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Register a new userDynamical decoupling of spin ensembles with strong anisotropic interactions
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Ensembles of dopants have widespread applications in quantum technology. The miniaturization of corresponding devices is however hampered by dipolar interactions that reduce the coherence at increased dopant density. We theoretically and experimentally investigate this limitation. We find that dynamical decoupling can alleviate, but not fully eliminate, the decoherence in crystals with strong anisotropic spin-spin interactions. Our findings can be generalized to all quantum systems with anisotropic g-factor used for quantum sensing, microwave-to-optical conversion, and quantum memory.
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We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that $pi$ rotations with small ($<$~10%) imperfections refocus instantaneous diffusion. Here, the intractable N-body problem of interacting dipoles is approximated by the average evolution of a single spin in a changing mean field. These calculations agree well with experiments and do not require powerful hardware. Our results add to past attempts to explain similar phenomena in solid state nuclear magnetic resonance (NMR). Although the fundamental physics of NMR are similar to ESR, the larger linewidths in ESR and stronger dipolar interactions between electron spins compared to nuclear spins preclude drawing conclusions from NMR studies alone. For bulk spins, we also find that using XYXY results in less inflation of the deduced echo decay times as compared to decays obtained with CPMG.
We analyze numerically the performance of the near-optimal quadratic dynamical decoupling (QDD) single-qubit decoherence errors suppression method [J. West et al., Phys. Rev. Lett. 104, 130501 (2010)]. The QDD sequence is formed by nesting two optimal Uhrig dynamical decoupling sequences for two orthogonal axes, comprising N1 and N2 pulses, respectively. Varying these numbers, we study the decoherence suppression properties of QDD directly by isolating the errors associated with each system basis operator present in the system-bath interaction Hamiltonian. Each individual error scales with the lowest order of the Dyson series, therefore immediately yielding the order of decoherence suppression. We show that the error suppression properties of QDD are dependent upon the parities of N1 and N2, and near-optimal performance is achieved for general single-qubit interactions when N1=N2.
We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to $77$ K suppresses longitudinal spin relaxation $T_1$ effects and DD microwave pulses are used to increase the transverse coherence time $T_2$ from $sim 0.7$ ms up to $sim 30$ ms. We extend previous work of single-axis (CPMG) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of AC magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.
We show how dynamical decoupling (DD) and quantum error correction (QEC) can be optimally combined in the setting of fault tolerant quantum computing. To this end we identify the optimal generator set of DD sequences designed to protect quantum information encoded into stabilizer subspace or subsystem codes. This generator set, comprising the stabilizers and logical operators of the code, minimizes a natural cost function associated with the length of DD sequences. We prove that with the optimal generator set the restrictive local-bath assumption used in earlier work on hybrid DD-QEC schemes, can be significantly relaxed, thus bringing hybrid DD-QEC schemes, and their potentially considerable advantages, closer to realization.
Quantum information requires protection from the adverse affects of decoherence and noise. This review provides an introduction to the theory of decoherence-free subspaces, noiseless subsystems, and dynamical decoupling. It addresses quantum information preservation as well protected computation.
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