No Arabic abstract
We introduce a non-Hermitian approximation of Bloch optical equations. This approximation provides a complete description of the excitation, relaxation and decoherence dynamics of ensembles of coupled quantum systems in weak laser fields, taking into account collective effects and dephasing. In the proposed method one propagates the wave function of the system instead of a complete density matrix. Relaxation and dephasing are taken into account via automatically-adjusted time-dependent gain and decay rates. As an application, we compute the numerical wave packet solution of a time-dependent non-Hermitian Schrodinger equation describing the interaction of electromagnetic radiation with a quantum nano-structure and compare the calculated transmission, reflection, and absorption spectra with those obtained from the numerical solution of the Liouville- von-Neumann equation. It is shown that the proposed wave packet scheme is significantly faster than the propagation of the full density matrix while maintaining small error. We provide the key ingredients for easy-to-use implementation of the proposed scheme and identify the limits and error scaling of this approximation.
We introduce an accurate non-Hermitian Schrodinger-type approximation of Bloch optical equations for two-level systems. This approximation provides a complete description of the excitation, relaxation and decoherence dynamics in both weak and strong laser fields. In this approach, it is sufficient to propagate the wave function of the quantum system instead of the density matrix, providing that relaxation and dephasing are taken into account via automatically-adjusted time-dependent gain and decay rates. The developed formalism is applied to the problem of scattering and absorption of electromagnetic radiation by a thin layer comprised of interacting two-level emitters.
Berry phases strongly affect the properties of crystalline materials, giving rise to modifications of the semiclassical equations of motion that govern wave-packet dynamics. In non-Hermitian systems, generalizations of the Berry connection have been analyzed to characterize the topology of these systems. While the topological classification of non-Hermitian systems is being developed, little attention has been paid to the impact of the new geometric phases on dynamics and transport. In this work, we derive the full set of semiclassical equations of motion for wave-packet dynamics in a system governed by a non-Hermitian Hamiltonian, including corrections induced by the Berry connection. We show that non-Hermiticity is manifested in anomalous weight rate and velocity terms that are present already in one-dimensional systems, in marked distinction from the Hermitian case. We express the anomalous weight and velocity in terms of the Berry connections defined in the space of left and right eigenstates and compare the analytical results with numerical lattice simulations. Our work specifies the conditions for observing the anomalous contributions to the semiclassical dynamics and thereby paves the way to their experimental detection, which should be within immediate reach in currently available metamaterials.
Knots have a twisted history in quantum physics. They were abandoned as failed models of atoms. Only much later was the connection between knot invariants and Wilson loops in topological quantum field theory discovered. Here we show that knots tied by the eigenenergy strings provide a complete topological classification of one-dimensional non-Hermitian (NH) Hamiltonians with separable bands. A $mathbb{Z}_2$ knot invariant, the global biorthogonal Berry phase $Q$ as the sum of the Wilson loop eigenphases, is proved to be equal to the permutation parity of the NH bands. We show the transition between two phases characterized by distinct knots occur through exceptional points and come in two types. We further develop an algorithm to construct the corresponding tight-binding NH Hamiltonian for any desired knot, and propose a scheme to probe the knot structure via quantum quench. The theory and algorithm are demonstrated by model Hamiltonians that feature for example the Hopf link, the trefoil knot, the figure-8 knot and the Whitehead link.
Bulk-boundary correspondence is the cornerstone of topological physics. In some non-Hermitian topological system this fundamental relation is broken in the sense that the topological number calculated for the Bloch energy band under the periodic boundary condition fails to reproduce the boundary properties under the open boundary. To restore the bulk-boundary correspondence in such non-Hermitian systems a framework beyond the Bloch band theory is needed. We develop a non-Hermitian Bloch band theory based on a modified periodic boundary condition that allows a proper description of the bulk of a non-Hermitian topological insulator in a manner consistent with its boundary properties. Taking a non-Hermitian version of the Su-Schrieffer-Heeger model as an example, we demonstrate our scenario, in which the concept of bulk-boundary correspondence is naturally generalized to non-Hermitian topological systems.
Emission of high-order harmonics from solids provides a new avenue in attosecond science. On one hand, it allows to investigate fundamental processes of the non-linear response of electrons driven by a strong laser pulse in a periodic crystal lattice. On the other hand, it opens new paths toward efficient attosecond pulse generation, novel imaging of electronic wave functions, and enhancement of high-order harmonic generation (HHG) intensity. A key feature of HHG in a solid (as compared to the well-understood phenomena of HHG in an atomic gas) is the delocalization of the process, whereby an electron ionized from one site in the periodic lattice may recombine with any other. Here, we develop an analytic model, based on the localized Wannier wave functions in the valence band and delocalized Bloch functions in the conduction band. This Wannier-Bloch approach assesses the contributions of individual lattice sites to the HHG process, and hence addresses precisely the question of localization of harmonic emission in solids. We apply this model to investigate HHG in a ZnO crystal for two different orientations, corresponding to wider and narrower valence and conduction bands, respectively. Interestingly, for narrower bands, the HHG process shows significant localization, similar to harmonic generation in atoms. For all cases, the delocalized contributions to HHG emission are highest near the band-gap energy. Our results pave the way to controlling localized contributions to HHG in a solid crystal, with hard to overestimate implications for the emerging area of atto-nanoscience.