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Register a new userOptimizing a Dynamical Decoupling Protocol for Solid-State Electronic Spin Ensembles in Diamond
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We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to $77$ K suppresses longitudinal spin relaxation $T_1$ effects and DD microwave pulses are used to increase the transverse coherence time $T_2$ from $sim 0.7$ ms up to $sim 30$ ms. We extend previous work of single-axis (CPMG) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of AC magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.
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Ensembles of dopants have widespread applications in quantum technology. The miniaturization of corresponding devices is however hampered by dipolar interactions that reduce the coherence at increased dopant density. We theoretically and experimentally investigate this limitation. We find that dynamical decoupling can alleviate, but not fully eliminate, the decoherence in crystals with strong anisotropic spin-spin interactions. Our findings can be generalized to all quantum systems with anisotropic g-factor used for quantum sensing, microwave-to-optical conversion, and quantum memory.
In this paper we study how to preserve entanglement and nonlocality under dephasing produced by classical noise with large low-frequency components, as $1/f$ noise, by Dynamical Decoupling techniques. We first show that quantifiers of entanglement and nonlocality satisfy a closed relation valid for two independent qubits locally coupled to a generic environment under pure dephasing and starting from a general class of initial states. This result allows to assess the efficiency of pulse-based dynamical decoupling for protecting nonlocal quantum correlations between two qubits subject to pure-dephasing local random telegraph and $1/f$-noise. We investigate the efficiency of an entanglement memory element under two-pulse echo and under sequences of periodic, Carr-Purcell and Uhrig dynamical decoupling. The Carr-Purcell sequence is shown to outperform the other sequences in preserving entanglement against both random telegraph and $1/f$ noise. For typical $1/f$ flux-noise figures in superconducting nanocircuits, we show that entanglement and its nonlocal features can be efficiently stored up to times one order of magnitude longer than natural entanglement disappearance times employing pulse timings of current experimental reach.
We use multi-pulse dynamical decoupling to increase the coherence lifetime (T2) of large numbers of nitrogen-vacancy (NV) electronic spins in room temperature diamond, thus enabling scalable applications of multi-spin quantum information processing and metrology. We realize an order-of-magnitude extension of the NV multi-spin T2 for diamond samples with widely differing spin environments. For samples with nitrogen impurity concentration <~1 ppm, we find T2 > 2 ms, comparable to the longest coherence time reported for single NV centers, and demonstrate a ten-fold enhancement in NV multi-spin sensing of AC magnetic fields.
Spin systems in solid state materials are promising qubit candidates for quantum information or quantum sensing. A major prerequisite here is the coherence of spin phase oscillations. In this work, we show a control sequence which, by applying RF pulses of variable detuning, allows to increase the spin phase oscillation visibility and to perform DC magnetometry as well. We experimentally demonstrate the scheme on single NV centers in diamond and analytically describe how the NV electron spin phase oscillations behave in the presence of classical noise models. We hereby introduce detuning as the enabling factor that modulates the filter function of the sequence, in order to achieve a visibility of the Ramsey fringes comparable to or longer than the Hahn-echo $T_2$ time and an improved sensitivity to DC magnetic fields in various experimental settings.
We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that $pi$ rotations with small ($<$~10%) imperfections refocus instantaneous diffusion. Here, the intractable N-body problem of interacting dipoles is approximated by the average evolution of a single spin in a changing mean field. These calculations agree well with experiments and do not require powerful hardware. Our results add to past attempts to explain similar phenomena in solid state nuclear magnetic resonance (NMR). Although the fundamental physics of NMR are similar to ESR, the larger linewidths in ESR and stronger dipolar interactions between electron spins compared to nuclear spins preclude drawing conclusions from NMR studies alone. For bulk spins, we also find that using XYXY results in less inflation of the deduced echo decay times as compared to decays obtained with CPMG.
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