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Register a new userDirac Cones, Topological Edge States, and Nontrivial Flat Bands in Two-Dimensional Semiconductors with a Honeycomb Nanogeometry
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We study theoretically two-dimensional single-crystalline sheets of semiconductors that form a honeycomb lattice with a period below 10 nm. These systems could combine the usual semiconductor properties with Dirac bands. Using atomistic tight-binding calculations, we show that both the atomic lattice and the overall geometry influence the band structure, revealing materials with unusual electronic properties. In rocksalt Pb chalcogenides, the expected Dirac-type features are clouded by a complex band structure. However, in the case of zinc-blende Cd-chalcogenide semiconductors, the honeycomb nanogeometry leads to rich band structures, including, in the conduction band, Dirac cones at two distinct energies and nontrivial flat bands and, in the valence band, topological edge states. These edge states are present in several electronic gaps opened in the valence band by the spin-orbit coupling and the quantum confinement in the honeycomb geometry. The lowest Dirac conduction band has S-orbital character and is equivalent to the pi-pi* band of graphene but with renormalized couplings. The conduction bands higher in energy have no counterpart in graphene; they combine a Dirac cone and flat bands because of their P-orbital character. We show that the width of the Dirac bands varies between tens and hundreds of meV. These systems emerge as remarkable platforms for studying complex electronic phases starting from conventional semiconductors. Recent advancements in colloidal chemistry indicate that these materials can be synthesized from semiconductor nanocrystals.
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We study corner states on a flat band in the square lattice. To this end, we introduce a two dimensional model including Su-Schrieffer-Heeger type bond alternation responsible for corner states as well as next-nearest neighbor hoppings yielding flat bands. The key symmetry of the model for corner states is space-time inversion ($cal PT$) symmetry, which guarantees quantized Berry phases. This implies that edge states as well as corner states would show up if boundaries are introduced to the system. We also argue that an infinitesimal $cal PT$ symmetry-breaking perturbation could drive flat bands into flat Chern bands.
We prescribe general rules to predict the existence of edge states and zero-energy flat bands in graphene nanoribbons and graphene edges of arbitrary shape. No calculations are needed. For the so-called {it{minimal}} edges, the projection of the edge translation vector into the zigzag direction of graphene uniquely determines the edge bands. By adding extra nodes to minimal edges, arbitrary modified edges can be obtained. The edge bands of modified graphene edges can be found by applying hybridization rules of the extra atoms with the ones belonging to the original edge. Our prescription correctly predicts the localization and degeneracy of the zero-energy bands at one of the graphene sublattices, confirmed by tight-binding and first-principle calculations. It also allows us to qualitatively predict the existence of $E e 0$ bands appearing in the energy gap of certain edges and nanoribbons.
The intriguing properties, especially Dirac physics in graphene, have inspired the pursuit of two-dimensional materials in honeycomb structure. Here we achieved a monolayer transition metal monochalcogenide AgTe on Ag(111) by tellurization of the substrate. High-resolution scanning tunneling microscopy, combined with low-energy electron diffraction, angle-resolved photoemission spectroscopy, and density functional theory calculations, demonstrates the planar honeycomb structure of AgTe. The first principle calculations further reveal that, protected by the in-plane mirror reflection symmetry, two Dirac node-line Fermions exist in the electronic structures of free-standing AgTe when spin-orbit coupling (SOC) is ignored. While in fact the SOC leads to the gap opening, and resulting in the emergence of the topologically nontrivial quantum spin Hall edge state. Importantly, our experiments evidence the chemical stability of the monolayer AgTe in ambient conditions. It is possible to study AgTe by more ex-situ measurements and even to apply it in novel electronic devices.
We study the collective dynamics of a two-dimensional honeycomb lattice of magnetic skyrmions. By performing large-scale micromagnetic simulations, we find multiple chiral and non-chiral edge modes of skyrmion oscillations in the lattice. The non-chiral edge states are due to the Tamm-Shockley mechanism, while the chiral ones are topologically protected against structure defects and hold different handednesses depending on the mode frequency. To interpret the emerging multiband nature of the chiral edge states, we generalize the massless Thieles equation by including a second-order inertial term of skyrmion mass as well as a third-order non-Newtonian gyroscopic term, which allows us to model the band structure of skrymion oscillations. Theoretical results compare well with numerical simulations. Our findings uncover the importance of high order effects in strongly coupled skyrmions and are helpful for designing novel topological devices.
The extraordinary electronic properties of Dirac materials, the two-dimensional partners of Weyl semimetals, arise from the linear crossings in their band structure. When the dispersion around the Dirac points is tilted, the emergence of intricate transport phenomena has been predicted, such as modified Klein tunnelling, intrinsic anomalous Hall effects and ferrimagnetism. However, Dirac materials are rare, particularly with tilted Dirac cones. Recently, artificial materials whose building blocks present orbital degrees of freedom have appeared as promising candidates for the engineering of exotic Dirac dispersions. Here we take advantage of the orbital structure of photonic resonators arranged in a honeycomb lattice to implement photonic lattices with semi-Dirac, tilted and, most interestingly, type-III Dirac cones that combine flat and linear dispersions. The tilted cones emerge from the touching of a flat and a parabolic band with a non-trivial topological charge. These results open the way to the synthesis of orbital Dirac matter with unconventional transport properties and, in combination with polariton nonlinearities, to the study of topological and Dirac superfluids in photonic lattices.
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