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Register a new userRaman-Scattering Detection of Nearly Degenerate $s$-Wave and $d$-Wave Pairing Channels in Iron-Based Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ and Rb$_{0.8}$Fe$_{1.6}$Se$_2$ Superconductors
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Added by
Florian Kretzschmar
Publication date
2012
fields
Physics
and research's language is
English
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We show that electronic Raman scattering affords a window into the essential properties of the pairing potential $V_{mathbf{k},mathbf{k^{prime}}}$ of iron-based superconductors. In Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ we observe band dependent energy gaps along with excitonic Bardasis-Schrieffer modes characterizing, respectively, the dominant and subdominant pairing channel. The $d_{x^2-y^2}$ symmetry of all excitons allows us to identify the subdominant channel to originate from the interaction between the electron bands. Consequently, the dominant channel driving superconductivity results from the interaction between the electron and hole bands and has the full lattice symmetry. The results in Rb$_{0.8}$Fe$_{1.6}$Se$_2$ along with earlier ones in Ba(Fe$_{0.939}$Co$_{0.061}$)$_2$As$_2$ highlight the influence of the Fermi surface topology on the pairing interactions.
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We have successfully grown high quality single crystals of SrFe$_2$As$_2$ and A$_{0.6}$K$_{0.4}$Fe$_2$As$_2$(A=Sr, Ba) using flux method. The resistivity, specific heat and Hall coefficient have been measured. For parent compound SrFe$_2$As$_2$, an anisotropic resistivity with $rho_c$ / $rho_{ab}$ as large as 130 is obtained at low temperatures. A sharp drop in both in-plane and out-plane resistivity due to the SDW instability is observed below 200 K. The angular dependence of in-plane magnetoresistance shows 2-fold symmetry with field rotating within ab plane below SDW transition temperature. This is consistent with a stripe-type spin ordering in SDW state. In K doped A$_{0.6}$K$_{0.4}$Fe$_2$As$_2$(A=Sr. Ba), the SDW instability is suppressed and the superconductivity appears with T$_c$ above 35 K. The rather low anisotropy in upper critical field between H$parallel$ab and H$parallel$c indicates inter-plane coupling play an important role in hole doped Fe-based superconductors.
The magnetic properties of iron-based superconductors $A$Fe$_2$As$_2$ ($A=$K, Cs, and Rb), which are characterized by the V-shaped dependence of the critical temperature ($T_{rm c}$) on pressure ($P$) were studied by means of the muon spin rotation/relaxation technique. In all three systems studied the magnetism was found to appear for pressures slightly below the critical one ($P_{rm c}$), i.e. at pressure where $T_{rm c}(P)$ changes the slope. Rather than competing, magnetism and superconductivity in $A$Fe$_2$As$_2$ are coexisting at $Pgtrsim P_{rm c}$ pressure region. Our results support the scenario of a transition from one pairing state to another, with different symmetries on either side of $P_{rm c}$.
Pairing symmetry which characterizes the superconducting pairing mechanism is normally determined by measuring the superconducting gap structure ($|Delta_k|$). Here, we report the measurement of a strain-induced gap modulation ($partial|Delta_k|$) in uniaxially strained Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ utilizing angle-resolved photoemission spectroscopy and $in$-$situ$ strain-tuning. We found that the uniaxial strain drives Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ into a nematic superconducting state which breaks the four-fold rotational symmetry of the superconducting pairing. The superconducting gap increases on the $d_{yz}$ electron and hole pockets while it decreases on the $d_{xz}$ counterparts. Such orbital selectivity indicates that orbital-selective pairing exists intrinsically in non-nematic iron-based superconductors. The $d_{xz}$ and $d_{yz}$ pairing channels are balanced originally in the pristine superconducting state, but become imbalanced under uniaxial strain. Our results highlight the important role of intra-orbital scattering in mediating the superconducting pairing in iron-based superconductors. It also highlights the measurement of $partial|Delta_k|$ as an effective way to characterize the superconducting pairing from a perturbation perspective.
We report the observation by angle-resolved photoemission spectroscopy of an impurity state located inside the superconducting gap of Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ and vanishing above the superconducting critical temperature, for which the spectral weight is confined in momentum space near the Fermi wave vector positions. We demonstrate, supported by theoretical simulations, that this in-gap state originates from weak non-magnetic scattering between bands with opposite sign of the superconducting gap phase. This weak scattering, likely due to off-plane Ba/K disorders, occurs mostly among neighboring Fermi surfaces, suggesting that the superconducting gap phase changes sign within holelike (and electronlike) bands. Our results impose severe restrictions on the models promoted to explain high-temperature superconductivity in these materials.
In unconventional superconductors, it is generally believed that understanding the physical properties of the normal state is a pre-requisite for understanding the superconductivity mechanism. In conventional superconductors like niobium or lead, the normal state is a Fermi liquid with a well-defined Fermi surface and well-defined quasipartcles along the Fermi surface. Superconductivity is realized in this case by the Fermi surface instability in the superconducting state and the formation and condensation of the electron pairs (Cooper pairing). The high temperature cuprate superconductors, on the other hand, represent another extreme case that superconductivity can be realized in the underdoped region where there is neither well-defined Fermi surface due to the pseudogap formation nor quasiparticles near the antinodal regions in the normal state. Here we report a novel scenario that superconductivity is realized in a system with well-defined Fermi surface but without quasiparticles along the Fermi surface in the normal state. High resolution laser-based angle-resolved photoemission measurements have been performed on an optimally-doped iron-based superconductor (Ba$_{0.6}$K$_{0.4}$)Fe$_2$As$_2$. We find that, while sharp superconducting coherence peaks emerge in the superconducting state on the hole-like Fermi surface sheets, no quasiparticle peak is present in the normal state. Its electronic behaviours deviate strongly from a Fermi liquid system. The superconducting gap of such a system exhibits an unusual temperature dependence that it is nearly a constant in the superconducting state and abruptly closes at T$_c$. These observations have provided a new platform to study unconventional superconductivity in a non-Fermi liquid system.
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