We study terahertz transmission through nano-patterned vanadium dioxide thin film. It is found that the patterning allows the lowering of the apparent transition temperature. For the case of the smallest width nano antennas, the transition temperature is lower by as many as ten degrees relative to the bare film, so that the nano patterned hysteresis curves completely separate themselves from their bare film counterparts. This early transition comes from the one order of magnitude enhanced effective dielectric constants by nano antennas. This phenomenon opens up the possibility of transition temperature engineering.
Electrons in correlated insulators are prevented from conducting by Coulomb repulsion between them. When an insulator-to-metal transition is induced in a correlated insulator by doping or heating, the resulting conducting state can be radically different from that characterized by free electrons in conventional metals. We report on the electronic properties of a prototypical correlated insulator vanadium dioxide (VO2) in which the metallic state can be induced by increasing temperature. Scanning near-field infrared microscopy allows us to directly image nano-scale metallic puddles that appear at the onset of the insulator-to-metal transition. In combination with far-field infrared spectroscopy, the data reveal the Mott transition with divergent quasiparticle mass in the metallic puddles. The experimental approach employed here sets the stage for investigations of charge dynamics on the nanoscale in other inhomogeneous correlated electron systems.
Plasmonic photoconductive antennas have great promise for increasing responsivity and detection sensitivity of conventional photoconductive detectors in time-domain terahertz imaging and spectroscopy systems. However, operation bandwidth of previously demonstrated plasmonic photoconductive antennas has been limited by bandwidth constraints of their antennas and photoconductor parasitics. Here, we present a powerful technique for realizing broadband terahertz detectors through large-area plasmonic photoconductive nano-antenna arrays. A key novelty that makes the presented terahertz detector superior to the state-of-the art is a specific large-area device geometry that offers a strong interaction between the incident terahertz beam and optical pump at the nanoscale, while maintaining a broad operation bandwidth. The large device active area allows robust operation against optical and terahertz beam misalignments. We demonstrate broadband terahertz detection with signal-to-noise ratio levels as high as 107 dB.
Dynamically switchable half-/quarter-wave plates have recently been the focus in the terahertz regime. Conventional design philosophy leads to multilayer metamaterials or narrowband metasurfaces. Here we propose a novel design philosophy and a VO2-metal hybrid metasurface for achieving broadband dynamically switchable half-/quarter-wave plate (HWP/QWP) based on the transition from the overdamped to the underdamped resonance. Results show that, by varying the VO2 conductivity by three orders of magnitude, the proposed metasurfaces function can be switched between an HWP with polarization conversion ratio larger than 96% and a QWP with ellipticity close to -1 over the broad working band of 0.8-1.2 THz. We expect that the proposed design philosophy will advance the engineering of metasurfaces for dynamically switchable functionalities beyond the terahertz regime.
Detection of local strain at the nanometer scale with high sensitivity remains challenging. Here we report near-field infrared nano-imaging of local strains in bilayer graphene through probing strain-induced shifts of phonon frequency. As a non-polar crystal, intrinsic bilayer graphene possesses little infrared response at its transverse optical (TO) phonon frequency. The reported optical detection of local strain is enabled by applying a vertical electrical field that breaks the symmetry of the two graphene layers and introduces finite electrical dipole moment to graphene phonon. The activated phonon further interacts with continuum electronic transitions, and generates a strong Fano resonance. The resulted Fano resonance features a very sharp near-field infrared scattering peak, which leads to an extraordinary sensitivity of ~0.002% for the strain detection. Our studies demonstrate the first nano-scale near-field Fano resonance, provide a new way to probe local strains with high sensitivity in non-polar crystals, and open exciting possibilities for studying strain-induced rich phenomena.
Spintronic terahertz (THz) emitter provides the advantages such as apparently broader spectrum, significantly lower cost, and more flexibility in compared with the commercial THz emitters, and thus attracts great interests recently. In past few years, efforts have been made in optimizing the material composition and structure geometry, and the conversion efficiency has been improved close to that of ZnTe crystal. One of the drawbacks of the current designs is the rather limited laser absorption - more than 50% energy is wasted and the conversion efficiency is thus limited. Here, we theoretically propose and experimentally demonstrate a novel device that fully utilizes the laser intensity and significantly improves the conversion efficiency. The device, which consists of a metal-dielectric photonic crystal structure, utilizes the interference between the multiple scattering waves to simultaneously suppress the reflection and transmission of the laser, and to reshape the laser field distributions. The experimentally detected laser absorption and THz generations show one-to-one correspondence with the theoretical calculations. We achieve the strongest THz pulse emission that presents a 1.7 times improvement compared to the currently designed spintronic emitter. This work opens a new pathway to improve the performance of spintronic THz emitter from the perspective of optics.