No Arabic abstract
The effect that dipole-dipole interactions have on the magneto-optical (MO) properties of magnetoplasmonic dimers is theoretically studied. The specific plasmonic versus magnetoplasmonic nature of the dimers metallic components and their specific location within the dimer plays a crucial role on the determination of these properties. We find that it is possible to generate an induced MO activity in a purely plasmonic component, even larger than that of the MO one, therefore dominating the overall MO spectral dependence of the system. Adequate stacking of these components may allow obtaining, for specific spectral regions, larger MO activities in systems with reduced amount of MO metal and therefore with lower optical losses. Theoretical results are contrasted and confirmed with experiments for selected structures.
Large surface plasmon polariton assisted enhancement of the magneto-optical activity has been observed in the past, through spectral measurements of the polar Kerr rotation in Co hexagonal antidot arrays. Here, we report a strong thickness dependence, which is unexpected given that the Kerr effect is considered a surface sensitive phenomena. The maximum Kerr rotation was found to be -0.66 degrees for a 100 nm thick sample. This thickness is far above the typical optical penetration depth of a continuous Co film, demonstrating that in the presence of plasmons the critical lengthscales are dramatically altered, and in this case extended. We therefore establish that the plasmon enhanced Kerr effect does not only depend on the in-plane structuring of the sample, but also on the out-of-plane geometrical parameters, which is an important consideration in magnetoplasmonic device design.
Intrinsically broken symmetries in the bulk of topological insulators (TIs) are manifested in their surface states. In spite of particle-hole asymmetry in TIs, it has often been assumed that their surface states are characterized by a particle-hole symmetric Dirac energy dispersion. In this work we demonstrate that the effect of particle-hole asymmetry is essential to correctly describe the energy spectrum and the magneto-optical response in TIs thin-films. In thin-films of TIs with a substantial degree of particle-hole symmetry breaking, such as Sb$_2$Te$_3$, the longitudinal optical conductivity displays absorption peaks arising from optical transitions between bulk and surface Landau levels for low photon energies. The transition energies between the bulk and surface Landau levels exhibit clearly discernable signatures from those between surface Landau levels due to their distinct magnetic field dependence. Bulk contributions to the magneto-optical conductivity in a TI thin-film are enhanced via one type of doping while being suppressed by the other. This asymmetric dependence on type of doping aids in revealing the particle-hole asymmetry in TI thin-films.
Magneto-optical transitions between Landau levels can provide precise spectroscopic information on the electronic structure and excitation spectra of graphene, enabling probes of substrate and many-body effects. We calculate the magneto-optical conductivity of large-size graphene flakes using a tight-binding approach. Our method allows us to directly compare the magneto-optical response of an isolated graphene flake with one aligned on hexagonal boron nitride giving rise to a periodic superlattice potential. The substrate interaction induces band gaps away from the Dirac point. In the presence of a perpendicular magnetic field Landau-level like structures emerge from these zero-field band gaps. The energy dependence of these satellite structures is, however, not easily accessible by conventional probes of the density of states by varying the back-gate voltage. Here we propose the magneto-optical probing of the superlattice perturbed spectrum. Our simulation includes magneto-excitonic effects in first-order perturbation theory. Our approach yields a quantitative explanation of recently observed Landau-level dependent renormalizations of the Fermi velocity.
The magneto-optical activity, namely the polarization conversion capabilities of high-index, non-absorbing, core-shell dielectric nanospheres is theoretically analyzed. We show that, in analogy with their plasmonic counterparts, the polarization conversion in resonant dielectric particles is linked to the amount of electromagnetic field probing the magneto-optical material in the system. However, in strong contrast with plasmon nanoparticles, due to the peculiar distribution of the internal fields in resonant dielectric spheres, the magneto-optical response is fully governed by the magnetic (dipolar and quadrupolar) resonances with little effect of the electric ones.
We demonstrate that yttrium iron garnet microspheres support optical whispering gallery modes similar to those in non-magnetic dielectric materials. The direction of the ferromagnetic moment tunes both the resonant frequency via the Voigt effect as well as the degree of polarization rotation via the Faraday effect. An understanding of the magneto-optical coupling in whispering gallery modes, where the propagation direction rotates with respect to the magnetization, is fundamental to the emerging field of cavity optomagnonics.