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Entanglement, magnetic and quadrupole moments properties of the mixed spin Ising-Heisenberg diamond chain

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 Added by Nerses Ananikian
 Publication date 2014
  fields Physics
and research's language is English




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Thermal entanglement, magnetic and quadrupole moments properties of the mixed spin-1/2 and spin-1 Ising-Heisenberg model on a diamond chain are considered. Magnetization and quadrupole moment plateaus are observed for the antiferromagnetic couplings. Thermal negativity as a measure of quantum entanglement of the mixed spin system is calculated. Different behavior for the negativity is obtained for the various values of Heisenberg dipolar and quadrupole couplings. The intermediate plateau of the negativity has been observed at absence of the single-ion anisotropy and quadrupole interaction term. When dipolar and quadrupole couplings are equal there is a similar behavior of negativity and quadrupole moment.



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The mixed spin-(1,1/2) Ising-Heisenberg model on a distorted diamond chain with the spin-1 nodal atoms and the spin-1/2 interstitial atoms is exactly solved by the transfer-matrix method. An influence of the geometric spin frustration and the parallelogram distortion on the ground state, magnetization, susceptibility and specific heat of the mixed-spin Ising-Heisenberg distorted diamond chain are investigated in detail. It is demonstrated that the zero-temperature magnetization curve may involve intermediate plateaus just at zero and one-half of the saturation magnetization. The temperature dependence of the specific heat may have up to three distinct peaks at zero magnetic field and up to four distinct peaks at a non-zero magnetic field. The origin of multipeak thermal behavior of the specific heat is comprehensively studied.
We consider a geometrically frustrated spin-1/2 Ising-Heisenberg diamond chain, which is an exactly solvable model when assuming part of the exchange interactions as Heisenberg ones and another part as Ising ones. A small $XY$ part is afterwards perturbatively added to the Ising couplings, which enabled us to derive an effective Hamiltonian describing the low-energy behavior of the modified but full quantum version of the initial model. The effective model is much simpler and free of frustration. It is shown that the $XY$ part added to the originally Ising interaction gives rise to the spin-liquid phase with continuously varying magnetization, which emerges in between the magnetization plateaus and is totally absent in the initial hybrid diamond-chain model. The elaborated approach can also be applied to other hybrid Ising-Heisenberg spin systems.
The effect of the canting of local anisotropy axes on the ground-state phase diagram and magnetization of a ferrimagnetic chain with regularly alternating Ising and Heisenberg spins is exactly examined in an arbitrarily oriented magnetic field. It is shown that individual contributions of Ising and Heisenberg spins to the total magnetization basically depend on the spatial orientation of the magnetic field and the canting angle between two different local anisotropy axes of the Ising spins.
169 - T. Hosaka , S. Hachiuma , H. Kuroe 2011
We study the multiferroic properties in the distorted tetrahedral quasi-one dimensional spin system Cu$_3$Mo$_2$O$_9$, in which the effects of the low dimensionality and the magnetic frustration are expected to appear simultaneously. We clarify that the antiferromagnetic order is formed together with ferroelectric properties at $T_{rm N}=7.9$ K under zero magnetic field and obtain the magnetic-field-temperature phase diagram by measuring dielectric constant and spontaneous electric polarization. It is found that the antiferromagnetic phase possesses a spontaneous electric polarization parallel to the c axis when the magnetic field $H$ is applied parallel to the a axis. On the other hand, there are three different ferroelectric phases in the antiferromagnetic phase for $H$ parallel to the c axis.
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Exactly solvable frustrated quantum spin models consisting of a diamond unit structure are presented. The ground states are characterized by tetramer-dimer states with a macroscopic degeneracy in a certain range of isotropic exchange interaction. The lower bound of the excitation gap is exactly calculated to be finite and the bulk entropy in the limit of zero temperature remains finite depending on the shape of the boundary of system. Residual entropy is in a range of 0~6.1% of the entropy at high temperature for hexagonal diamond lattice and 0~8.4% for square diamond lattice. These diamond lattices are generalized to any dimensions and it is likely to be synthesized experimentally.
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