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When two or more metallic nanoparticles are in close proximity, their plasmonic modes may interact through the near field, leading to additional resonances of the coupled system or to shifts of their resonant frequencies. This process is analogous to atom-hybridization, as had been proposed by Gersten and Nitzan and modeled by Nordlander et al. The coupling between plasmonic modes can be in-phase (symmetric) or out-of-phase (anti-symmetric), reflecting correspondingly, the bonding and anti-bonding nature of such configurations. Since the incoming light redistributes the charge distribution around the metallic nanoparticles, its polarization features play a major role in the nonlinear optical probing of the energy-level landscape upon hybridization. Thus, controlling the nature of coupling between metallic nanostructures is of a great importance as it enables tuning their spectral responses leading to novel devices which may surpass the diffraction limit.
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Optimizing the shape of nanostructures and nano antennas for specific optical properties has evolved to be a very fruitful activity. With modern fabrication tools a large variety of possibilities is available for shaping both nanoparticles and nanocavities; in particular nanocavities in thin metal films have emerged as attractive candidates for new metamaterials and strong linear and nonlinear optical systems. Here we rationally design metallic nanocavities to boost their Four Wave Mixing response by resonating the optical plasmonic resonances with the incoming and generated beams. The linear and nonlinear optical responses as well as the propagation of the electric fields inside the cavities are derived from the solution of Maxwell equations by using the 3D finite-differences time domain method. The observed conversion-efficiency of near infra-red to visible light equals or surpasses that of BBO of equivalent thickness. Implications to further optimization for efficient and broadband ultrathin nonlinear optical materials are discussed.
Vibrational ultrastrong coupling (USC), where the light-matter coupling strength is comparable to the vibrational frequency of molecules, presents new opportunities to probe the interactions of molecules with zero-point fluctuations, harness cavity-enhanced chemical reactions, and develop novel devices in the mid-infrared regime. Here we use epsilon-near-zero nanocavities filled with a model polar medium (SiO$_2$) to demonstrate USC between phonons and gap plasmons. We present classical and quantum mechanical models to quantitatively describe the observed plasmon-phonon USC phenomena and demonstrate a splitting of up to 50% of the resonant frequency. Our wafer-scale nanocavity platform will enable a broad range of vibrational transitions to be harnessed for USC applications.
We find the exact Bloch oscillations in zigzag arrays of curved optical waveguides under the influence of arbitrary long-range coupling. The curvature induces a linear transverse potential gradient in the equations of the light evolution. In the case of arrays with second-order coupling, steady states can be obtained as linear combinations of Bessel functions of integer index. The corresponding eigenvalues are equally spaced and form the well-known Wannier-Stark ladder, the spacing being independent of the second-order coupling. We also solve exactly the wave packet dynamics and compare it with experimental results. Accordingly we find that a broad optical pulse performs Bloch oscillations. Frequency doubling of the fundamental Bloch frequency sets up at finite values of the second-order coupling. On the contrary when a single waveguide is initially excited, a breathing mode is activated with no signature of Bloch oscillations. We present a generalization of our results to waveguide arrays subject to long-range coupling. In the general case the centroid of the wave packet shows the occurrence of multiples of the Bloch frequency up to the order of the interaction.
We present a new approach to long range coupling based on a combination of adiabatic passage and lateral leakage in thin shallow ridge waveguides on a silicon photonic platform. The approach enables transport of light between two isolated waveguides through a mode of the silicon slab that acts as an optical bus. Due to the nature of the adiabatic protocol, the bus mode has minimal population and the transport is highly robust. We prove the concept and examine the robustness of this approach using rigorous modelling. We further demonstrate the utility of the approach by coupling power between two waveguides whilst bypassing an intermediate waveguide. This concept could form the basis of a new interconnect technology for silicon integrated photonic chips.
In the quest to enhance light-matter interactions and miniaturize photonics devices, it is crucial to create a strong field enhancement with lower material losses. Here we combine a plasmonic Fano resonance supported by the silver cluster and anapole states realized by the silicon disk to create a larger field enhancement with less loss through a strong coupling effect. Besides, by varying the gap size we find that the resonances wavelength and the Rabi-splitting can be tuned over a wide range of wavelength, which can achieve a giant splitting energy over 300 meV. We further demonstrate that it is the interference of magnetic currents loops which induces the strong coupling. Due to the strong coupling, the hybrid antenna can provide both larger decay rate and radiative decay rate, which makes it promising for high-performance miniaturized optical devices.
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