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Register a new userSpatially resolved quantum nano-optics of single photons using an electron microscope
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We report on the experimental demonstration of single photon state generation and characterization in an electron microscope. In this aim we have used low intensity relativistic (energy between 60kV and 100 keV) electrons beams focused in a ca 1 nm probe to excite diamond nanoparticles. This triggered individual neutral Nitrogen-vacancies (NV0) centers to emit photon which could be gathered and sent to a Hanbury Brown Twiss intensity interferometer. The detection of a dip in the correlation function at small time delays clearly demonstrates antibunching and thus the creation of non-classical light states. Specifically, we have also demonstrated single photon state detection. We unveil the mechanism behind quantum states generation in an electron microscope, and show that it clearly makes cathodoluminescence the nanometer scale analog of photoluminescence rather than electroluminescence. By using an extremely small electron probe size and the ability to monitor its position with sub nanometer resolution, we also show the possibility of measuring the quantum character of the emitted beam with deep sub wavelength resolution.
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Single photons carrying spin angular momentum (SAM), i.e., circularly polarized single photons generated typically by subjecting a quantum emitter (QE) to a strong magnetic field at low temperatures are at the core of chiral quantum optics enabling non-reciprocal single-photon configurations and deterministic spin-photon interfaces. Here we propose a conceptually new approach to the room-temperature generation of SAM-coded single photons (SSPs) entailing QE non-radiative coupling to surface plasmons that are transformed, by interacting with an optical metasurface, into a collimated stream of SSPs with the designed handedness. We report on the design, fabrication and characterization of SSP sources consisting of dielectric circular nanoridges with azimuthally varying widths deterministically fabricated on a dielectric-protected silver film around a nanodiamond containing a nitrogen-vacancy centre. With properly engineered phases of QE-originated fields scattered by nanoridges, the out-coupled photons feature a well-defined SAM (with the chirality > 0.8) and high directionality (collection efficiency up to 92%).
We report on the structural and optical properties of individual bowtie nanoantennas both on glass and semiconducting GaAs substrates. The antennas on glass (GaAs) are shown to be of excellent quality and high uniformity reflected by narrow size distributions with standard deviations for the triangle and gap size of $sigma_s^{glass}=4.5nm$ ($sigma_s^{GaAs}=2.6nm$) and $sigma_g^{glass}=5.4nm$ ($sigma_g^{GaAs}=3.8nm$), respectively. The corresponding optical properties of individual nanoantennas studied by differential reflection spectroscopy show a strong reduction of the localised surface plasmon polariton resonance linewidth from $0.21eV$ to $0.07eV$ upon reducing the antenna size from $150nm$ to $100nm$. This is attributed to the absence of inhomogeneous broadening as compared to optical measurements on nanoantenna ensembles. The inter-particle coupling of an individual bowtie nanoantenna, which gives rise to strongly localised and enhanced electromagnetic hotspots, is demonstrated using polarization-resolved spectroscopy, yielding a large degree of linear polarization of $rho_{max}sim80%$. The combination of highly reproducible nanofabrication and fast, non-destructive and non-contaminating optical spectroscopy paves the route towards future semiconductor-based nano-plasmonic circuits, consisting of multiple photonic and plasmonic entities.
Ultra-fast transmission electron microscopy (UTEM) combines sub-picosecond time-resolution with the versatility of TEM spectroscopies. It allows one to study the dynamics of materials properties combining complementary techniques. However, until now, time-resolved cathodoluminescence, which is expected to give access to the optical properties dynamics, was still unavailable in a UTEM. In this paper, we report time-resolved cathodoluminescence measurements in an ultrafast transmission electron microscope. We measured lifetime maps, with a 12 nm spatial resolution and sub-nanoseconds resolution, of nano-diamonds with a high density of NV center. This study paves the way to new applications of UTEM and to correlative studies of optically active nanostructures.
We propose a device consisting in an antidot periodically driven in time by a magnetic field as a fractional quantum Hall counterpart of the celebrated mesoscopic capacitor-based single electron source. We fully characterize the setup as an ideal emitter of individual quasiparticles and electrons into fractional quantum Hall edge channels of the Laughlin sequence. Our treatment relies on a master equation approach and identifies the optimal regime of operation for both types of sources. The quasiparticle/quasihole emission regime involves in practice only two charge states of the antidot, allowing for an analytic treatment. We show the precise quantization of the emitted charge, we determine its optimal working regime, and we compute the phase noise/shot noise crossover as a function of the escape time from the emitter. The emission of electrons, which calls for a larger amplitude of the drive, requires a full numerical treatment of the master equations as more quasiparticle charge states are involved. Nevertheless, in this case the emission of one electron charge followed by one hole per period can also be achieved, and the overall shape of the noise spectrum is similar to that of the quasiparticle source, but the presence of additional quasiparticle processes enhances the noise amplitude.
We demonstrate real-time detection of self-interfering electrons in a double quantum dot embedded in an Aharonov-Bohm interferometer, with visibility approaching unity. We use a quantum point contact as a charge detector to perform time-resolved measurements of single-electron tunneling. With increased bias voltage, the quantum point contact exerts a back-action on the interferometer leading to decoherence. We attribute this to emission of radiation from the quantum point contact, which drives non-coherent electronic transitions in the quantum dots.
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