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Register a new userSelf-consistent Description of Graphene Quantum Amplifier
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Added by
Nikolay Chtchelkatchev
Publication date
2016
fields
Physics
and research's language is
English
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High level of dissipation in normal metals makes challenging development of active and passive plasmonic devices. One possible solution to this problem is to use alternative materials. Graphene is a good candidate for plasmonics in near infrared (IR) region. In this paper we develop quantum theory of a graphene plasmon generator. We account for the first time quantum correlations and dissipation effects that allows describing such regimes of quantum plasmonic amplifier as surface plasmon emitting diode and surface plasmon amplifier by stimulated emission of radiation. Switching between these generation types is possible in situ with variance of graphene Fermi-level or gain transition frequency. We provide explicit expressions for dissipation and interaction constants through material parameters and find the generation spectrum and correlation function of second order which predicts laser statistics.
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Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other quantum emitters while the possibility of achieving strong second-order nonlinearities remains unexplored. Here, we describe a novel technique to realize such nonlinearities using graphene, exploiting the strong per-photon fields associated with tightly confined graphene plasmons in combination with spatially nonlocal nonlinear optical interactions. We show that in properly designed graphene nanostructures, these conditions enable extremely strong internal down-conversion between a single quantized plasmon and an entangled plasmon pair, or the reverse process of second harmonic generation. A separate issue is how such strong internal nonlinearities can be observed, given the nominally weak coupling between these plasmon resonances and free-space radiative fields. On one hand, by using the collective coupling to radiation of nanostructure arrays, we show that the internal nonlinearities can manifest themselves as efficient frequency conversion of radiative fields at extremely low input powers. On the other hand, the development of techniques to efficiently couple to single nanostructures would allow these nonlinear processes to occur at the level of single input photons.
The rapid generation of non-classical light serves as the foundation for exploring quantum optics and developing applications such as secure communication or generation of NOON-states. While strongly coupled quantum dot-photonic crystal resonator systems have great potential as non-classical light sources due to their promise of tailored output statistics, the generation of indistinguishable photons has been obscured due to the strongly dissipative nature of such systems. Here, we demonstrate that the recently discovered self-homodyne suppression technique can be used to overcome this limitation and tune the quantum statistics of transmitted light, achieving indistinguishable photon emission competitive with state-of-the-art metrics. Furthermore, our nanocavity-based platform directly lends itself to scalable on-chip architectures for quantum information.
We investigate the resonance energy transfer (RET) rate between two quantum emitters near a suspended graphene sheet in vacuum under the influence of an external magnetic field. We perform the analysis for low and room temperatures and show that, due to the extraordinary magneto-optical response of graphene, it allows for an active control and tunability of the RET even in the case of room temperature. We also demonstrate that the RET rate is extremely sensitive to small variations of the applied magnetic field, and can be tuned up to a striking six orders of magnitude for quite realistic values of magnetic field. Moreover, we evidence the fundamental role played by the magnetoplasmon polaritons supported by the graphene monolayer as the dominant channel for the RET within a certain distance range. Our results suggest that magneto-optical media may take the manipulation of energy transfer between quantum emitters to a whole new level, and broaden even more its great spectrum of applications.
Nonradiative transfer processes are often regarded as loss channels for an optical emitter1, since they are inherently difficult to be experimentally accessed. Recently, it has been shown that emitters, such as fluorophores and nitrogen vacancy centers in diamond, can exhibit a strong nonradiative energy transfer to graphene. So far, the energy of the transferred electronic excitations has been considered to be lost within the electron bath of the graphene. Here, we demonstrate that the trans-ferred excitations can be read-out by detecting corresponding currents with picosecond time resolution. We electrically detect the spin of nitrogen vacancy centers in diamond electronically and con-trol the nonradiative transfer to graphene by electron spin resonance. Our results open the avenue for incorporating nitrogen vacancy centers as spin qubits into ultrafast electronic circuits and for harvesting non-radiative transfer processes electronically.
We show that graphene-dielectric multilayers give rise to an unusual tunability of the Casimir-Lifshitz forces, and allow to easily realize completely different regimes within the same structure. Concerning thermal effects, graphene-dielectric multilayers take advantage from the anomalous features predicted for isolated suspended graphene sheets, even though they are considerably affected by the presence of the dielectric substrate. They can also archive the anomalous non-monotonic thermal metallic behavior by increasing the graphene sheets density and their Fermi energy. In addition to a strong thermal modulation occurring at short separations, in a region where the force is orders of magnitude larger than the one occurring at large distances, the force can be also adjusted by varying the number of graphene layers as well as their Fermi energy levels, allowing for relevant force amplifications which can be tuned, very rapidly and in-situ, by simply applying an electric potential. Our predictions can be relevant for both Casimir experiments and micro/nano electromechanical systems and in new devices for technological applications.
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