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High-spin structures of 124-131Te: Competition of proton and neutron pair breakings

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 Publication date 2013
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The 124-131Te nuclei have been produced as fission fragments in two fusion reactions induced by heavy-ions (12C + 238U at 90 MeV bombarding energy and 18O + 208Pb at 85 MeV) and studied with the Euroball array. Their high-spin level schemes have been extended to higher excitation energy from the triple gamma-ray coincidence data. The gamma-gamma angular correlations have been analyzed in order to assign spin and parity values to many observed states. Moreover the half-lives of isomeric states have been measured from the delayed coincidences between the fission-fragment detector SAPhIR and Euroball, as well as from the timing information of the Ge detectors. The behaviors of the yrast structures identified in the present work are first discussed in comparison with the general features known in the mass region, particularly the breakings of neutron pairs occupying the nuh11/2 orbit identified in the neighboring Sn nuclei. The experimental level schemes are then compared to shell-model calculations performed in this work. The analysis of the wave functions shows the effects of the proton-pair breaking along the yrast lines of the heavy Te isotopes.



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In the present work recently available experimental data for high-spin states of four nuclei, $^{124}_{ 52}$Te, $^{125}_{ 52}$Te, $^{126}_{ 52}$Te, and $^{127}_{ 52}$Te have been interpreted using state-of-the-art shell model calculations. The calculations have been performed in the $50-82$ valence shell composed of $1g_{7/2}$, $2d_{5/2}$, $1h_{11/2}$, $3s_{1/2}$, and $2d_{3/2}$ orbitals. We have compared our results with the available experimental data for excitation energies and transition probabilities, including high-spin states. The results are in reasonable agreement with the available experimental data. The wave functions, particularly, the specific proton and neutron configurations which are involved to generate the angular momentum along the yrast lines are discussed. We have also estimated overall contribution of three-body forces in the energy level shifting. Finally, results with modified effective interaction are also reported.
Odd-odd 136Cs nuclei have been produced in the 18O + 208Pb and 12C + 238U fusion-fission reactions and their gamma rays studied with the Euroball array. The high-spin level scheme has been built up to ~ 4.7 MeV excitation energy and spin I ~ 16 hbar from the triple gamma-ray coincidence data. The configurations of the three structures observed above ~ 2 MeV excitation energy are first discussed by analogy with the proton excitations identified in the semi-magic 137Cs nucleus, which involve the three high-j orbits lying above the Z=50 gap, pi g_{7/2}, pi d_{5/2} and pi h_{11/2}. This is confirmed by the results of shell-model calculations performed in this work.
Five N=82 isotones have been produced in two fusion-fission reactions and their gamma-rays studied with the Euroball array. The high-spin states of 139La have been identified for the first time, while the high-spin yrast and near-to-yrast structures of the four others have been greatly extended. From angular correlation analysis,spin values have been assigned to some states of 136Xe and 137Cs. Several cascades involving gamma-rays of 139La have been found to be delayed, they deexcite an isomeric state with T1/2= 315(35) ns located at 1800-keV excitation energy. The excited states of these five N=82 isotones are expected to be due to various proton excitations involving the three high-j subshells located above the Z=50 shell closure. This is confirmed by the results of shell-model calculations performed in this work. In addition, high-spin states corresponding to the excitation of the neutron core have been unambiguously identified in 136Xe, 137Cs, and 138Ba.
The high-spin states of the two neutron-rich nuclei, 88Kr and 89R have been studied from the 18O + 208Pb fusion-fission reaction. Their level schemes were built from triple gamma-ray coincidence data and gamma-gamma angular correlations were analyzed in order to assign spin and parity values to most of the observed states. The two levels schemes evolve from collective structures to single-particle excitations as a function of the excitation energy. Comparison with results of shell-model calculations gives the specific proton and neutron configurations which are involved to generate the angular momentum along the yrast lines.
The general phenomenon of shell structure in atomic nuclei has been understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and Suess.They realized that the experimental evidence for nuclear magic numbers could be explained by introducing a strong spin-orbit interaction in the nuclear shell model potential. However, our detailed knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers ($N = Z$), the unique nature of the atomic nucleus as an object composed of two distinct types of fermions can be expressed as enhanced correlations arising between neutrons and protons occupying orbitals with the same quantum numbers. Such correlations have been predicted to favor a new type of nuclear superfluidity; isoscalar neutron-proton pairing, in addition to normal isovector pairing (see Fig. 1). Despite many experimental efforts these predictions have not been confirmed. Here, we report on the first observation of excited states in $N = Z = 46$ nucleus $^{92}$Pd. Gamma rays emitted following the $^{58}$Ni($^{36}$Ar,2$n$)$^{92}$Pd fusion-evaporation reaction were identified using a combination of state-of-the-art high-resolution {gamma}-ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutron-proton coupling scheme, different from the previous prediction. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling) in the ground and low-lying excited states of the heaviest N = Z nuclei. The strong isoscalar neutron- proton correlations in these $N = Z$ nuclei are predicted to have a considerable impact on their level structures, and to influence the dynamics of the stellar rapid proton capture nucleosynthesis process.
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