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Register a new userFrom Spin Glass to Quantum Spin Liquid Ground States in Molybdate Pyrochlores
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We present new magnetic heat capacity and neutron scattering results for two magnetically frustrated molybdate pyrochlores: $S=1$ oxide Lu$_2$Mo$_2$O$_7$ and $S={frac{1}{2}}$ oxynitride Lu$_2$Mo$_2$O$_5$N$_2$. Lu$_2$Mo$_2$O$_7$ undergoes a transition to an unconventional spin glass ground state at $T_f {sim} 16$ K. However, the preparation of the corresponding oxynitride tunes the nature of the ground state from spin glass to quantum spin liquid. The comparison of the static and dynamic spin correlations within the oxide and oxynitride phases presented here reveals the crucial role played by quantum fluctuations in the selection of a ground state. Furthermore, we estimate an upper limit for a gap in the spin excitation spectrum of the quantum spin liquid state of the oxynitride of ${Delta} {sim} 0.05$ meV or ${frac{Delta}{|theta|}}sim0.004$, in units of its antiferromagnetic Weiss constant ${theta} {sim}-121$ K.
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We propose the idea of a spin-lattice liquid, in which spin and lattice degrees of freedom are strongly coupled and remain disordered and fluctuating down to low temperatures. We show that such a state arises naturally from a microscopic analysis of a class of molybdate pyrochlore compounds, and is driven by a giant magnetoelastic effect. Finally, we argue that this could explain some of the experimental features of Y$_2$Mo$_2$O$_7$.
This article is an introductory review of the physics of quantum spin liquid (QSL) states. Quantum magnetism is a rapidly evolving field, and recent developments reveal that the ground states and low-energy physics of frustrated spin systems may develop many exotic behaviors once we leave the regime of semi-classical approaches. The purpose of this article is to introduce these developments. The article begins by explaining how semi-classical approaches fail once quantum mechanics become important and then describes the alternative approaches for addressing the problem. We discuss mainly spin $1/2$ systems, and we spend most of our time in this article on one particular set of plausible spin liquid states in which spins are represented by fermions. These states are spin-singlet states and may be viewed as an extension of Fermi liquid states to Mott insulators, and they are usually classified in the category of so-called $SU(2)$, $U(1)$ or $Z_2$ spin liquid states. We review the basic theory regarding these states and the extensions of these states to include the effect of spin-orbit coupling and to higher spin ($S>1/2$) systems. Two other important approaches with strong influences on the understanding of spin liquid states are also introduced: (i) matrix product states and projected entangled pair states and (ii) the Kitaev honeycomb model. Experimental progress concerning spin liquid states in realistic materials, including anisotropic triangular lattice systems ($kappa$-(ET)$_{2}$Cu$_{2}$(CN)$_{3}$ and EtMe$_{3}$Sb[(Pd(dmit)$_{2}$]$_{2}$), kagome lattice systems (ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$) and hyperkagome lattice systems (Na$_{4}$Ir$_{3}$O$_{8}$), is reviewed and compared against the corresponding theories.
The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions, materials closely related to the spin ices Ho2Ti2O7 and Dy2Ti2O7. Here we establish a general theory of magnetic order in these materials. We find that many of their most interesting properties can be traced back to the accidental degeneracies where phases with different symmetry meet. These include the ordered ground state selection by fluctuations in Er2Ti2O7, the dimensional-reduction observed in Yb2Ti2O7, and the absence of magnetic order in Er2Sn2O7.
Quantum spin liquids (QSLs) are exotic phases of matter exhibiting long-range entanglement and supporting emergent gauge fields. A vigorous search for experimental realizations of these states has identified several materials with properties hinting at QSL physics. A key issue in understanding these QSL candidates is often the interplay of weak disorder of the crystal structure with the spin liquid state. It has recently been pointed out that in at least one important class of candidate QSLs - pyrochlore magnets based on non-Kramers ions such as Pr$^{3+}$ or Tb$^{3+}$- structural disorder can actually promote a $U(1)$ QSL ground state. Here we set this proposal on a quantitative footing by analyzing the stability of the QSL state in the minimal model for these systems: a random transverse field Ising model. We consider two kinds of instability, which are relevant in different limits of the phase diagram: condensation of spinons and confinement of the $U(1)$ gauge fields. Having obtained stability bounds on the QSL state we apply our results directly to the disordered candidate QSL Pr$_2$Zr$_2$O$_7$. We find that the available data for currently studied samples of Pr$_2$Zr$_2$O$_7$ is most consistent with it a ground state outside the spin liquid regime, in a paramagnetic phase with quadrupole moments near saturation due to the influence of structural disorder.
We study AKLT models on locally tree-like lattices of fixed connectivity and find that they exhibit a variety of ground states depending upon the spin, coordination and global (graph) topology. We find a) quantum paramagnetic or valence bond solid ground states, b) critical and ordered Neel states on bipartite infinite Cayley trees and c) critical and ordered quantum vector spin glass states on random graphs of fixed connectivity. We argue, in consonance with a previous analysis, that all phases are characterized by gaps to local excitations. The spin glass states we report arise from random long ranged loops which frustrate Neel ordering despite the lack of randomness in the coupling strengths.
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