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Register a new userElectric field gradient wave (EFGW) in iron-based superconductor Ba(0.6)K(0.4)Fe2As2 studied by Mossbauer spectroscopy
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Added by
Krzysztof Ruebenbauer
Publication date
2013
fields
Physics
and research's language is
English
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The optimally doped 122 iron-based superconductor Ba(0.6)K(0.4)Fe2As2 has been studied by 57Fe Moessbauer spectroscopy versus temperature ranging from 4.2 K till 300 K with particular attention paid to the superconducting transition around 38 K. The spectra do not contain magnetic components and they exhibit quasi-continuous distribution of quadrupole split doublets. A distribution follows the electric field gradient (EFG) spatial modulation (wave) - EFGW. The EFGW is accompanied by some charge density wave (CDW) having about an order of magnitude lesser influence on the spectrum. The EFGW could be modeled as widely separated narrow sheets with the EFG increasing from small till maximum value almost linearly and subsequently dropping back to the original value in a similar fashion - across the sheet. One encounters very small and almost constant EFG between sheets. The EFGW shape and amplitude as well as the amplitude of CDW are strongly affected by a superconducting transition. All modulations are damped significantly at transition (38 K) and recover at a temperature being about 14 K lower. The maximum quadrupole splitting at 4.2 K amounts to about 2.1 mm/s, while the dispersion of CDW seen on the iron nuclei could be estimated far away from the superconducting gap opening and at low temperature as 0.5 el./a.u.^3. It drops to about 0.3 el./a.u.^3 just below transition to the superconducting state.
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The nature of the pairing state in iron-based superconductors is the subject of much debate. Here we argue that in one material, the stoichiometric iron pnictide KFe2As2, there is overwhelming evidence for a d-wave pairing state, characterized by symmetry-imposed vertical line nodes in the superconducting gap. This evidence is reviewed, with a focus on thermal conductivity and the strong impact of impurity scattering on the critical temperature Tc. We then compare KFe2As2 to Ba0.6K0.4Fe2As2, obtained by Ba substitution, where the pairing symmetry is s-wave and the Tc is ten times higher. The transition from d-wave to s-wave within the same crystal structure provides a rare opportunity to investigate the connection between band structure and pairing mechanism. We also compare KFe2As2 to the nodal iron-based superconductor LaFePO, for which the pairing symmetry is probably not d-wave, but more likely s-wave with accidental line nodes.
We used high-resolution scanning tunneling spectroscopy to study the hole-doped iron pnictide superconductor Ba$_{0.6}$K$_{0.4}$Fe$_{2}$As$_{2}$ ($T_c=38$ K). Features of a bosonic excitation (mode) are observed in the measured quasiparticle density of states. The bosonic features are intimately associated with the superconducting order parameter and have a mode energy of $sim$14 meV, similar to the spin resonance measured by inelastic neutron scattering. These results indicate a strong electron-spin excitation coupling in iron pictnide superconductors, similar to that in high-$T_c$ copper oxide superconductors.
In unconventional superconductors, it is generally believed that understanding the physical properties of the normal state is a pre-requisite for understanding the superconductivity mechanism. In conventional superconductors like niobium or lead, the normal state is a Fermi liquid with a well-defined Fermi surface and well-defined quasipartcles along the Fermi surface. Superconductivity is realized in this case by the Fermi surface instability in the superconducting state and the formation and condensation of the electron pairs (Cooper pairing). The high temperature cuprate superconductors, on the other hand, represent another extreme case that superconductivity can be realized in the underdoped region where there is neither well-defined Fermi surface due to the pseudogap formation nor quasiparticles near the antinodal regions in the normal state. Here we report a novel scenario that superconductivity is realized in a system with well-defined Fermi surface but without quasiparticles along the Fermi surface in the normal state. High resolution laser-based angle-resolved photoemission measurements have been performed on an optimally-doped iron-based superconductor (Ba$_{0.6}$K$_{0.4}$)Fe$_2$As$_2$. We find that, while sharp superconducting coherence peaks emerge in the superconducting state on the hole-like Fermi surface sheets, no quasiparticle peak is present in the normal state. Its electronic behaviours deviate strongly from a Fermi liquid system. The superconducting gap of such a system exhibits an unusual temperature dependence that it is nearly a constant in the superconducting state and abruptly closes at T$_c$. These observations have provided a new platform to study unconventional superconductivity in a non-Fermi liquid system.
We show that electronic Raman scattering affords a window into the essential properties of the pairing potential $V_{mathbf{k},mathbf{k^{prime}}}$ of iron-based superconductors. In Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ we observe band dependent energy gaps along with excitonic Bardasis-Schrieffer modes characterizing, respectively, the dominant and subdominant pairing channel. The $d_{x^2-y^2}$ symmetry of all excitons allows us to identify the subdominant channel to originate from the interaction between the electron bands. Consequently, the dominant channel driving superconductivity results from the interaction between the electron and hole bands and has the full lattice symmetry. The results in Rb$_{0.8}$Fe$_{1.6}$Se$_2$ along with earlier ones in Ba(Fe$_{0.939}$Co$_{0.061}$)$_2$As$_2$ highlight the influence of the Fermi surface topology on the pairing interactions.
We have performed 31P-NMR measurements on the s-wave superconductor LaRu4P12 to investigate the magnetic field effect of the nuclear spin-lattice relaxation rate 1/T1 on a conventional full-gap superconductor. With increasing magnetic field, the Hebel-Slichter peak immediately below Tc in 1=T1 was suppressed, and the magnetic field dependence of 1/T1 at 0.8 K, well below Tc, was proportional to H2. These behaviors can be fully understood by the orbital pair-breaking effect in a single-band s-wave superconductor
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