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Register a new userCooperative emission of a pulse train in an optically thick scattering medium
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An optically thick cold atomic cloud emits a coherent flash of light in the forward direction when the phase of an incident probe field is abruptly changed. Because of cooperativity, the duration of this phenomena can be much shorter than the excited lifetime of a single atom. Repeating periodically the abrupt phase jump, we generate a train of pulses with short repetition time, high intensity contrast and high efficiency. In this regime, the emission is fully governed by cooperativity even if the cloud is dilute.
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We consider the simultaneous propagation of a pair of Raman-resonant, frequency-modulated (chirped) laser pulses in an optically thick medium, modeled by an ensemble of $Lambda$-atoms. A self-organization (matching`) effect is shown for the chirped pulse pair, which leads to a quasi-lossless propagation. Furthermore, we demonstrate that a well-defined coherent superposition of the atomic ground states and, correspondingly, a coherence is robustly created in the medium that can be controlled by amplitudes of the laser pulses. The proposed scheme can be applied to substantially increase the efficiency of the optical wave mixing processes, as well as in other nonlinear processes where the initial preparation of a spatially extended medium in a coherent superposition state is required.
A means for precise experimental characterization of the dielectric susceptibility of an atomic gas inside and optical cavity is important for design and operation of quantum light matter interfaces, particularly in the context of quantum information processing. Here we present a numerically optimised theoretical model to predict the spectral response of an atom-filled cavity, accounting for both homogeneous and inhomogeneous broadening at high optical densities. We investigate the regime where the two broadening mechanisms are of similar magnitude, which makes the use of common approximations invalid. Our model agrees with an experimental implementation with warm caesium vapour in a ring cavity. From the cavity response, we are able to extract important experimental parameters, for instance the ground state populations, total number density and the magnitudes of both homogeneous and inhomogeneous broadening.
We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT generated through high-order harmonic generation (HHG) in argon we achieve a total pulse energy close to 1 $mu$J, a central energy of 35 eV and a total bandwidth of $sim30$ eV. The APT is focused by broadband optics in a neon gas target to an intensity of $3cdot10^{12} $W$cdot$cm$^{-2}$. By tuning the photon energy across the threshold for the sequential process the double ionization signal can be turned on and off, indicating that the two-photon double ionization predominantly occurs through a sequential process. The demonstrated performance opens up possibilities for future XUV-XUV pump-probe experiments with attosecond temporal resolution in a photon energy range where it is possible to unravel the dynamics behind direct vs. sequential double ionization and the associated electron correlation effects.
Scattering of light at a distribution of scatterers is an intrinsically cooperative process, which means that the scattering rate and the angular distribution of the scattered light are essentially governed by bulk properties of the distribution, such as its size, shape, and density, although local disorder and density fluctuations may have an important impact on the cooperativity. Via measurements of the radiation pressure exerted by a far-detuned laser beam on a very small and dense cloud of ultracold atoms, we are able to identify the respective roles of superradiant acceleration of the scattering rate and of Mie scattering in the cooperative process. They lead respectively to a suppression or an enhancement of the radiation pressure. We observe a maximum in the radiation pressure as a function of the induced phase shift, marking the borderline of the validity of the Rayleigh-Debye-Gans approximation from a regime, where Mie scattering is more complex. Our observations thus help to clarify the intricate relationship between Rayleigh scattering of light at a coarse-grained ensemble of individual scatterers and Mie scattering at the bulk density distribution.
Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic targets and reveal a quantum interference associated with different momentum components of the incident broadband electron pulse, which coherently modulates both the elastic and inelastic scattering cross sections. We show that the quantum interference has a high spatial sensitivity at the level of Angstroms, offering potential applications in high-resolution ultrafast electron microscopy. Our findings are rationalized by a simple model.
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