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Register a new userThermal Conductivity of the Quasi One-Dimensional Spin System Sr_2_V_3_O_9_
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We have measured the thermal conductivity along the [101] direction, kappa_[101]_, along the [10-1] direction, kappa_[10-1]_, and along the b-axis, kappa_b_, of the quasi one-dimensional S=1/2 spin system Sr_2_V_3_O_9_ in magnetic fields up to 14 T, in order to find the thermal conductivity due to spinons and to clarify whether the spin-chains run along the [101] or [10-1] direction. It has been found that both kappa_[101]_, kappa_[10-1]_ and kappa_b_ show one peak around 10 K in zero field and that the magnitude of kappa_[10-1]_ is larger than those of kappa_[101]_ and kappa_b_. By the application of magnetic field along the heat current, the peak of kappa_[10-1]_ is markedly suppressed, while the peaks of kappa_[101]_ and kappa_b_ little change. These results indicate that there is a large contribution of spinons to kappa_[10-1]_ and suggest that the spin-chains run along the [10-1] direction.
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We have measured the thermal conductivity along different directions of the S = 1/2 one-dimensional (1D) spin system Sr2V3O9 in magnetic fields up to 14 T. It has been found that the thermal conductivity along the [10-1] direction, k{appa}[10-1], is large and markedly suppressed by the application of magnetic field, indicating that there is a large contribution of spinons to k{appa}[10-1] and that the spin chains run along the [10-1] direction. The maximum value of the thermal conductivity due to spinons is ~14 W/Km along the [10-1] direction, supporting the empirical law that the magnitude of the thermal conductivity due to spinons is roughly proportional to the antiferromagnetic interaction between the nearest neighboring spins.
We have measured the thermal conductivity along the c-axis parallel to the spin-chains, kappa_c, of the one-dimensional antiferromagnetic spin system SrCuO_2, using as-grown and O_2-annealed single-crystals grown from raw materials with 99.9% (3N) and 99.99% (4N) purity. The value of kappa_c around 50K, where large contribution of the thermal conductivity due to spinons, kappa_spinon, is observed, is markedly enhanced by both the increase of the purity of raw materials and the O_2-annealing. Therefore, the increase of kappa_c implies that kappa_spinon is enhanced due to the decrease of spin defects caused by impurities in raw materials and by oxygen defects. The mean free path of spinons is as large as about 24000 angstrom at low temperatures in the O_2-annealed single-crystal grown from raw materials with 4N purity.
We have measured the thermal conductivity of the geometrically frustrated quasi-onedimensional spin system Cu$_3$Mo$_2$O$_9$ in magnetic fields. A contribution of the thermal conductivity due to spins has been observed in the thermal conductivity along the spin chains. The thermal conductivity due to phonons, $kappa_{rm phonon}$, has been found to decrease by the application of a magnetic field, which has been explained as being due to the reduction in the spin gap originating from the spin-singlet dimers. Moreover, it has been found that $kappa_{rm phonon}$ increases with increasing field in high fields above ~7 T at low temperatures. This suggests the existence of a novel field-induced spin state and is discussed in terms of the possible spin-chirality ordering in a frustrated Mott insulator.
We study an incommensurate long-range order induced by an external magnetic field in a quasi-one-dimensional bond-alternating spin system, F5PNN, focusing on the role of the frustrating interaction which can be enhanced by a high-pressure effect. On the basis of the density matrix renormalization group analysis of a microscopic model for F5PNN, we present several H-T phase diagrams for typical parameters of the frustrating next-nearest-neighbour coupling and the interchain interaction, and then discuss how the field-induced incommensurate order develops by the frustration effect in such phase diagrams. A magnetization plateau at half the saturation moment is also mentioned.
The dynamical properties of free and bound domain-wall excitations in Ising-chain materials have recently become the focus of intense research interest. New materials and spectrometers have made it possible to control the environment of coupled Ising chains by both effective internal and applied external fields, which can be both longitudinal and transverse, and thus to demonstrate how the resulting magnetic phase transitions and the nature of the associated excited states obey fundamental symmetry properties. In RbCoCl$_3$, the weakly coupled Ising chains form a triangular lattice whose frustrated geometry and magnetic ordering transitions at low temperature open new possibilities for the Ising-chain environment. We have investigated the structure and magnetism in RbCoCl$_3$ by high-resolution x-ray diffraction and neutron scattering measurements on powder and single crystal samples between 1.5 K and 300 K. Upon cooling, the Co$^{2+}$ spins develop one-dimensional antiferromagnetic correlations along the chain axis ($c$-axis) below 90 K. Below the first Neel temperature, $T_{N1}$ = 28 K, a partial 3D magnetic order sets in, with propagation vector ${vec k}_1$ = (1/3,1/3,1), the moments aligned along the $c$-axis and every third chain uncorrelated from its neighbours. Only below a second magnetic phase transition at $T_{N2}$ = 13 K does the system achieve a fully ordered state, with two additional propagation vectors: ${vec k}_2$ = (0,0,1) establishes a honeycomb $c$-axis order, in which 1/3 of the chains are subject to a strong effective mean field due to their neighbours whereas 2/3 experience no net field, while ${vec k}_3$ = (1/2,0,1) governs a small, staggered in-plane ordered moment. We conclude that RbCoCl$_3$ is an excellent material to study the physics of Ising chains in a wide variety of temperature-controlled environments.
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