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Register a new userExtraordinary magnetoresistance in graphite: experimental evidence for the time-reversal symmetry breaking
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The ordinary magnetoresistance (MR) of doped semiconductors is positive and quadratic in a low magnetic field, B, as it should be in the framework of the Boltzmann kinetic theory or in the conventional hopping regime. We observe an unusual highly-anisotropic in-plane MR in graphite, which is neither quadratic nor always positive. In a certain current direction MR is negative and linear in B in fields below a few tens of mT with a crossover to a positive MR at higher fields, while in a perpendicular current direction we observe a giant super-linear and positive MR. These extraordinary MRs are respectively explained by a hopping magneto-conductance via non-zero angular momentum orbitals, and by the magneto-conductance of inhomogeneous media. The linear orbital NMR is a unique signature of the broken time-reversal symmetry (TRS) in graphite. While some local paramagnetic centers could be responsible for the broken TRS, the observed large diamagnetism suggests a more intriguing mechanism of this breaking, involving superconducting clusters with unconventional (chiral) order parameters and spontaneously generated normal-state current loops in graphite.
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We report the magnetic and superconducting properties of locally noncentrosymmetric SrPtAs obtained by muon-spin-rotation/relaxation (muSR) measurements. Zero-field muSR reveals the occurrence of small spontaneous static magnetic fields with the onset of superconductivity. This finding suggests that the superconducting state of SrPtAs breaks time-reversal symmetry. The superfluid density as determined by transverse field muSR is nearly flat approaching T = 0 K proving the absence of extended nodes in the gap function. By symmetry, several superconducting states supporting time-reversal symmetry breaking in SrPtAs are allowed. Out of these, a dominantly d + id (chiral d-wave) order parameter is most consistent with our experimental data.
Spontaneous time-reversal symmetry (TRS) breaking plays an important role in studying strongly correlated unconventional superconductors. When the superconducting gap functions with different pairing symmetries compete, an Ising ($Z_2$) type symmetry breaking occurs due to the locking of the relative phase $Deltatheta_{12}$ via a second order Josephson coupling. The phase locking can take place even in the normal state in the phase fluctuation regime before the onset of superconductivity. If $Deltatheta_{12}=pmfrac{pi}{2}$, then TRS is broken, otherwise, if $Deltatheta_{12}=0$, or, $pi$, rotational symmetry is broken leading to a nematic state. In both cases, the order parameters possess a 4-fermion structure beyond the scope of mean-field theory. We employ an effective two-component $XY$-model assisted by a renormalization group analysis to address this problem. In addition, a quartetting, or, charge-``4e, superconductivity can also occur above $T_c$. Monte-Carlo simulations are performed and the results are in a good agreement with the renormalization group analysis. Our results provide useful guidance for studying novel symmetry breakings in strongly correlated superconductors.
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