the mesoscopic conductor. The scheme involves multiple readings of Ramsey sequences at the different coupling strengths $lambda_j$ and we find the optimal distribution for these couplings $lambda_j$ as well as the optimal distribution $N_j$ of $N = sum N_j$ measurements among the different couplings $lambda_j$. We determine the precision scaling for the moments $langle Q^n rangle$ with the number $N$ of invested resources and show that the standard quantum limit can be approached when many additional couplings $pgg 1$ are included in the measurement scheme.
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The internal dynamics of a double quantum dot system is renormalized due to coupling respectively with transport electrodes and a dissipative heat bath. Their essential differences are identified unambiguously in the context of full counting statistics. The electrode coupling caused level detuning renormalization gives rise to a fast-to-slow transport mechanism, which is not resolved at all in the average current, but revealed uniquely by pronounced super-Poissonian shot noise and skewness. The heat bath coupling introduces an interdot coupling renormalization, which results in asymmetric Fano factor and an intriguing change of line shape in the skewness.
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