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Register a new userEffects of Neutron Irradiation on Pinning Force Scaling in State-of-the-Art Nb3Sn Wires
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Thomas Baumgartner Ph.D.
Publication date
2013
fields
Physics
and research's language is
English
Authors
T. Baumgartner
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We present an extensive irradiation study involving five state-of-the-art Nb3Sn wires which were subjected to sequential neutron irradiation up to a fast neutron fluence of 1.6 * 10^22 m^-2 (E > 0.1 MeV). The volume pinning force of short wire samples was assessed in the temperature range from 4.2 to 15 K in applied fields of up to 7 T by means of SQUID magnetometry in the unirradiated state and after each irradiation step. Pinning force scaling computations revealed that the exponents in the pinning force function differ significantly from those expected for pure grain boundary pinning, and that fast neutron irradiation causes a substantial change in the functional dependence of the volume pinning force. A model is presented, which describes the pinning force function of irradiated wires using a two-component ansatz involving a point-pinning contribution stemming from radiation induced pinning centers. The dependence of this point-pinning contribution on fast neutron fluence appears to be a universal function for all examined wire types.
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Pinning force data, Fp, of a variety of Fe-based high-Tc superconductors (11-, 111-, 122- and 1111-type) were analyzed by means of a scaling approach based on own experimental data and an extensive collection of literature data. The literature data were mostly replotted, but also converted from critical current measurements together with data for the irreversibility line when available from the same authors. Using the scaling approaches of Dew-Hughes and Kramer, we determined the scaling behavior and the best fits to the theory. The data of most experiments analyzed show a good scaling behavior at high temperatures when plotting the normalized pinning force Fp/Fp,max versus the irreversibility field, Hirr. The resulting peak positions, h0, were found at 0.3 for the 11-type materials, at 0.48 for the 111-type materials, between 0.32 and 0.5 for the 1111-type materials and between 0.25 and 0.71 for the 122-type materials. This high peak position ensures a good performance of the materials in high applied magnetic fields and is, therefore, a very promising result concerning the possible applications of the Fe-based high-Tc superconductors.
In powder-in-tube (PIT) Nb3Sn composites, the A15 phase forms between a central tin-rich core and a coaxial Nb tube, thus causing the tin content and superconducting properties to vary with radius across the A15 layer. Since this geometry is also ideal for magnetic characterization of the superconducting properties with the field parallel to the tube axis, a system of concentric shells with varying tin content was used to simulate the superconducting properties, the overall severity of the Sn composition gradient being defined by an index N. Using well-known scaling relationships and property trends developed in an earlier experimental study, the critical current density for each shell was calculated, and from this the magnetic moment of each shell was found. By summing these moments, experimentally measured properties such as pinning-force curves and Kramer plots could be simulated. We found that different tin profiles have only a minor effect on the shape of Kramer plots, but a pronounced effect on the irreversibility fields defined by the extrapolation of Kramer plots. In fact, these extrapolated values H_K are very close to a weighted average of the superconducting properties across the layer for all N. The difference between H_K and the upper critical field commonly seen in experiments is a direct consequence of the different ways measurements probe the simulated Sn gradients. Sn gradients were found to be significantly deleterious to the critical current density Jc, since reductions to both the elementary pinning force and the flux pinning scaling field H_K compound the reduction in Jc. The simulations show that significant gains in Jc of Nb3Sn strands might be realized by circumventing strong compositional gradients of tin.
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Sintered samples of MgB2 were irradiated in a fission reactor. Defects in the bulk microstructure are produced during this process mainly by the 10B(n,a)7Li reaction while collisions of fast neutrons with the lattice atoms induce much less damage. Self-shielding effects turn out to be very important and lead to a highly inhomogeneous defect distribution in the irradiated samples. The resulting disorder enhances the normal state resistivity and the upper critical field. The irreversibility line shifts to higher fields at low temperatures and the measured critical current densities increase following irradiation.
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