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Register a new userExcitation-Transfer Plasmonic Nanosensors based on Dynamical Phase Transitions
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Raul Bustos-Marun A
Publication date
2012
fields
Physics
and research's language is
English
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Dynamical Phase transitions (DPTs) describe the abrupt change in the dynamical properties of open systems when a single control parameter is slightly modified. Recently we found that this phenomenon is also present in a simple model of a linear array of metallic nanoparticles (NPs) in the form of a localized-delocalized DPT. In this work we show how to take advantage of DPTs in order to design a new kind of plasmonic sensor which should own some unique characteristics. For example, if it were used as plasmon ruler it would not follow the so called universal plasmon ruler equation [Nano Letters 2007, 7, 2080-2088], exhibiting instead an on-off switching feature. This basically means that a signal should only be observed when the control/measured parameter, i.e. a distance in the case of plasmon rulers, has a very precise and pre-determined value. Here, we demonstrate their feasibility and unique characteristics, showing that they combine high sensitivity with this on-off switching feature in terms of different distances and local dielectric constants. This property has the potentiality to be used in the design of new plasmonic devices such as plasmonic circuits activated only under certain environmental conditions.
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The traditional concept of phase transitions has, in recent years, been widened in a number of interesting ways. The concept of a topological phase transition separating phases with a different ground state topology, rather than phases of different symmetries, has become a large widely studied field in its own right. Additionally an analogy between phase transitions, described by non-analyticities in the derivatives of the free energy, and non-analyticities which occur in dynamically evolving correlation functions has been drawn. These are called dynamical phase transitions and one is often now far from the equilibrium situation. In these short lecture notes we will give a brief overview of the history of these concepts, focusing in particular on the way in which dynamical phase transitions themselves can be used to shed light on topological phase transitions and topological phases. We will go on to focus, first, on the effect which the topologically protected edge states, which are one of the interesting consequences of topological phases, have on dynamical phase transitions. Second we will consider what happens in the experimentally relevant situations where the system begins either in a thermal state rather than the ground state, or exchanges particles with an external environment.
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