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Register a new userThermal Conductivity due to Spinons in the One-Dimensional Quantum Spin System Sr2V3O9
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We have measured the thermal conductivity along different directions of the S = 1/2 one-dimensional (1D) spin system Sr2V3O9 in magnetic fields up to 14 T. It has been found that the thermal conductivity along the [10-1] direction, k{appa}[10-1], is large and markedly suppressed by the application of magnetic field, indicating that there is a large contribution of spinons to k{appa}[10-1] and that the spin chains run along the [10-1] direction. The maximum value of the thermal conductivity due to spinons is ~14 W/Km along the [10-1] direction, supporting the empirical law that the magnitude of the thermal conductivity due to spinons is roughly proportional to the antiferromagnetic interaction between the nearest neighboring spins.
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We have measured the thermal conductivity along the c-axis parallel to the spin-chains, kappa_c, of the one-dimensional antiferromagnetic spin system SrCuO_2, using as-grown and O_2-annealed single-crystals grown from raw materials with 99.9% (3N) and 99.99% (4N) purity. The value of kappa_c around 50K, where large contribution of the thermal conductivity due to spinons, kappa_spinon, is observed, is markedly enhanced by both the increase of the purity of raw materials and the O_2-annealing. Therefore, the increase of kappa_c implies that kappa_spinon is enhanced due to the decrease of spin defects caused by impurities in raw materials and by oxygen defects. The mean free path of spinons is as large as about 24000 angstrom at low temperatures in the O_2-annealed single-crystal grown from raw materials with 4N purity.
We have measured the thermal conductivity along the [101] direction, kappa_[101]_, along the [10-1] direction, kappa_[10-1]_, and along the b-axis, kappa_b_, of the quasi one-dimensional S=1/2 spin system Sr_2_V_3_O_9_ in magnetic fields up to 14 T, in order to find the thermal conductivity due to spinons and to clarify whether the spin-chains run along the [101] or [10-1] direction. It has been found that both kappa_[101]_, kappa_[10-1]_ and kappa_b_ show one peak around 10 K in zero field and that the magnitude of kappa_[10-1]_ is larger than those of kappa_[101]_ and kappa_b_. By the application of magnetic field along the heat current, the peak of kappa_[10-1]_ is markedly suppressed, while the peaks of kappa_[101]_ and kappa_b_ little change. These results indicate that there is a large contribution of spinons to kappa_[10-1]_ and suggest that the spin-chains run along the [10-1] direction.
Observing constituent particles with fractional quantum numbers in confined and deconfined states is an interesting and challenging problem in quantum many-body physics. Here we further explore a computational scheme [Y. Tang and A. W. Sandvik, Phys. Rev. Lett. {bf 107}, 157201 (2011)] based on valence-bond quantum Monte Carlo simulations of quantum spin systems. Using several different one-dimensional models, we characterize $S=1/2$ spinon excitations using the spinon size and confinement length (the size of a bound state). The spinons have finite size in valence-bond-solid states, infinite size in the critical region, and become ill-defined in the Neel state. We also verify that pairs of spinons are deconfined in these uniform spin chains but become confined upon introducing a pattern of alternating coupling strengths (dimerization) or coupling two chains (forming a ladder). In the dimerized system an individual spinon can be small when the confinement length is large---this is the case when the imposed dimerization is weak but the ground state of the corresponding uniform chain is a spontaneously formed valence-bond-solid (where the spinons are deconfined). Based on our numerical results, we argue that the situation $lambda ll Lambda$ is associated with weak repulsive short-range spinon-spinon interactions. In principle both the length-scales can be individually tuned from small to infinite (with $lambda le Lambda$) by varying model parameters. In the ladder system the two lengths are always similar, and this is the case also in the dimerized systems when the corresponding uniform chain is in the critical phase. In these systems the effective spinon-spinon interactions are purely attractive and there is only a single large length scale close to criticality, which is reflected in the standard spin correlations as well as in the spinon characteristics.
Quantum spin systems exhibit an enormous range of collective excitations, but their spin waves, gapped triplons, fractional spinons, or yet other modes are generally held to be mutually exclusive. Here we show by neutron spectroscopy on SeCuO$_3$ that magnons, triplons, and spinons are present simultaneously. We demonstrate that this is a consequence of a structure consisting of two coupled subsystems and identify all the interactions of a minimal magnetic model. Our results serve qualitatively to open the field of multi-excitation spin systems and quantitatively to constrain the complete theoretical description of one member of this class of materials.
We have measured the thermal conductivity of the geometrically frustrated quasi-onedimensional spin system Cu$_3$Mo$_2$O$_9$ in magnetic fields. A contribution of the thermal conductivity due to spins has been observed in the thermal conductivity along the spin chains. The thermal conductivity due to phonons, $kappa_{rm phonon}$, has been found to decrease by the application of a magnetic field, which has been explained as being due to the reduction in the spin gap originating from the spin-singlet dimers. Moreover, it has been found that $kappa_{rm phonon}$ increases with increasing field in high fields above ~7 T at low temperatures. This suggests the existence of a novel field-induced spin state and is discussed in terms of the possible spin-chirality ordering in a frustrated Mott insulator.
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