No Arabic abstract
Remote sensing of magnetic nanoparticles has exciting applications for magnetic nanoparticle hyperthermia and molecular detection. We introduce, simulate, and experimentally demonstrate an innovation---a sensing coil that is geometrically decoupled from the excitation field---for magnetic nanoparticle spectroscopy that increases the flexibility and capabilities of remote detection. The decoupling enhances the sensitivity absolutely; to small amounts of nanoparticles, and relatively; to small changes in the nanoparticle dynamics. We adapt a previous spectroscopic method that measures the relaxation time of nanoparticles and demonstrate a new measurement of nanoparticle temperature that could potentially be used concurrently during hyperthermia.
Using finite element micromagnetic simulations, we study how resonant magnetisation dynamics in thin magnetic discs with perpendicular anisotropy are influenced by magnetostatic coupling to a magnetic nanoparticle. We identify resonant modes within the disc using direct magnetic eigenmode calculations and study how their frequencies and profiles are changed by the nanoparticles stray magnetic field. We demonstrate that particles can generate shifts in the resonant frequency of the discs fundamental mode which exceed resonance linewidths in recently studied spin torque oscillator devices. Importantly, it is shown that the simulated shifts can be maintained over large field ranges (here up to 1T). This is because the resonant dynamics (the basis of nanoparticle detection here) respond directly to the nanoparticle stray field, i.e. detection does not rely on nanoparticle-induced changes to the magnetic ground state of the disk. A consequence of this is that in the case of small disc-particle separations, sensitivities to the particle are highly mode- and particle-position-dependent, with frequency shifts being maximised when the intense stray field localised directly beneath the particle can act on a large proportion of the discs spins that are undergoing high amplitude precession.
The spectral characteristics of near-field thermal emission from nanoparticle arrays are explained by comparison to the dispersions for propagating modes. Using the coupled dipole model, we analytically calculate the spectral emission from single particles, chains, planes, and 3D arrays of SiO2 and SiC. We show that the differences in their spectra are due to the existence or absence of propagating surface phonon polariton modes and that the emission is dominated by these modes when they are present. This work paves the way for understanding and control of near-field radiation in nanofluids, nanoparticle beds, and certain metamaterials.
The traditional theory of magnetic moments for chiral phonons is based on the picture of the circular motion of the Born effective charge, typically yielding a small fractional value of the nuclear magneton. Here we investigate the adiabatic evolution of electronic states induced by lattice vibration of a chiral phonon and obtain an electronic orbital magnetization in the form of a topological second Chern form. We find that the traditional theory needs to be refined by introducing a $bm{k}$ resolved Born effective charge, and identify another contribution from the phonon-modified electronic energy together with the momentum-space Berry curvature. The second Chern form can diverge when there is a Yangs monopole near the parameter space of interest as illustrated by considering a phonon at the Brillouin zone corner in a gaped graphene model. We also find large magnetic moments for the optical phonon in bulk topological materials where non-topological contribution is also important. The magnetic moment experiences a sign change when the band inversion happens.
A wire that conducts an electric current will give rise to circular magnetic field (the {O}rsted magnetic field) that is easily calculated using the Maxwell-Ampere equation. For wires with diameters in the macroscopic scale, this is an established physical law that has been demonstrated for two centuries. The Maxwell-Ampere equation is based on the argument that the induction of {O}rsted magnetic field is only a result of the displacement of charge. An alternative derivation of the {O}rsted magnetic field in conductors was suggested in [J. Mag. Mag. Mat. 504, 166660 (2020)] (will be called the current magnetization hypothesis (CMH) thereupon), which proposes that the {O}rsted magnetic field results from a two-body interaction. The present work establishes computationally, using simplified wire models, that the CMH reproduces the results of the Maxwell-Ampere equation for wires with a square cross section. Thus, CMH is proposed as a microscopic theory of magnetic induction, in contrast to the Maxwellian continuum theory of magnetic induction. I demonstrate that CMH could resolve the apparent contradiction between the observed induced magnetic field and that predicted by the Maxwell-Ampere equation in nanowires, as was reported in [Phys. Rev. B 99, 014436 (2019)]. The CMH shows that a possible reason for such contradiction is the presence of non-conductive surface layers in conductors.
We experimentally study magnetization dynamics in magnetic tunnel junctions driven by femtosecond-laser-induced surface acoustic waves. The acoustic pulses induce a magnetization precession in the free layer of the magnetic tunnel junction through magnetoelastic coupling. The frequency and amplitude of the precession shows a pronounced dependence on the applied magnetic field and the laser excitation position. Comparing the acoustic-wave-induced precession frequencies with precession induced by charge currents and with micromagnetic simulations we identify spatially non-uniform magnetization modes localized close the edge regions as being responsible for the optically induced magnetization dynamics. The experimental scheme even allows us to coherently control the magnetization precession using two acoustic pulses. This might prove important for future applications requiring ultrafast spin manipulation. Additionally, our results directly pinpoint the importance of acoustic pulses since they could be relevant when investigating optically-induced temperature effects in magnetic structures.