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Register a new userPhoton correlations for colloidal nanocrystals and their clusters
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Images of semiconductor `dot in rods and their small clusters are studied by measuring the second-order correlation function with a spatially resolving ICCD camera. This measurement allows one to distinguish between a single dot and a cluster and, to a certain extent, to estimate the number of dots in a cluster. A more advanced measurement is proposed, based on higher-order correlations, enabling more accurate determination of the number of dots in a small cluster. Nonclassical features of the light emitted by such a cluster are analyzed.
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Dynamical materials that capable of responding to optical stimuli have always been pursued for designing novel photonic devices and functionalities, of which the response speed and amplitude as well as integration adaptability and energy effectiveness are especially critical. Here we show ultrafast pulse generation by exploiting the ultrafast and sensitive nonlinear dynamical processes in tunably solution-processed colloidal epsilon-near-zero (ENZ) transparent conducting oxide (TCO) nanocrystals (NCs), of which the potential respond response speed is >2 THz and modulation depth is ~23% pumped at ~0.7 mJ/cm2, benefiting from the highly confined geometry in addition to the ENZ enhancement effect. These ENZ NCs may offer a scalable and printable material solution for dynamic photonic and optoelectronic devices.
This review describes an emerging field of waveguide quantum electrodynamics (WQED) studying interaction of photons propagating in a waveguide with localized quantum emitters. In such systems, atoms and guided photons are hybridized with each other and form polaritons that can propagate along the waveguide, contrary to the cavity quantum optics setup. Emerging in such a system collective light-atom interactions result in super- and sub-radiant quantum states, that are promising for quantum information processing, and give rise to peculiar quantum correlations between photons. The review is aimed at both experimentalists and theoreticians from various fields of physics interested in the rapidly developing subject of WQED. We highlight recent groundbreaking experiments performed for different quantum platforms, including cold atoms, superconducting qubits, semiconductor quantum dots, quantum solid-state defects and at the same time provide a comprehensive introduction into various theoretical techniques to study atom-photon interactions in the waveguide.
Solution processible colloidal quantum dots hold great promise for realizing single-photon sources embedded into scalable quantum technology platforms. However, the high-yield integration of large numbers of individually addressable colloidal quantum dots in a photonic circuit has remained an outstanding challenge. Here, we report on integrating individual colloidal core-shell quantum dots (CQDs) into a nanophotonic network that allows for excitation and efficient collection of single-photons via separate waveguide channels. An iterative electron beam lithography process provides a viable method to position single emitters at predefined positions in a photonic integrated circuit with yield that approaches unity. Our work moves beyond the bulk optic paradigm of confocal microscopy and paves the way for supplying chip-scale quantum networks with single photons from large numbers of simultaneously controllable quantum emitters.
We consider the propagation of classical and non-classical light in multi-mode optical waveguides. We focus on the evolution of the few-photon correlation functions, which, much like the light-intensity distribution in such systems, evolve in a periodic manner, culminating in the revival of the initial correlation pattern at the end of each period. It is found that when the input state possesses non trivial symmetries, the correlation revival period can be longer than that of the intensity, and thus the same intensity pattern can display different correlation patterns. We experimentally demonstrate this effect for classical, pseudo-thermal light, and compare the results with the predictions for non-classical, quantum light.
Elevated-temperature polyol-based colloidal-chemistry approach allows for the development of size-tunable (50 and 86 nm) assemblies of maghemite iso-oriented nanocrystals, with enhanced magnetization. 1H-Nuclear Magnetic Resonance (NMR) relaxometric experiments show that the ferrimagnetic cluster-like colloidal entities exhibit a remarkable enhancement (4 to 5 times) in the transverse relaxivity, if compared to that of the superparamagnetic contrast agent Endorem, over an extended frequency range (1-60 MHz). The marked increase of the transverse relaxivity r2 at a clinical magnetic field strength (1.41 T), which is 405.1 and 508.3 mM-1 s-1 for small and large assemblies respectively, allows to relate the observed response to the raised intra-aggregate magnetic material volume fraction. Furthermore, cell tests with murine fibroblast culture medium confirmed the cell viability in presence of the clusters. We discuss the NMR dispersion profiles on the basis of relaxivity models to highlight the magneto-structural characteristics of the materials for improved T2-weighted magnetic resonance images.
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