No Arabic abstract
We analyze the transformation from insulator to metal induced by thermal fluctuations within the Falicov-Kimball model. Using the Dynamic Mean Field Theory (DMFT) formalism on the Bethe lattice we find rigorously the temperature dependent Density of States ($DOS$) at half filling in the limit of high dimensions. At zero temperature (T=0) the system is ordered to form the checkerboard pattern and the $DOS$ has the gap $Delta$ at the Fermi level $varepsilon_F=0$, which is proportional to the interaction constant $U$. With an increase of $T$ the $DOS$ evolves in various ways that depend on $U$. For $U>U_{cr}$ the gap persists for any $T$ (then $Delta >0$), so the system is always an insulator. However, if $U < U_{cr}$, two additional subbands develop inside the gap. They become wider with increasing $T$ and at a certain $U$-dependent temperature $T_{MI}$ they join with each other at $varepsilon_F$. Since above $T_{MI}$ the $DOS$ is positive at $varepsilon_F$, we interpret $T_{MI}$ as the transformation temperature from insulator to metal. It appears, that $T_{MI}$ approaches the order-disorder phase transition temperature $T_{O-DO}$ when $U$ is close to 0 or $ U_{cr}$, but $T_{MI}$ is substantially lower than $T_{O-DO}$ for intermediate values of $U$. Having calculated the temperature dependent $DOS$ we study thermodynamic properties of the system starting from its free energy $F$. Then we find how the order parameter $d$ and the gap $Delta $ change with $T$ and we construct the phase diagram in the variables $T$ and $U$, where we display regions of stability of four different phases: ordered insulator, ordered metal, disordered insulator and disordered metal. Finally, we use a low temperature expansion to demonstrate the existence of a nonzero DOS at a characteristic value of U on a general bipartite lattice.
It has long been thought that strongly correlated systems are adiabatically connected to their noninteracting counterpart. Recent developments have highlighted the fallacy of this traditional notion in a variety of settings. Here we use a class of strongly correlated electron systems as a platform to illustrate the kind of quantum phases and fluctuations that are created by strong correlations. Examples are quantum critical states that violate the Fermi liquid paradigm, unconventional superconductivity that goes beyond the BCS framework, and topological semimetals induced by the Kondo interaction. We assess the prospect of designing other exotic phases of matter, by utilizing alternative degrees of freedom or alternative interactions, and point to the potential of these correlated states for quantum technology.
We investigate the thermal-driven charge density wave (CDW) transition of two cubic superconducting intermetallic systems Lu(Pt1-xPdx)2In and (Sr1-xCax)3Ir4Sn13 by means of x-ray diffraction technique. A detailed analysis of the CDW modulation superlattice peaks as function of temperature is performed for both systems as the CDW transition temperature T_CDW is suppressed to zero by an non-thermal control parameter. Our results indicate an interesting crossover of the classical thermal-driven CDW order parameter critical exponent from a three-dimensional universality class to a mean-field tendency, as T_CDW vanishes. Such behavior might be associated with presence of quantum fluctuations which influences the classical second-order phase transition, strongly suggesting the presence of a quantum critical point (QCP) at T_CDW = 0. This also provides experimental evidence that the effective dimensionality exceeds its upper critical dimension due to a quantum phase transition.
We present angle-resolved photoemission experiments on 1T-TiSe2 at temperatures ranging from 13K to 288K. The data evidence a dramatic renormalization of the conduction band below 100K, whose origin can be explained with the exciton condensate phase model. The renormalization translates into a substantial effective mass reduction of the dominant charge carriers and can be directly related to the low temperature downturn of the resistivity of 1T-TiSe2. This observation is in opposition to the common belief that strong interactions produce heavier quasiparticles through an increased effective mass.
Electron correlations amplify quantum fluctuations and, as such, they have been recognized as the origin of a rich landscape of quantum phases. Whether and how they lead to gapless topological states is an outstanding question, and a framework that allows for determining novel phases and identifying new materials is in pressing need. Here we advance a general approach, in which strong correlations cooperate with crystalline symmetry to drive gapless topological states. We test this design principle by exploring Kondo lattice models and materials whose space group symmetries may promote different kinds of electronic degeneracies, with a particular focus on square-net systems. Weyl-Kondo nodal-line semimetals -- with nodes pinned to the Fermi energy -- are identified in both two and three dimensions. We apply the approach to identify materials for the realization of these correlation-driven topological semimetal phases. Our findings illustrate the potential of the proposed design principle to guide the search for new topological phases and materials in a broad range of strongly correlated systems.
We investigate the 1/3 monolayer $alpha$-Pb/Si(111) surface by scanning tunneling spectroscopy (STS) and fully relativistic first-principles calculations. We study both the high-temperature $sqrt{3}timessqrt{3}$ and low-temperature $3times 3$ reconstructions and show that, in both phases, the spin-orbit interaction leads to an energy splitting as large as $25%$ of the valence-band bandwidth. Relativistic effects, electronic correlations and Pb-substrate interaction cooperate to stabilize a correlated low-temperature paramagnetic phase with well-developed lower and upper Hubbard bands coexisting with $3times3$ periodicity. By comparing the Fourier transform of STS conductance maps at the Fermi level with calculated quasiparticle interference from non-magnetic impurities, we demonstrate the occurrence of two large hexagonal Fermi sheets with in-plane spin polarizations and opposite helicities.