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Register a new userUniversal scaling of the critical temperature for thin films near the superconducting-to-insulating transition
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Thin superconducting films form a unique platform for geometrically-confined, strongly-interacting electrons. They allow an inherent competition between disorder and superconductivity, which in turn enables the intriguing superconducting-to-insulator transition and believed to facilitate the comprehension of high-Tc superconductivity. Furthermore, understanding thin film superconductivity is technologically essential e.g. for photo-detectors, and quantum-computers. Consequently, the absence of an established universal relationships between critical temperature ($T_c$), film thickness ($d$) and sheet resistance ($R_s$) hinders both our understanding of the onset of the superconductivity and the development of miniaturised superconducting devices. We report that in thin films, superconductivity scales as $d^.$$T_c(R_s)$. We demonstrated this scaling by analysing the data published over the past 46 years for different materials (and facilitated this database for further analysis). Moreover, we experimentally confirmed the discovered scaling for NbN films, quantified it with a power law, explored its possible origin and demonstrated its usefulness for superconducting film-based devices.
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We present a high-resolution microwave spectrometer to measure the frequency-dependent complex conductivity of a superconducting thin film near the critical temperature. The instrument is based on a broadband measurement of the complex reflection coefficient, $S_{rm 11}$, of a coaxial transmission line, which is terminated to a thin film sample with the electrodes in a Corbino disk shape. In the vicinity of the critical temperature, the standard calibration technique using three known standards fails to extract the strong frequency dependence of the complex conductivity induced by the superconducting fluctuations. This is because a small unexpected difference between the phase parts of $S_{rm 11}$ for a short and load standards gives rise to a large error in the detailed frequency dependence of the complex conductivity near the superconducting transition. We demonstrate that a new calibration procedure using the normal-state conductivity of a sample as a load standard resolves this difficulty. The high quality performance of this spectrometer, which covers the frequency range between 0.1 GHz and 10 GHz, the temperature range down to 10 K, and the magnetic field range up to 1 T, is illustrated by the experimental results on several thin films of both conventional and high temperature superconductors.
Copper oxide superconductors have continually fascinated the communities of condensed matter physics and material sciences because they host the highest ambient-pressure superconducting transition temperature (Tc) and mysterious physics. Searching for the universal correlation between the superconducting state and its normal state or neighboring ground state is believed to be an effective way for finding clues to elucidate the underlying mechanism of the superconductivity. One of the common pictures for the copper oxide superconductors is that a well-behaved metallic phase will present after the superconductivity is entirely suppressed by chemical doping or application of the magnetic field. Here, we report a different observation of universal quantum transition from superconducting state to insulating-like state under pressure in the under-, optimally- and over-doped Bi2212 superconductors with two CuO2 planes in a unit cell. The same phenomenon has been also found in the Bi2201 superconductor with one CuO2 plane and the Bi2223 superconductor with three CuO2 planes in a unit cell. These results not only provide fresh information but also pose a new challenge for achieving a unified understanding on the underlying physics of the high-Tc superconductivity.
Two principles govern the critical temperature for superconducting transitions: (1)~intrinsic strength of the pair coupling and (2)~effect of the many-body environment on the efficiency of that coupling. Most discussions take into account only the first but we argue that the properties of unconventional superconductors are governed more often by the second, through dynamical symmetry relating normal and superconducting states. Differentiating these effects is essential to charting a path to the highest-temperature superconductors.
FeTe, a non-superconducting parent compound in the iron-chalcogenide family, becomes superconducting after annealing in oxygen. Under the presence of magnetism, spin-orbit coupling, inhomogeneity and lattice distortion, the nature of its superconductivity is not well understood. Here, we combined mutual inductance technique with magneto transport to study the magnetization and superconductivity of FeTe thin films. We found that the films with the highest Tc showed non-saturating superfluid density and a strong magnetic hysteresis distinct from that in a homogeneous superconductor. Such hysteresis can be well explained by a two-level critical state model and suggested the importance of granularity to superconductivity in this compound.
By investigating the bulk superconducting state via dc magnetization measurements, we have discovered a common resurgence of the superconductive transition temperatures (Tcs) of the monolayer Bi2Sr2CuO6+{delta} (Bi2201) and bilayer Bi2Sr2CaCu2O8+{delta} (Bi2212) to beyond the maximum Tcs (Tc-maxs) predicted by the universal relation between Tc and doping (p) or pressure (P) at higher pressures. The Tc of under-doped Bi2201 initially increases from 9.6 K at ambient to a peak at ~ 23 K at ~ 26 GPa and then drops as expected from the universal Tc-P relation. However, at pressures above ~ 40 GPa, Tc rises rapidly without any sign of saturation up to ~ 30 K at ~ 51 GPa. Similarly, the Tc for the slightly overdoped Bi2212 increases after passing a broad valley between 20-36 GPa and reaches ~ 90 K without any sign of saturation at ~ 56 GPa. We have therefore attributed this Tc-resurgence to a possible pressure-induced electronic transition in the cuprate compounds due to a charge transfer between the Cu 3d_(x^2-y^2 ) and the O 2p bands projected from a hybrid bonding state, leading to an increase of the density of states at the Fermi level, in agreement with our density functional theory calculations. Similar Tc-P behavior has also been reported in the trilayer Br2Sr2Ca2Cu3O10+{delta} (Bi2223). These observations suggest that higher Tcs than those previously reported for the layered cuprate high temperature superconductors can be achieved by breaking away from the universal Tc-P relation through the application of higher pressures.
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