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High-spin structures of five N=82 isotones: 136Xe, 137Cs, 138Ba, 139La, and 140Ce

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 Publication date 2012
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Five N=82 isotones have been produced in two fusion-fission reactions and their gamma-rays studied with the Euroball array. The high-spin states of 139La have been identified for the first time, while the high-spin yrast and near-to-yrast structures of the four others have been greatly extended. From angular correlation analysis,spin values have been assigned to some states of 136Xe and 137Cs. Several cascades involving gamma-rays of 139La have been found to be delayed, they deexcite an isomeric state with T1/2= 315(35) ns located at 1800-keV excitation energy. The excited states of these five N=82 isotones are expected to be due to various proton excitations involving the three high-j subshells located above the Z=50 shell closure. This is confirmed by the results of shell-model calculations performed in this work. In addition, high-spin states corresponding to the excitation of the neutron core have been unambiguously identified in 136Xe, 137Cs, and 138Ba.



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Odd-odd 136Cs nuclei have been produced in the 18O + 208Pb and 12C + 238U fusion-fission reactions and their gamma rays studied with the Euroball array. The high-spin level scheme has been built up to ~ 4.7 MeV excitation energy and spin I ~ 16 hbar from the triple gamma-ray coincidence data. The configurations of the three structures observed above ~ 2 MeV excitation energy are first discussed by analogy with the proton excitations identified in the semi-magic 137Cs nucleus, which involve the three high-j orbits lying above the Z=50 gap, pi g_{7/2}, pi d_{5/2} and pi h_{11/2}. This is confirmed by the results of shell-model calculations performed in this work.
291 - A. Hennig , M. Spieker , V. Werner 2015
Background: Excitations with mixed proton-neutron symmetry have been previously observed in the $N=52$ isotones. Besides the well established quadrupole mixed-symmetry states (MSS), octupole and hexadecapole MSS have been recently proposed for the nuclei $^{92}$Zr and $^{94}$Mo. Purpose: The heaviest stable $N=52$ isotone $^{96}$Ru was investigated to study the evolution of octupole and hexadecapole MSS with increasing proton number. Methods: Two inelastic proton-scattering experiments on $^{96}$Ru were performed to extract branching ratios, multipole mixing ratios, and level lifetimes. From the combined data, absolute transition strengths were calculated. Results: Strong $M1$ transitions between the lowest-lying $3^-$ and $4^+$ states were observed, providing evidence for a one-phonon mixed-symmetry character of the $3^{(-)}_2$ and $4^+_2$ states. Conclusions: $sdg$-IBM-2 calculations were performed for $^{96}$Ru. The results are in excellent agreement with the experimental data, pointing out a one-phonon hexadecapole mixed-symmetry character of the $4^+_2$ state. The $big< 3^-_1||M1||3^{(-)}_2big>$ matrix element is found to scale with the $<2^+_{mathrm{s}}||M1||2^+_{mathrm{ms}}>$ matrix element.
Excited states in the $N=40$ isotone $^{62}$Ti were populated via the $^{63}$V$(p,2p)$$^{62}$Ti reaction at $sim$200~MeV/u at the Radioactive Isotope Beam Factory and studied using $gamma$-ray spectroscopy. The energies of the $2^+_1 rightarrow 0^{+}_{mathrm{gs}}$ and $4^+_1 rightarrow 2^+_1$ transitions, observed here for the first time, indicate a deformed $^{62}$Ti ground state. These energies are increased compared to the neighboring $^{64}$Cr and $^{66}$Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings. The shell-model calculations for $^{62}$Ti show a dominant configuration with four neutrons excited across the $N=40$ gap. Likewise, they indicate that the $N=40$ island of inversion extends down to $Z=20$, disfavoring a possible doubly magic character of the elusive $^{60}$Ca.
A measurement of the $^{50}$Ti($d$,$p$)$^{51}$Ti reaction at 16 MeV was performed using a Super Enge Split Pole Spectrograph to measure the magnitude of the $N=32$ subshell gap in Ti. Seven states were observed that had not been observed in previous ($d$,$p$) measurements, and the textit{L} transfer values for six previously measured states were either changed or measured for the first time. The results were used to determine single neutron energies for the $p_{3/2}$, $p_{1/2}$ and $f_{5/2}$ orbitals. The resulting single neutron energies in $^{51}$Ti confirm the existence of the $N=32$ gap in Ti. These single neutron energies and those from previous measurements in $^{49}$Ca, $^{53}$Cr and $^{55}$Fe are compared to values from a covariant density functional theory calculation.
The 124-131Te nuclei have been produced as fission fragments in two fusion reactions induced by heavy-ions (12C + 238U at 90 MeV bombarding energy and 18O + 208Pb at 85 MeV) and studied with the Euroball array. Their high-spin level schemes have been extended to higher excitation energy from the triple gamma-ray coincidence data. The gamma-gamma angular correlations have been analyzed in order to assign spin and parity values to many observed states. Moreover the half-lives of isomeric states have been measured from the delayed coincidences between the fission-fragment detector SAPhIR and Euroball, as well as from the timing information of the Ge detectors. The behaviors of the yrast structures identified in the present work are first discussed in comparison with the general features known in the mass region, particularly the breakings of neutron pairs occupying the nuh11/2 orbit identified in the neighboring Sn nuclei. The experimental level schemes are then compared to shell-model calculations performed in this work. The analysis of the wave functions shows the effects of the proton-pair breaking along the yrast lines of the heavy Te isotopes.
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