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Register a new userLinear response theory for arbitrary periodic signals
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We extend Kubos Linear Response Theory (LRT) to periodic input signals with arbitrary shapes and obtain exact analytical formulas for the energy dissipated by the system for a variety of signals. These include the square and sawtooth waves, or pulsed signals such as the rectangular, sine and $delta$-pulses. It is shown that for a given input energy, the dissipation may be substantially augmented by exploiting different signal shapes. We also apply our results in the context of magnetic hyperthermia, where small magnetic particles are used as local heating centers in oncological treatments.
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Fluctuation dissipation theorems connect the linear response of a physical system to a perturbation to the steady-state correlation functions. Until now, most of these theorems have been derived for finite-dimensional systems. However, many relevant physical processes are described by systems of infinite dimension in the Gaussian regime. In this work, we find a linear response theory for quantum Gaussian systems subject to time dependent Gaussian channels. In particular, we establish a fluctuation dissipation theorem for the covariance matrix that connects its linear response at any time to the steady state two-time correlations. The theorem covers non-equilibrium scenarios as it does not require the steady state to be at thermal equilibrium. We further show how our results simplify the study of Gaussian systems subject to a time dependent Lindbladian master equation. Finally, we illustrate the usage of our new scheme through some examples. Due to broad generality of the Gaussian formalism, we expect our results to find an application in many physical platforms, such as opto-mechanical systems in the presence of external noise or driven quantum heat devices.
Activated surface diffusion with interacting adsorbates is analyzed within the Linear Response Theory framework. The so-called interacting single adsorbate model is justified by means of a two-bath model, where one harmonic bath takes into account the interaction with the surface phonons, while the other one describes the surface coverage, this leading to defining a collisional friction. Here, the corresponding theory is applied to simple systems, such as diffusion on flat surfaces and the frustrated translational motion in a harmonic potential. Classical and quantum closed formulas are obtained. Furthermore, a more realistic problem, such as atomic Na diffusion on the corrugated Cu(001) surface, is presented and discussed within the classical context as well as within the framework of Kramers theory. Quantum corrections to the classical results are also analyzed and discussed.
We consider thermodynamically consistent autonomous Markov jump processes displaying a macroscopic limit in which the logarithm of the probability distribution is proportional to a scale-independent rate function (i.e., a large deviations principle is satisfied). In order to provide an explicit expression for the probability distribution valid away from equilibrium, we propose a linear response theory performed at the level of the rate function. We show that the first order non-equilibrium contribution to the steady state rate function, $g(x)$, satisfies $u(x)cdot abla g(x) = -beta dot W(x)$ where the vector field $u(x)$ defines the macroscopic deterministic dynamics, and the scalar field $dot W(x)$ equals the rate at which work is performed on the system in a given state $x$. This equation provides a practical way to determine $g(x)$, significantly outperforms standard linear response theory applied at the level of the probability distribution, and approximates the rate function surprisingly well in some far-from-equilibrium conditions. The method applies to a wealth of physical and chemical systems, that we exemplify by two analytically tractable models - an electrical circuit and an autocatalytic chemical reaction network - both undergoing a non-equilibrium transition from a monostable phase to a bistable phase. Our approach can be easily generalized to transient probabilities and non-autonomous dynamics. Moreover, its recursive application generates a virtual flow in the probability space which allows to determine the steady state rate function arbitrarily far from equilibrium.
We analyse the linear response properties of the uniformly heated granular gas. The intensity of the stochastic driving fixes the value of the granular temperature in the non-equilibrium steady state reached by the system. Here, we investigate two specific situations. First, we look into the ``direct relaxation of the system after a single (small) jump of the driving intensity. This study is carried out by two different methods. Not only do we linearise the evolution equations around the steady state, but also derive generalised out-of-equilibrium fluctuation-dissipation relations for the relevant response functions. Second, we investigate the behaviour of the system in a more complex experiment, specifically a Kovacs-like protocol with two jumps in the driving. The emergence of anomalous Kovacs response is explained in terms of the properties of the direct relaxation function: it is the second mode changing sign at the critical value of the inelasticity that demarcates anomalous from normal behaviour. The analytical results are compared with numerical simulations of the kinetic equation, and a good agreement is found.
Basing on the theory of Feynmans influence functional and its hierarchical equations of motion, we develop a linear response theory for quantum open systems. Our theory provides an effective way to calculate dynamical observables of a quantum open system at its steady-state, which can be applied to various fields of non-equilibrium condensed matter physics.
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